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High-harmonic generation (HHG) is a strong-field phenomenon that is sensitive to the attosecond dynamics of tunnel ionization and coherent transport of electron-hole pairs in solids. While the foundations of solid HHG have been established,…

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

We analytically describe the strong-field light-electron interaction using a quantized coherent laser state with arbitrary photon number. We obtain a light-electron wave function which is a closed-form solution of the time-dependent…

Atomic Physics · Physics 2017-03-20 I. A. Gonoskov , N. Tsatrafyllis , I. K. Kominis , P. Tzallas

Bridging quantum optics and strong-field physics provides a pathway to explore how quantum light shapes extreme nonlinear light-matter interactions. However, direct characterization of non-classical light at damage-threshold intensities…

Quantum Physics · Physics 2026-02-17 Tsendsuren Khurelbaatar , R. T. Sang , Igor Litvinyuk

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths…

Preparation of nonclassical light with special quantum properties is essential for quantum technologies. High-harmonic generation (HHG) is a process which not only enables the creation of attosecond pulses but also has the potential to…

Quantum Physics · Physics 2026-03-03 Ákos Gombkötő , Péter Ádám , David Theidel , Tamás Kiss

In strong-field physics and attosecond science, intense light induces ultrafast electron dynamics. Such ultrafast dynamics of electrons in matter is at the core of phenomena such as high harmonic generation (HHG), where these dynamics lead…

Entanglement in high-dimensional quantum systems, where one or more degrees of freedom of light are involved, offers increased information capacities and enables new quantum protocols. Here, we demonstrate a functional source of…

The field of attosecond physics has expanded significantly in recent years, yet experimental facilities supporting attosecond pump attosecond probe spectroscopy remain rare. Here, we present a newly constructed beamline for the generation…

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

Two light pulses propagating with ultra-slow group velocities in a coherently prepared atomic gas exhibit dissipation-free nonlinear coupling of an unprecedented strength. This enables a single-photon pulse to coherently control or…

Quantum Physics · Physics 2009-10-31 M. D. Lukin , A. Imamoglu

In recent years nanoscale coherent imaging has emerged as an indispensable imaging modality allowing to surpass the resolution limit given by classical imaging optics. At the same time, attosecond science has experienced enormous progress…

Intense light-matter interaction largely relies on the use of high-power light sources, creating fields comparable to, or even stronger than, the field keeping the electrons bound in atoms. Under such conditions, the interaction induces…

Quantum Physics · Physics 2025-10-23 P. Stammer , J. Rivera-Dean , P. Tzallas , M. F. Ciappina , M. Lewenstein

We propose the generation of attosecond entangled bi-photons in the extreme-ultraviolet regime by two-photon decay of a metastable atomic state as a source similar to spontaneous parametric down-conversion photons. The 1s2s $^1S_0$…

Quantum Physics · Physics 2025-11-25 Yimeng Wang , Siddhant Pandey , Chris H. Greene , Niranjan Shivaram

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

Atomic Physics · Physics 2025-03-31 Xinhua Xie

Entangled photons have the remarkable ability to be more sensitive to signal and less sensitive to noise than classical light. Joint photons can sample an object collectively, resulting in faster phase accumulation and higher spatial…

Optics · Physics 2015-09-04 Chien-Hung Lu , Matthew Reichert , Xiaohang Sun , Jason W. Fleischer

Transient absorption is a very powerful observable in attosecond experiments on atoms, molecules and solids and is frequently used in experiments employing phase-locked few-cycle infrared and XUV laser pulses derived from high harmonic…

Atomic Physics · Physics 2020-08-26 Lorenz Drescher , Marc J. J. Vrakking , Jochen Mikosch

Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…

In the past two decades high-harmonic generation (HHG) has become a key process in ultra-fast science due to the extremely short time-structure of the underlying electron dynamics being imprinted in the emitted harmonic light bursts. After…

Atomic Physics · Physics 2012-01-25 Markus C. Kohler , Thomas Pfeifer , Karen Z. Hatsagortsyan , Christoph H. Keitel