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Ultrafast optical pump - optical probe and optical pump - terahertz probe spectroscopy were performed on vanadium dioxide (VO2) and vanadium sesquioxide (V2O3) thin films over a wide temperature range. A comparison of the experimental data…

Vanadium dioxide, VO2, and its metal-insulator transition at T=340K continues to receive considerable interest. The question whether the physics of the insulating low-temperature phase is dominated by the Mott or the Peierls scenario, i.e.…

Strongly Correlated Electrons · Physics 2008-11-10 Jan M. Tomczak , Silke Biermann

Nonequilibrium systems driven by external energy sources host unexplored physics; yet phase transitions beyond thermal equilibrium remain elusive. Here, we demonstrate that electric current induces structural phase transitions in…

Vanadium dioxide, a well-known Mott insulator, is a highly studied electronic material with promising applications in information processing and storage. While fully crystalline layers exhibit exceptional properties, such as a sharp and…

We report the first application of critical cluster techniques to the Mott metal-insulator transition in vanadium dioxide. We show that the geometric properties of the metallic and insulating puddles observed by scanning near-field infrared…

Strongly Correlated Electrons · Physics 2016-01-27 Shuo Liu , B. Phillabaum , E. W. Carlson , K. A. Dahmen , N. S. Vidhyadhiraja , M. M. Qazilbash , D. N. Basov

We numerically demonstrate a reconfigurable extraordinary terahertz transmission based on a phase-change material of vanadium dioxide (VO2). The proposed hybrid metasurface is composed of an array of subwavelength apertures perforated on a…

Optics · Physics 2026-05-08 S. Hadi Badri , Hadi Soofi , Sanam Saeidnahaei S

We experimentally demonstrate that a thin (~150 nm) film of vanadium dioxide (VO2) deposited on sapphire has an anomalous thermal emittance profile when heated, which arises due to the optical interaction between the film and the substrate…

The single crystal VO2, exihibiting a first-order metal-insulator transition (MIT) at 67.2 degrees C and an insulator-insulator transition (IIT) at ~49.7 degrees C, is grown. From synchrotron-based x-ray microdiffraction analysis, the IIT…

We present {\it ab initio} LDA+DMFT results for the many-particle density of states of $VO_{2}$ on the metallic side of the strongly first-order ($T$-driven) insulator-metal transition. In strong contrast to LDA predictions, there is {\it…

Strongly Correlated Electrons · Physics 2015-06-24 M. S. Laad , L. Craco , E. Müller-Hartmann

The metal-insulator transition (MIT) in vanadium dioxide VO$_2$ due to V-V dimerization has been extensively discussed for decades. While it is widely acknowledged that electron correlations, Peierls instabilities, and molecular orbital…

Strongly Correlated Electrons · Physics 2024-03-12 Shunsuke Kitou , Akitoshi Nakano , Masato Imaizumi , Yuiga Nakamura , Ichiro Terasaki , Taka-hisa Arima

We present a combined density-functional theory and dynamical mean-field theory (DFT+DMFT) study of the full structural phase space of rutile-based vanadium dioxide (VO$_2$), including also the less studied M2 and T phases, using an…

Strongly Correlated Electrons · Physics 2026-03-30 Peter Mlkvik , Nicola A. Spaldin , Claude Ederer

Synchrotron X-ray total scattering studies of structural changes in rutile VO2 at the metal-insulator transition temperature of 340 K reveal that monoclinic and tetragonal phases of VO2 coexist in equilibrium, as expected for a first-order…

Materials Science · Physics 2010-08-10 Serena A. Corr , Daniel P. Shoemaker , Brent C. Melot , Ram Seshadri

Memristors are passive circuit elements which behave as resistors with memory. The recent experimental realization of a memristor has triggered interest in this concept and its possible applications. Here, we demonstrate memristive response…

Strongly Correlated Electrons · Physics 2015-05-13 Tom Driscoll , Hyun-Tak Kim , Byung-Gyu Chae , Massimiliano Di Ventra , D. N. Basov

Vanadium dioxide has been identified as a promising phase-changing material for use in tunable plasmonic devices. In this study, we present a comprehensive modal analysis of single-phase and multi-phase vanadium dioxide nanoparticles.…

We present measurements of the optical spectra on single crystals of spinel-type compound \cis. This material undergoes a sharp metal-insulator transition at 230 K. Upon entering the insulating state, the optical conductivity shows an…

Strongly Correlated Electrons · Physics 2009-11-10 N. L. Wang , G. H. Cao , P. Zheng , G. Li , Z. Fang , T. Xiang , H. Kitazawa , T. Matsumoto

The high-pressure behavior of monoclinic VO$_2$ is revisited by a combination of Raman spectroscopy and X-ray diffraction on a single crystal under hydrostatic conditions at room temperature. A soft mode is observed up to P$_c$ = 13.9(1)…

Strongly Correlated Electrons · Physics 2025-01-14 P. Bouvier , L. Bussmann , D. Machon , I. Breslavetz , G. Garbarino , P. Strobel , V. Dmitriev

Quantum interference can produce a pivotal effective photon-photon interaction, enabling the exploration of various quantum information technologies that beyond the possibilities of classical physics. While such an effective interaction is…

Quantum Physics · Physics 2025-10-21 Chaojie Wang , Xutong Li , Xiuyi Ma , Yuning Zhang , Meng Wu , Weifang Lu , Yuanyuan Chen , Xiubao Sui , Lixiang Chen

An electrical study of thin $VO_{2}$ films in the vicinity of the structural phase transition at $68^{0}C$ shows (a) that the electrical resistance $R$ follows $log (R)$ $\propto$ $-T$ over the $T$-range, $20 < T < 80 ^{0}C$ covering both…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 R. G. Mani , S. Ramanathan

The influence of Coulomb correlation on magnetic and spectral properties in metallic rutile phase of vanadium dioxide is studied by state of the art LDA+DMFT method. Calculation results in strongly correlated metallic state with an…

Strongly Correlated Electrons · Physics 2015-05-18 A. S. Belozerov , A. I. Poteryaev , V. I. Anisimov

The phase diagram of VO$_2$ strained or doped with several trivalent ions consists of four phases; in order of increasing temperatures, three (M1, T and M2) are insulating while the fourth (R), above ~340 K, is metallic. These phases and…

Strongly Correlated Electrons · Physics 2024-03-26 Larisa Patlagan , George M. Reisner , Shani Neyshtadt-Ronel , Yoav Kalcheim , Bertina Fisher