Related papers: Attosecond quantum spectroscopy with entangled pho…
Quantum high-harmonic generation (HHG) is a prominent and growing field of research with potential capabilities of providing high photon-number entangled states of light. However, there is an open debate regarding the theory level required…
High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…
Conventional nonlinear spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the…
The interaction of strong near-infrared (NIR) laser pulses with wide-bandgap dielectrics produces high harmonics in the extreme ultraviolet (XUV) wavelength range. These observations have opened up the possibility of attosecond metrology in…
This perspective introduces attosecond path qubits: measurement-defined two-level subsystems that arise naturally in strong-field physics from the coherent interference of distinguishable quantum pathways. These effective qubits are…
Two-photon processes are crucial in applications like microscopy and microfabrication, but their low cross-section requires intense illumination and limits, e.g., the penetration depth in nonlinear microscopy. Entangled states have been…
High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…
Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…
Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…
Entanglement is a key resource in quantum technologies, enhancing precision and resolution in imaging and sensing by leveraging the cross-correlation of photon pairs. This correlation enables precise time synchronization of photons reaching…
Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to…
Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…
Characterizing the quantum state of intense light fields on sub-cycle timescales remains beyond the reach of existing methods. Here, we show that attosecond streaking provides direct, phase-sensitive access to the quantum properties of the…
Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…
Squeezed light has revolutionized quantum metrology by enhancing interferometry for sensitive applications such as the detection of gravitational waves. Squeezed light has also played a pivotal role in quantum information science with…
The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV)…
Accurately controlling the quantum coherence of photons is pivotal for their applications in quantum sensing and quantum imaging. Here, we propose the utilization of quantum entanglement and local phase manipulation techniques to control…
Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…
The optical phase of the driving field in the process of high harmonic generation and the coherence properties of the harmonics are fundamental concepts in attosecond physics. Here, we consider to drive the process by incoherent classical…
Optical coherence encodes information about the correlations of the electromagnetic field. In combination with quantum optical approaches, it allows for the study of the correlations between photons. Since the pioneering papers of Glauber,…