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Recently, $\alpha$-$\textrm{RuCl}_3$ has attracted much attention as a possible material realization of the honeycomb Kitaev model, which may stabilize a quantum-spin-liquid state. Compared to extensive studies on its magnetic properties,…

Mott insulators with strong spin-orbit coupling display a strongly anisotropic response to applied magnetic fields. This applies in particular to Kitaev materials, with $\alpha$-RuCl$_3$ and Na$_2$IrO$_3$ representing two important…

Strongly Correlated Electrons · Physics 2020-10-06 Eric C. Andrade , Lukas Janssen , Matthias Vojta

The Mott insulator $\alpha$-RuCl$_3$ has generated great interest in the community due to its possible field-induced Kitaev quantum spin liquid state. Despite enormous effort spent trying to obtain the form of the low energy Hamiltonian,…

Quantum spin liquid involves fractionalized quasipariticles such as spinons and visons. They are expressed as itinerant Majorana fermions and $Z_2$ fluxes in the Kitaev model with bond-dependent exchange interactions on a honeycomb spin…

Strongly Correlated Electrons · Physics 2020-02-05 Y. Nagai , T. Jinno , Y. Yoshitake , J. Nasu , Y. Motome , M. Itoh , Y. Shimizu

Anisotropic low-temperature properties of the cubic spinel helimagnet ZnCr2Se4 in the single-domain spin-spiral state are investigated by a combination of neutron scattering, thermal conductivity, ultrasound velocity, and dilatometry…

Compounds of transition metal ions with strong spin-orbit coupling recently attracted attention due to the possibility to host frustrated bond-dependent anisotropic magnetic interactions. In general, such interactions lead to complex phase…

Strongly Correlated Electrons · Physics 2019-02-21 Juraj Rusnačko , Dorota Gotfryd , Jiří Chaloupka

Magnetic properties of the substitution series Ru$_{1-x}$Cr$_x$Cl$_3$ were investigated to determine the evolution from the anisotropic Kitaev magnet $\alpha$-RuCl$_3$ with $J_{\rm eff} = 1/2$ magnetic Ru$^{3+}$ ions to the isotropic…

Strongly Correlated Electrons · Physics 2019-07-02 G. Bastien , M. Roslova , M. H. Haghighi , K. Mehlawat , J. Hunger , A. Isaeva , T. Doert , M. Vojta , B. Büchner , A. U. B. Wolter

We present high-resolution measurements of the thermal expansion and the magnetostriction of TlCuCl$_{3}$ which shows field-induced antiferromagnetic order. We find pronounced anomalies in the field and temperature dependence of different…

Strongly Correlated Electrons · Physics 2009-11-10 N. Johannsen , A. Vasiliev , A. Oosawa , H. Tanaka , T. Lorenz

Polarized neutron scattering experiments reveal the anisotropy of magnetic correlations in the candidate Kitaev material $\alpha$-RuCl$_3$. The anisotropy of the inelastic response at the magnetic Bragg positions is just opposite to the…

Strongly Correlated Electrons · Physics 2025-09-10 Markus Braden , Xiao Wang , Alexandre Bertin , Paul Steffens , Yixi Su

Recent experiments reveal that the honeycomb ruthenium trichloride {\alpha}-RuCl3 is a prime candidate of the Kitaev quantum spin liquid (QSL). However, there is no theoretical model which can properly describe its experimental dynamical…

Strongly Correlated Electrons · Physics 2017-08-16 Y. S. Hou , H. J. Xiang , X. G. Gong

We present comprehensive inelastic neutron spectroscopic maps of the magnetic field-induced disordered phase of the Kitaev quantum spin liquid candidate material $\alpha$-RuCl$_3$. For fields along both in-plane high-symmetry directions we…

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

Strongly Correlated Electrons · Physics 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

$^7$Li nuclear magnetic resonance (NMR) and terahertz (THz) spectroscopies are used to probe magnetic excitations and their field dependence in the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$. Spin-lattice relaxation rate ($1/T_1$)…

Strongly Correlated Electrons · Physics 2020-06-16 M. Majumder , M. Prinz-Zwick , S. Reschke , A. Zubtsovskii , T. Dey , F. Freund , N. Büttgen , A. Jesche , I. Kézsmárki , A. A. Tsirlin , P. Gegenwart

Spin $\frac{1}{2}$ honeycomb materials have gained substantial interest due to their exotic magnetism and possible application in quantum computing. However, in all current materials out-of-plane interactions are interfering with the…

We present time-resolved magneto-optical spectroscopy on the magnetic Mott-Hubbard-insulating Kitaev spin liquid candidate $\alpha$-RuCl$_3$ to investigate the nonequilibrium dynamics of its antiferromagnetically ordered zigzag groundstate…

The local magnetic properties of Yb$^{3+}$ in the layered honeycomb material YbCl$_{3}$ were investigated by electron spin resonance on single crystals. For in-plane and out-of-plane field orientations the $g$-factor shows a clear…

Strongly Correlated Electrons · Physics 2023-08-15 Jörg Sichelschmidt , Ellen Häußler , Ekaterina Vinokurova , M. Baenitz , Thomas Doert

The spin-orbit assisted Mott insulator $\alpha$-RuCl3 is proximate to the coveted quantum spin liquid (QSL) predicted by the Kitaev model. In the search for the pure Kitaev QSL, reducing the dimensionality of this frustrated magnet by…

A pressure-induced collapse of magnetic ordering in $\beta$-Li$_2$IrO$_3$ at $P_m\sim1.5- 2$ GPa has previously been interpreted as evidence for possible emergence of spin liquid states in this hyperhoneycomb iridate, raising prospects for…

We present magnetization measurements carried out on polycrystalline and single-crystalline samples of $\alpha$-Li$_2$IrO$_3$ under hydrostatic pressures up to 2 GPa and establish the temperature-pressure phase diagram of this material. The…

Substitution effects of Os for Ru in {\alpha}-RuCl3 are investigated in a wide composition range of 0 =< x =< 0.67 in Ru1-xOsxCl3 by X-ray and electron diffraction, magnetic susceptibility, heat capacity, and Raman spectroscopy…