English

Laser excitation of the $^{229}$Th nuclear isomeric transition in a solid-state host

Atomic Physics 2024-04-19 v1 Nuclear Experiment

Abstract

LiSrAlF6_6 crystals doped with 229^{229}Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that produces red-shifted fluorescence that decays with a timescale of a few seconds. The second is a narrow, laser-linewidth-limited spectral feature at 148.38219(4)stat(20)sys148.38219(4)_{\textrm{stat}}(20)_{\textrm{sys}} nm (2020407.3(5)stat(30)sys2020407.3(5)_{\textrm{stat}}(30)_{\textrm{sys}} GHz) that decays with a lifetime of 568(13)stat(20)sys568(13)_{\textrm{stat}}(20)_{\textrm{sys}} s. This feature is assigned to the excitation of the 229^{229}Th nuclear isomeric state, whose energy is found to be 8.355733(2)stat(10)sys8.355733(2)_{\textrm{stat}}(10)_{\textrm{sys}} eV in 229^{229}Th:\thor:LiSrAlF6_6.

Keywords

Cite

@article{arxiv.2404.12311,
  title  = {Laser excitation of the $^{229}$Th nuclear isomeric transition in a solid-state host},
  author = {R. Elwell and Christian Schneider and Justin Jeet and J. E. S. Terhune and H. W. T. Morgan and A. N. Alexandrova and H. B. Tran Tan and Andrei Derevianko and Eric R. Hudson},
  journal= {arXiv preprint arXiv:2404.12311},
  year   = {2024}
}

Comments

Submitted to Physical Review Letters on March 25, 2024