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We describe a novel approach to directly measure the energy of the narrow, low-lying isomeric state in $^{229}$Th. Since nuclear transitions are far less sensitive to environmental conditions than atomic transitions, we argue that the…

Atomic Physics · Physics 2010-02-09 Wade G. Rellergert , D. DeMille , R. R. Greco , M. P. Hehlen , J. R. Torgerson , Eric R. Hudson

A comprehensive theoretical study of direct laser excitation of a nuclear state based on the density matrix formalism is presented. The nuclear clock isomer $^{229\text{m}}$Th is discussed in detail, as it could allow for direct laser…

Conical intersections are crossing points or lines between two or more adiabatic electronic potential energy surfaces in the multi-dimensional coordinate space of colliding atoms and molecules. Conical intersections and corresponding…

Atomic Physics · Physics 2023-04-19 Hui Li , Ming Li , Alexander Petrov , Eite Tiesinga , Svetlana Kotochigova

The 8 eV first nuclear excited state in $^{229}$Th is a candidate for implementing an nuclear clock. Doping $^{229}$Th into ionic crystals such as CaF$_2$ is expected to suppress non-radiative decay, enabling nuclear spectroscopy and the…

Electron assisted neutron exchange process in solid state environment is investigated. It is shown that if a metal is irradiated with free electrons then the $e+$ $_{Z}^{A_{1}}X+$ $_{Z}^{A_{2}}X\rightarrow e^{\prime }+$ $%_{Z}^{A_{1}-1}X+$…

General Physics · Physics 2017-01-25 Péter Kálmán , Tamás Keszthelyi

The ability to design quantum systems that decouple from environmental noise sources is highly desirable for development of quantum technologies with optimal coherence. The chemical tunability of electronic states in magnetic molecules…

The formation and field-induced switching of defect dipoles in acceptor doped lead titanate is described by a kinetic model representing an extension of the well established Arlt-Neumann model [Ferroelectrics {\bf 76}, 303 (1987)]. Energy…

Materials Science · Physics 2013-11-20 Paul Erhart , Petra Träskelin , Karsten Albe

According to the Schiff theorem an external electric field vanishes at atomic nucleus in a neutral atom, i.e. it is completely shielded by electrons. This makes a nuclear electric dipole moment (EDM) unobservable. In this paper an extension…

Atomic Physics · Physics 2018-10-10 V. V. Flambaum

The isotope $^{229}$Th is the only nucleus known to possess an excited state $^{229m}$Th in the energy range of a few electron volts, a transition energy typical for electrons in the valence shell of atoms, but about four orders of…

We propose a simple approach to measure the energy of the few-eV isomeric state in Th-229. To this end, U-229 nuclei are doped into VUV-transparent crystals, where they undergo alpha decay into Th-229, and, with a probability of 2%,…

Nuclear Experiment · Physics 2016-08-11 Simon Stellmer , Matthias Schreitl , Georgy Kazakov , Johannes Sterba , Thorsten Schumm

Solid-state $^{229}$Th nuclear clocks are set to provide new opportunities for precision metrology and fundamental physics. Taking advantage of a nuclear transition's inherent low sensitivity to its environment, orders of magnitude more…

Nuclei with static intrinsic octupole deformation or a soft octupole vibrational mode lead to strongly enhanced collective nuclear Schiff? moments. Interaction between electrons and these Schiff moments produce enhanced time reversal (T)…

Nuclear Theory · Physics 2020-01-15 V. V. Flambaum , H. Feldmeier

We report the results of a direct search for the $^{229}$Th ($I^{p} = 3/2^+\leftarrow 5/2^+$) nuclear isomeric transition, performed by exposing $^{229}$Th-doped LiSrAlF$_6$ crystals to tunable vacuum-ultraviolet synchrotron radiation and…

The results of experimental studies of the low-energy isomeric state in the $^{229}$Th nucleus are presented. The work is consisted of several stages. During the first stage $^{229}$Th nuclei were excited with the inverse internal…

We explore the thermoelectric properties of gold atomic chains bridging gold electrodes by means of \textit{ab initio} and semi-empirical calculations, and heuristic reasoning. We predict the thermoelectric voltage induced by a temperature…

Mesoscale and Nanoscale Physics · Physics 2018-09-28 Alireza Saffarzadeh , Firuz Demir , George Kirczenow

The proposal for the development of a nuclear optical clock has triggered a multitude of experimental and theoretical studies. In particular the prediction of an unprecedented systematic frequency uncertainty of about $10^{-19}$ has…

Atomic Physics · Physics 2020-11-10 Lars von der Wense , Benedict Seiferle

While it is well established that elevated temperatures can induce surface roughening of metal surfaces, the effect of a high electric field on the atomic structure at ambient temperature has not been investigated in detail. Here we show…

We consider the prototypical deuterium-tritium fusion reaction. At intermediate initial kinetic energies (in the keV regime), a major bottle-neck of this reaction is the Coulomb barrier between the nuclei, which is overcome by tunneling.…

Nuclear Theory · Physics 2019-10-30 Friedemann Queisser , Ralf Schützhold

Previously we proposed a new approach of exciting the $^{229}$Th nucleus using laser-driven electron recollision [W. Wang et al., Phys. Rev. Lett. 127, 052501 (2021)]. The current article is aimed to elaborate the method by explaining…

Atomic Physics · Physics 2022-08-15 Xu Wang

We investigate theoretically a nuclear excitation mechanism involving absorption of non-resonant photons leveraged by the coupling to the atomic shell. The nuclear non-resonant photoexcitation is assisted by electron recombination which…

Nuclear Theory · Physics 2026-04-28 Nan Xue , Zuoye Liu , Ziwen Li , Adriana Pálffy , Jianmin Yuan , Yuanbin Wu , Xiangjin Kong , Yu-Gang Ma