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We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

Strongly Correlated Electrons · Physics 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš

In the study of dynamic charge order correlations in the cuprates, most high energy-resolution resonant inelastic x-ray scattering (RIXS) measurements have focused on momenta along the high-symmetry directions of the copper oxide plane.…

Quasi-one-dimensional systems exhibit many-body effects elusive in higher dimensions. A prime example is spin-orbital separation, which has been measured by resonant inelastic X-ray scattering (RIXS) in Sr$_2$CuO$_3$. Here, we theoretically…

Strongly Correlated Electrons · Physics 2022-10-03 Aaron Müller , Francesco Grandi , Martin Eckstein

We determine how the elementary excitations of iridium-oxide materials, which are dominated by a strong relativistic spin-orbit coupling, appear in Resonant Inelastic X-ray Scattering (RIXS). Whereas the RIXS spectral weight at the L2 x-ray…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Giniyat Khaliullin , Jeroen van den Brink

I present a tractable theory for the Resonant Inelastic X-ray Scattering (RIXS) spectral function of magnons. The low-energy transition operator is written as a product of local spin operators times fundamental x-ray absorption spectra.…

Strongly Correlated Electrons · Physics 2011-07-05 M. W. Haverkort

Continued improvement of the energy resolution of resonant inelastic x-ray scattering (RIXS) spectrometers is crucial for fulfilling the potential of this technique in the study of electron dynamics in materials of fundamental and…

Instrumentation and Detectors · Physics 2017-09-11 Jungho Kim , D. Casa , Ayman Said , Richard Krakora , B. J. Kim , Elina Kasman , Xianrong Huang , T. Gog

We present an ab initio study of neutral core and valence electronic excitations in {\alpha}-Al2O3 by solving the Bethe-Salpeter equation (BSE) of many-body perturbation theory within an all-electron framework. Calculated spectra at the Al…

Materials Science · Physics 2024-01-26 M. Laura Urquiza , Matteo Gatti , Francesco Sottile

We analyze resonant inelastic x-ray scattering (RIXS) at the Cu K edge in a typical orbital-ordered compound KCuF3 on the basis of a microscopic theory. Spectral shape and its dependence on polarization direction and momentum transfer of…

Strongly Correlated Electrons · Physics 2014-06-20 Takuji Nomura

Resonant inelastic x-ray scattering (RIXS) has become a very powerful experimental technique to probe a broad range of intrinsic elementary excitations, for example, from low energy phonons and (bi-)magnons to high energy $d$-$d$,…

Strongly Correlated Electrons · Physics 2019-06-20 Y. L. Wang , G. Fabbris , M. P. M. Dean , G. Kotliar

Imperfections in the surface of intracavity elements of an optical ring resonator can scatter light from one mode into the counterpropagating mode. The phase-locking of the cavity modes induced by this backscattering is a well-known example…

Optics · Physics 2009-11-13 G. Krenz , S. Bux , S. Slama , C. Zimmermann , Ph. W. Courteille

Coherent control of quantum dynamics is key to a multitude of fundamental studies and applications alike. In the visible or longer-wavelength domains, near-resonant light fields have become the primary tool to control electron dynamics.…

Using a model Hamiltonian, we discuss how we could interpret data obtained from transition metal $K$-edge resonant inelastic x-ray scattering (RIXS) experiments. By analyzing the creation of valence excitations from the screening of the…

Materials Science · Physics 2008-08-08 K. H. Ahn , A. J. Fedro , Michel van Veenendaal

Recent advancements in ultrashort and intense X-ray sources have enabled the utilisation of resonant inelastic X-ray scattering (RIXS) as a probing technique for monitoring photoinduced dynamics in molecular systems. To account for dynamic…

Chemical Physics · Physics 2024-03-19 Antonia Freibert , David Mendive-Tapia , Oriol Vendrell , Nils Huse

Despite significant progress in resonant inelastic x-ray scattering (RIXS) experiments on cuprates at the Cu L-edge, a theoretical understanding of the cross-section remains incomplete in terms of elementary excitations and the connection…

Strongly Correlated Electrons · Physics 2016-05-16 Chunjing Jia , Krzysztof Wohlfeld , Yao Wang , Brian Moritz , Thomas P. Devereaux

Ru M$_3$-edge resonant inelastic x-ray scattering (RIXS) measurements of RuCl$_3$ with 27 meV resolution reveals a spin-orbit exciton without noticeable splitting. We extract values for the spin-orbit coupling constant ($\lambda=154\pm2$…

Strongly Correlated Electrons · Physics 2020-01-29 Blair W Lebert , Subin Kim , Valentina Bisogni , Ignace Jarrige , Andi M Barbour , Young-June Kim

This paper makes a comparison between x-ray absorption (XAS) and resonant inelastic x-ray scattering (RIXS) in the rare earths. Atomic calculations are given for 2p -> 4f and 2p -> 5d XAS. The latter calculation includes the contraction and…

Materials Science · Physics 2009-10-30 Michel van Veenendaal , Robert Benoist

We describe an ab initio approach to simulate L-edge X-ray absorption (XAS) and 2p3d resonant inelastic X-ray scattering (RIXS) spectroscopies. We model the strongly correlated electronic structure within a restricted active space and…

Chemical Physics · Physics 2023-06-01 Seunghoon Lee , Huanchen Zhai , Garnet Kin-Lic Chan

Resonant inelastic X-ray scattering (RIXS) has become an important scientific tool. Nonetheless, conventional high-resolution RIXS measurements (<100 meV), especially in the soft x-ray range, require large and low-throughput grating…

Materials Science · Physics 2020-06-22 Daniel J. Higley , Hirohito Ogasawara , Sioan Zohar , Georgi L. Dakovski

We theoretically analyze the intensity of the resonant inelastic X-ray scattering (RIXS) based on Ansatz that the electron is fractionalized into two components. By fitting the angle resolved photoemission spectroscopy (ARPES) data of a…

Strongly Correlated Electrons · Physics 2021-07-26 Masatoshi Imada

We study theoretically resonant inelastic x-ray scattering (RIXS) at the Cu $L_3$-edge in a typical parent compound of high-$T_c$ cuprate superconductors La$_2$CuO$_4$ on the basis of a detailed electronic band structure. We construct a…

Strongly Correlated Electrons · Physics 2015-08-20 Takuji Nomura