English

Field evolution of low-energy excitations in the hyperhoneycomb magnet $\beta$-Li$_2$IrO$_3$

Strongly Correlated Electrons 2020-06-16 v2

Abstract

7^7Li nuclear magnetic resonance (NMR) and terahertz (THz) spectroscopies are used to probe magnetic excitations and their field dependence in the hyperhoneycomb Kitaev magnet β\beta-Li2_2IrO3_3. Spin-lattice relaxation rate (1/T11/T_1) measured down to 100\,mK indicates gapless nature of the excitations at low fields (below Hc2.8H_c\simeq 2.8\,T), in contrast to the gapped magnon excitations found in the honeycomb Kitaev magnet α\alpha-RuCl3_3 at zero applied magnetic field. At higher temperatures in β\beta-Li2_2IrO3_3, 1/T11/T_1 passes through a broad maximum without any clear anomaly at the N\'eel temperature TN38T_N\simeq 38\,K, suggesting the abundance of low-energy excitations that are indeed observed as two peaks in the THz spectra, both correspond to zone-center magnon excitations. At higher fields (above HcH_c), an excitation gap opens, and a re-distribution of the THz spectral weight is observed without any indication of an excitation continuum, in contrast to α\alpha-RuCl3_3 where an excitation continuum was reported.

Keywords

Cite

@article{arxiv.1910.03251,
  title  = {Field evolution of low-energy excitations in the hyperhoneycomb magnet $\beta$-Li$_2$IrO$_3$},
  author = {M. Majumder and M. Prinz-Zwick and S. Reschke and A. Zubtsovskii and T. Dey and F. Freund and N. Büttgen and A. Jesche and I. Kézsmárki and A. A. Tsirlin and P. Gegenwart},
  journal= {arXiv preprint arXiv:1910.03251},
  year   = {2020}
}

Comments

6 pages, 4 figures