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We investigate the phononic in-plane longitudinal low-temperature thermal conductivity kappa_ab of the Kitaev quantum magnet alpha-RuCl3 for large in-plane magnetic fields up to 33 T. Our data reveal for fields larger than the critical…

We study the self-energy of phonons, magnetoelastically coupled to the two-dimensional Kitaev spin-model on the honeycomb lattice. Fractionalization of magnetic moments into mobile Majorana matter and a static $\mathbb{Z}_{2}$ gauge field…

Strongly Correlated Electrons · Physics 2020-01-15 Alexandros Metavitsiadis , Wolfram Brenig

We examine the role of spin-orbit coupling in the electronic structure of $\alpha$-RuCl3, in which Ru ions in 4d5 configuration form a honeycomb lattice. The measured optical spectra exhibit a clear optical gap and excitations within the…

Strongly Correlated Electrons · Physics 2014-08-06 K. W. Plumb , J. P. Clancy , L. Sandilands , V. Vijay Shankar , Y. F. Hu , K. S. Burch , Hae-Young Kee , Young-June Kim

The Kitaev model predicts that quantum spin liquids (QSLs) will form at low temperatures under certain special conditions, and materials hosting the QSL state are frequently sought. The layered honeycomb lattice material {\alpha}-RuCl3 has…

Materials Science · Physics 2022-01-24 Danrui Ni , Xin Gui , Kelly M. Powderly , R. J. Cava

Single-crystal x-ray diffraction studies with synchrotron radiation on the honeycomb iridate $\alpha$-Li$_{2}$IrO$_{3}$ reveal a pressure-induced structural phase transition with symmetry lowering from monoclinic to triclinic at a critical…

Maximizing the ratio between Kitaev and residual Heisenberg interactions is a major goal in nowadays research on Kitaev-Heisenberg quantum magnets. Here we investigate Kitaev-Heisenberg exchange in a recently discovered crystalline phase of…

Strongly Correlated Electrons · Physics 2023-12-15 Pritam Bhattacharyya , Liviu Hozoi , Quirin Stahl , Jochen Geck , Nikolay A. Bogdanov

We present magnetization measurements on polycrystalline $\beta$-Li$_2$IrO$_3$ under hydrostatic pressures up to 3~GPa and construct the temperature-pressure phase diagram of this material. Our data confirm that magnetic order breaks down…

Strongly Correlated Electrons · Physics 2021-10-26 Bin Shen , Anton Jesche , Maximilian L. Seidler , Friedrich Freund , Philipp Gegenwart , Alexander A. Tsirlin

The insulating ferrimagnet Cu2OSeO3 shows a rich variety of phases such as skyrmion lattice and helical magnetism controlled by interplay of different exchange interactions which can be tuned by external pressure. In this work we have…

We derive the microscopic spin Hamiltonian for rhombohedral CrI$_3$ using extensive first-principles density functional theory (DFT) calculations which incorporate spin-orbit coupling and Hubbard U. Our calculations indicate a dominant…

Spin waves in the zigzag ordered state on a honeycomb lattice are investigated within a Hubbard model with spin-dependent hopping terms. Roles of the emergent Kitaev, Heisenberg, Dzyaloshinskii-Moriya, and symmetric-off-diagonal spin…

Strongly Correlated Electrons · Physics 2019-03-12 Shubhajyoti Mohapatra , Avinash Singh

Novel ground states might be realized in honeycomb lattices with strong spin-orbit coupling. Here we study the electronic structure of ${\alpha}$-RuCl$_3$, in which the Ru ions are in a d5 configuration and form a honeycomb lattice, by…

Strongly Correlated Electrons · Physics 2016-09-21 A. Koitzsch , C. Habenicht , E. Mueller , M. Knupfer , B. Buechner , H. Kandpal , J. van den Brink , D. Nowak , A. Isaeva , Th. Doert

The excitations in the Kitaev spin liquid (KSL) can be described by Majorana fermions, which have characteristic field dependence of bulk gap and topological edge modes. In the high-field state of layered honeycomb magnet $\alpha$-RuCl$_3$,…

Strongly Correlated Electrons · Physics 2024-03-13 K. Imamura , Y. Mizukami , O. Tanaka , R. Grasset , M. Konczykowski , N. Kurita , H. Tanaka , Y. Matsuda , M. G. Yamada , K. Hashimoto , T. Shibauchi

The Kitaev spin liquid, a ground state of the bond-dependent Kitaev model in a honeycomb lattice has been a centre of attraction, since a microscopic theory to realize such an interaction in solid-state materials was discovered. A challenge…

Strongly Correlated Electrons · Physics 2022-05-20 Jiefu Cen , Hae-Young Kee

Frustrated magnets with strong spin-orbit coupling promise to host topological states of matter, with fractionalized excitations and emergent gauge fields. Kitaev's proposal for a honeycomb-lattice Majorana spin liquid has triggered an…

Strongly Correlated Electrons · Physics 2021-05-19 P. Lampen-Kelley , L. Janssen , E. C. Andrade , S. Rachel , J. -Q. Yan , C. Balz , D. G. Mandrus , S. E. Nagler , M. Vojta

We propose a theoretical model for a gapless spin liquid phase that may have been observed in a recent experiment on $\mathrm{H_3Li Ir_2 O_6}$. Despite the insulating and non-magnetic nature of the material, the specific heat coefficient…

Strongly Correlated Electrons · Physics 2018-03-29 Kevin Slagle , Wonjune Choi , Li Ern Chern , Yong Baek Kim

We report high-pressure magnetization and $^{35}$Cl NMR studies on $\alpha$-RuCl$_3$ with pressure up to 1.5~GPa. At low pressures, the magnetic ordering is identified by both the magnetization data and the NMR data, where the $T_N$ shows a…

Strongly Correlated Electrons · Physics 2017-12-06 Y. Cui , J. Zheng , K. Ran , Jinsheng Wen , Zhengxin Liu , B. Liu , Wenan Guo , Weiqiang Yu

Intensive studies of the interplay between spin-orbit coupling (SOC) and electronic correlations in transition metal compounds have recently been undertaken. In particular, $j_{\rm eff}$ = 1/2 bands on a honeycomb lattice provide a pathway…

Strongly Correlated Electrons · Physics 2015-06-24 Heung-Sik Kim , V. Vijay Shankar , Andrei Catuneanu , Hae-Young Kee

The low-temperature magnetic phases in the layered honeycomb lattice material $\alpha$-RuCl$_3$ have been studied as a function of in-plane magnetic field. In zero field this material orders magnetically below 7 K with so-called zigzag…

Strongly Correlated Electrons · Physics 2017-06-07 J. A. Sears , Y. Zhao , Z. Xu , J. W. Lynn , Young-June Kim

We use an exact numerical diagonalization method to calculate the dynamical spin structure factors (DSFs) of three ab-initio models and one ab-initio-guided model for a honeycomb-lattice magnet $\alpha$-RuCl$_3$. We also use thermal pure…

Strongly Correlated Electrons · Physics 2019-06-07 Takafumi Suzuki , Sei-ichiro Suga

The honeycomb compound $\alpha$-RuCl$_3$ is widely discussed as a proximate Kitaev spin-liquid material. This scenario builds on spin-orbit entangled $j = 1/2$ moments arising for a $t_{2g}^5$ electron configuration with strong spin-orbit…

Strongly Correlated Electrons · Physics 2020-10-21 P. Warzanowski , N. Borgwardt , K. Hopfer , T. C. Koethe , P. Becker , V. Tsurkan , A Loidl , M. Hermanns , P. H. M. van Loosdrecht , M. Grüninger
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