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At the fundamental level, full description of light-matter interaction requires quantum treatment of both matter and light. However, for standard light sources generating intense laser pulses carrying quadrillions of photons in a coherent…

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…

Intense extreme-ultraviolet (XUV) pulses enable the investigation of XUV-induced nonlinear processes and are a prerequisite for the development of attosecond pump - attosecond probe experiments. While highly nonlinear processes in the XUV…

Infrared and visible light beams carrying orbital angular momentum (OAM) are currently thoroughly studied for their extremely broad applicative prospects, among which are quantum information, micromachining and diagnostic tools. Here we…

Optics · Physics 2016-08-31 R. Géneaux , A. Camper , T. Auguste , O. Gobert , J. Caillat , R. Taeïb , T. Ruchon

High-order harmonic generation driven by intense extreme ultraviolet (EUV) fields merges quantum optics and attosecond science, giving rise to an appealing route for the generation of coherent EUV and soft X-ray light for high-resolution…

We investigate the generation of even and odd harmonics using an intense laser and a weak second harmonic field. Our theoretical approach is based on solving the saddle-point equations within the Strong Field Approximation. The phase of the…

Quantum Physics · Physics 2015-03-18 J. M. Dahlström , A. L'Huillier , J. Mauritsson

Quantum phenomena such as entanglement can improve fundamental limits on the sensitivity of a measurement probe. In optical interferometry, a probe consisting of $N$ entangled photons provides up to a $\sqrt{N}$ enhancement in phase…

We present a study of photon statistics associated with high-order harmonic generation (HHG) involving one-mode and intermodal correlations of the high harmonic photons. The aim of the paper is to give insight into the nonclassical…

Quantum Physics · Physics 2021-09-15 Ákos Gombkötő , Péter Földi , Sándor Varró

The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion…

Atomic Physics · Physics 2015-09-04 Niranjan Shivaram , Xiao-Min Tong , Henry Timmers , Arvinder Sandhu

We present an innovative beamline for extreme ultraviolet (XUV)-infrared (IR) pump-probe reflection spectroscopy in solids with attosecond temporal resolution. The setup uses an actively stabilized interferometer, where attosecond pulse…

High harmonic generation (HHG) in solids has recently emerged as a powerful all-optical approach for probing material properties and ultrafast electron dynamics in quantum systems. It has been widely applied for studying two-dimensional and…

Optics · Physics 2026-04-28 Eyal Uzner , Ofer Neufeld

Correlated photon pairs, carrying strong quantum correlations, have been harnessed to bring quantum advantages to various fields from biological imaging to range finding. Such inherent non-classical properties support extracting more valid…

Quantum Physics · Physics 2020-06-18 Zhan-Ming Li , Shi-Bao Wu , Jun Gao , Heng Zhou , Zeng-Quan Yan , Ruo-Jing Ren , Si-Yuan Yin , Xian-Min Jin

We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…

Quantum Physics · Physics 2021-06-23 Zhedong Zhang , Tao Peng , Xiaoyu Nie , Girish S. Agarwal , Marlan O. Scully

High harmonic spectra generated in condensed matter carry the fingerprints of sub-cycle electronic motion and the energy structure of the studied system. Here we show that tailoring the waveform of mid-infrared driving light by using a…

The production of pairs of entangled photons simply by focusing a laser beam onto a crystal with a non-linear optical response was used to test quantum mechanics and to open new approaches in imaging. The development of the latter was…

Quantum Physics · Physics 2019-08-09 Paul-Antoine Moreau , Ermes Toninelli , Thomas Gregory , Miles J. Padgett

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

High harmonic generation (HHG) from condensed matter phase holds promise to promote future cutting-edge research in the emerging field of attosecond nanoscopy. The key for the progress of the field relies on the capability of the existing…

Optics · Physics 2021-07-07 Hicham Agueny

Interferometry is a fundamental technique in physics, enabling precise measurements through the interference of waves. High-harmonic generation (HHG) in solids has emerged as a powerful method for probing ultrafast electronic dynamics…

Non-classical and entangled light states are of fundamental interest in quantum mechanics and they are a powerful tool for the emergence of new quantum technologies. The development of methods that can lead to the generation of such light…

Quantum Physics · Physics 2025-03-18 Th. Lamprou , P. Stammer , J. Rivera-Dean , N. Tsatrafyllis , M. F. Ciappina , M. Lewenstein , P. Tzallas