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Related papers: Electronic Bridge processes in $^{229}$Th-doped Li…

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The electronic defect states resulting from doping $^{229}$Th in CaF$_2$ offer a unique opportunity to excite the nuclear isomeric state $^{229m}$Th at approximately 8 eV via electronic bridge mechanisms. We consider bridge schemes…

When Th nuclei are doped in CaF$_2$ crystals, a set of electronic defect states appears in the crystal bandgap which would otherwise provide complete transparency to vacuum-ultraviolet radiation. The coupling of these defect states to the 8…

An alternative method to determine the excitation energy of the $~^{229\rm{m}}\rm{Th}$ isomer via the laser-induced electronic bridge is investigated theoretically. In the presence of an optical or ultra-violet laser at energies that…

Atomic Physics · Physics 2018-03-13 Pavlo V. Bilous , Ekkehard Peik , Adriana Pálffy

The 8.4 eV transition in the $^{229}$Th nucleus is the basis for a high-precision nuclear clock with exceptional sensitivity to new physics effects. We have identified several cases in the Th$^+$ ion where electronic excitations closely…

Atomic Physics · Physics 2025-04-29 V. A. Dzuba , V. V. Flambaum

The excitation of the 8 eV $^{229m}$Th isomer through the electronic bridge mechanism in highly charged ions is investigated theoretically. By exploiting the rich level scheme of open $4f$ orbitals and the robustness of highly charged ions…

We consider the excitation of the nuclear transition ^{229g}Th - ^{229m}Th near 7.6 eV in singly ionized thorium via an electronic bridge process. The process relies on the excitation of the electron shell by two laser photons whose sum…

Atomic Physics · Physics 2010-10-27 S. G. Porsev , V. V. Flambaum , E. Peik , Chr. Tamm

The nuclear transition between the ground and the low-energy isomeric state in the ^{229}Th nucleus is of interest due to its high sensitivity to a hypothetical temporal variation of the fundamental constants and a possibility to build a…

Atomic Physics · Physics 2021-05-04 S. G. Porsev , C. Cheung , M. S. Safronova

Electronic bridge excitation of the 76 eV nuclear isomeric state in $^{235}$U is shown to be strongly enhanced in the U$^{7+}$ ion, potentially enabling laser excitation of this nucleus. This is because the electronic spectrum has a very…

Atomic Physics · Physics 2019-01-08 J. C. Berengut

We investigate the deexcitation of the $^{229}$Th nucleus via the excitation of an electron. Detailed calculations are performed for the enhancement of the nuclear decay width due to this so called electron bridge (EB) compared to the…

Atomic Physics · Physics 2018-03-14 Robert A. Müller , Andrey V. Volotka , S. Fritzsche , A. Surzhykov

We have studied the effect of atomic electrons on the nuclear transition from the isomeric {229m}Th state to the ground {229g}Th state in {229}Th+ due to the electronic bridge process. The exact value of the nuclear transition frequency is…

Atomic Physics · Physics 2014-11-20 S. G. Porsev , V. V. Flambaum

The 229Th nucleus possesses a unique low-frequency transition at 8.4 eV, which is being considered for the development of an extremely accurate nuclear clock. We investigate an electronic bridge process in the Th III ion, where nuclear…

Atomic Physics · Physics 2025-05-15 V. A. Dzuba , V. V. Flambaum

We have considered an effect of atomic electrons due to the electronic bridge process on the nuclear $^{229m}$Th -- $^{229g}$Th transition in ^{229}$Th$^{3+}$. Based on a recent experimental result we assumed the energy difference between…

Atomic Physics · Physics 2010-04-29 S. G. Porsev , V. V. Flambaum

For the isotope $^{229}$Th we investigate the possibility of two-photon laser spectroscopy of the nuclear clock transition (148.38 nm) using intense monochromatic laser field at twice the wavelength (296.76 nm). Our estimates show that due…

Thorium-doped LiCaAlF$_6$ and LiSrAlF$_6$ (Th:LiCAF and Th:LiSAF) are promising crystals for a solid-state nuclear clock based on the 8 eV transition in $^{229}$Th; however, their complex crystal structures complicate understanding the…

Materials Science · Physics 2026-01-13 Martin Pimon , Tobias Kirschbaum , Thorsten Schumm , Adriana Pálffy , Andreas Grüneis

The $^{229}$Th nucleus has a unique transition at only 8 eV which could be used for a novel nuclear clock. We investigate theoretically the prospects of driving this transition with vortex light beams carrying orbital angular momentum.…

Atomic Physics · Physics 2024-04-22 Tobias Kirschbaum , Thorsten Schumm , Adriana Pálffy

We have recently described a novel method for the construction of a solid-state optical frequency reference based on doping $^{229}$Th into high energy band-gap crystals. Since nuclear transitions are far less sensitive to environmental…

Thorium-229 possesses the lowest nuclear first excited state with an energy of about 8 eV. The extremely narrow linewidth of the nuclear first excited state with the uncertainty of 53 THz prevents the direct laser excitation and the…

Atomic Physics · Physics 2024-05-14 Lin Li , Zi Li , Chen Wang , Wen-Ting Gan , Xia Hua , Xin Tong

Building on recent advances of the embedded cluster approach combined with multiconfigurational theory, this work investigates the electronic states in thorium-doped CaF2 crystals. Th:CaF2 is currently establishing as a promising material…

Materials Science · Physics 2024-10-15 Kamil Nalikowski , Valera Veryazov , Kjeld Beeks , Thorsten Schumm , Marek Krosnicki

After nearly fifty years of searching, the vacuum ultraviolet $^{229}$Th nuclear isomeric transition has recently been directly laser excited [1,2] and measured with high spectroscopic precision [3]. Nuclear clocks based on this transition…

LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that…

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