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Resonant inelastic x-ray scattering (RIXS) at the copper K absorption edge has been performed for heavily overdoped samples of La$_{2-x}$Sr$_{x}$CuO$_{4}$ with $x= 0.25$ and 0.30. We have observed the charge transfer and molecular-orbital…

Superconductivity · Physics 2009-11-11 S. Wakimoto , Young-June Kim , Hyunkyung Kim , H. Zhang , T. Gog , R. J. Birgeneau

We develop a framework to evaluate the time-dependent resonant inelastic X-ray scattering (RIXS) signal with the use of non-equilibrium dynamical mean field theory simulations. The approach is based on the solution of a time-dependent…

Strongly Correlated Electrons · Physics 2021-03-24 Martin Eckstein , Philipp Werner

Although orbital degrees of freedom are a factor of fundamental importance in strongly correlated transition metal compounds, orbital correlations and dynamics remain very difficult to access, in particular by neutron scattering. Via a…

Strongly Correlated Electrons · Physics 2015-03-20 Pasquale Marra , Krzysztof Wohlfeld , Jeroen van den Brink

Effective symmetry-based transition operators for resonant inelastic X-ray scattering (RIXS) are derived that show how the scattering between different states depends on the polarization of the incoming and outgoing X-rays. In spherical…

Strongly Correlated Electrons · Physics 2011-06-06 Michel van Veenendaal

We present a formalism for the resonant inelastic x-ray scattering (RIXS) cross section. The resulting compact expression in terms of polarizability matrix elements, particularly lends itself to the implementation in an all-electron…

Materials Science · Physics 2022-08-17 Christian Vorwerk , Francesco Sottile , Claudia Draxl

We discuss the calculation of resonant inelastic x-ray scattering (RIXS) with Xclaim, a multi-plaform code for the calculation of core-hole spectroscopy based on a ligand-field multiplet model. RIXS can be calcuated with a ligand-field…

Strongly Correlated Electrons · Physics 2015-08-05 Javier Fernandez-Rodriguez , Brian Toby , Michel van Veenendaal

Ultrafast optical pulses are an increasingly important tool for controlling quantum materials and triggering novel photo-induced phase transitions. Understanding these dynamic phenomena requires a probe sensitive to spin, charge, and…

Strongly Correlated Electrons · Physics 2020-10-21 Matteo Mitrano , Yao Wang

We develop a formalism to study the Resonant Inelastic X-ray Scattering (RIXS) response in metals based on the diagrammatic expansion for its cross section. The standard approach to the solution of the RIXS problem relies on two key…

Strongly Correlated Electrons · Physics 2019-11-20 A. M. Tsvelik , R. M. Konik , N. V. Prokof'ev , I. S. Tupitsyn

We study the magnetic excitation spectra of resonant inelastic x-ray scattering (RIXS) at the $L$-edge from undoped cuprates beyond the fast collision approximation. We analyse the effect of the symmetry breaking ground state on the RIXS…

Strongly Correlated Electrons · Physics 2015-06-24 Jun-ichi Igarashi , Tatsuya Nagao

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

Materials Science · Physics 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

Resonant inelastic X-ray scattering (RIXS) is a promising technique for obtaining electron-phonon coupling constants. However, the ability to extract these coupling constants throughout the Brillouin zone for crystalline materials remains…

Materials Science · Physics 2018-12-19 Andrey Geondzhian , Keith Gilmore

The real-space multiple-scattering (RSMS) approach is applied to model non-resonant inelastic scattering from deep core electron levels over a broad energy spectrum. This approach is applicable to aperiodic or periodic systems alike and…

Other Condensed Matter · Physics 2009-11-11 J. A. Soininen , A. L. Ankudinov , J. J. Rehr

Entanglement plays a central role in quantum technologies, yet its characterization and control in materials remain challenging. Recent developments in spectrum-based entanglement witnesses have enabled new strategies for quantifying…

Quantum Physics · Physics 2025-12-09 Zecheng Shen , Shuhan Ding , Zijun Zhao , Francesco A. Evangelista , Yao Wang

Resonant inelastic x-ray scattering (RIXS) is a well-established tool for studying electronic, nuclear and collective dynamics of excited atoms, molecules and solids. An extension of this powerful method to a time-resolved probe technique…

Chemical Physics · Physics 2015-11-03 Victor Kimberg , Nina Rohringer

We present a combined oxygen $K$-edge x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) study of the bilayer ruthenate Ca$_3$Ru$_2$O$_7$. Our RIXS experiments on Ca$_3$Ru$_2$O$_7$ were carried out on the…

Strongly Correlated Electrons · Physics 2025-04-01 K. von Arx , F. Forte , M. Horio , V. Granata , Q. Wang , L. Das , Y. Sassa , R. Fittipaldi , C. G. Fatuzzo , O. Ivashko , Y. Tseng , E. Paris , A. Vecchione , T. Schmitt , M. Cuoco , J. Chang

Recent experiments show that indirect resonant inelastic X-ray scattering (RIXS) is a new probe of spin dynamics. Here I derive the cross-section for magnetic RIXS and determine the momentum dependent four-spin correlation function that it…

Strongly Correlated Electrons · Physics 2015-06-25 Jeroen van den Brink

Resonant inelastic x-ray scattering (RIXS) has become a powerful tool in the study of the electronic structure of condensed matter. Although the linewidths of many RIXS features are narrow, the experimental broadening can often hamper the…

Strongly Correlated Electrons · Physics 2012-02-13 J. Laverock , A. R. H. Preston , D. Newby , K. E. Smith , S. B. Dugdale

Resonant inelastic x-ray scattering (RIXS) is an extremely valuable tool for the study of elementary, including magnetic, excitations in matter. Latest developments of this technique mostly aimed at improving the energy resolution and…

Resonant inelastic x-ray scattering (RIXS) tuned for the Cu L edge is a possible tool to detect charge excitations in cuprate superconductors. We theoretically investigate the possibility for observing a collective charge excitation by the…

Strongly Correlated Electrons · Physics 2015-08-03 Takami Tohyama , Kenji Tsutsui , Michiyasu Mori , Shigetoshi Sota , Seiji Yunoki