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We present a thorough experimental study of the three-dimensional hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$, using a combination of inelastic neutron scattering (INS), time-domain THz spectroscopy, and heat capacity measurements.…

We present high-pressure (2 GPa) $^7$Li nuclear magnetic resonance (NMR) measurements on single crystals of the hyper-honeycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$. The spectra show evidence for a structural phase transition around 200 K…

Strongly Correlated Electrons · Physics 2025-12-16 Aimé Verrier , Vikram Nagarajan , Louis-Thomas Gendron , James G. Analytis , Jeffrey A. Quilliam

The layered honeycomb iridate $\alpha$-Li$_2$IrO$_3$ displays an incommensurate magnetic structure with counterrotating moments on nearest-neighbor sites, proposed to be stabilized by strongly-frustrated anisotropic Kitaev interactions…

Strongly Correlated Electrons · Physics 2019-03-06 Sungkyun Choi , S. Manni , J. Singleton , C. V. Topping , T. Lancaster , S. J. Blundell , D. T. Adroja , V. Zapf , P. Gegenwart , R. Coldea

Detailed magnetization, specific heat, and $^7$Li nuclear magnetic resonance (NMR) measurements on single crystals of the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$ are reported. At high temperatures, {\cred anisotropy of the…

Strongly Correlated Electrons · Physics 2019-07-30 M. Majumder , F. Freund , T. Dey , M. Prinz-Zwick , N. Büttgen , Y. Skourski , A. Jesche , A. A. Tsirlin , P. Gegenwart

We report on the results of 23Na NMR in the honeycomb lattice magnet Na2Co2TeO6 which has been nominated as a Kitaev material. Measurements of magnetic shift and width of the NMR line as functions of temperature and magnetic field show that…

Strongly Correlated Electrons · Physics 2022-12-21 Jun Kikuchi , Takayuki Kamoda , Nobuyoshi Mera , Yodai Takahashi , Kouji Okumura , Yukio Yasui

Kitaev-type interactions between neighbouring magnetic moments emerge in the honeycomb material ${\alpha}$-RuCl3. It is debated however whether these Kitaev interactions are ferromagnetic or antiferromagnetic. With electron energy loss…

We present a theoretical study of the static and dynamical properties of the Kitaev magnet $\beta$-Li$_2$IrO$_3$ based on the minimal $J$-$K$-$\Gamma$ model. We argue that the incommensurate magnetic order of $\beta$-Li$_2$IrO$_3$ can be…

Strongly Correlated Electrons · Physics 2018-03-20 Samuel Ducatman , Ioannis Rousochatzakis , Natalia B. Perkins

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

We report on magnetization $M(H)$, dc/ac magnetic susceptibility $\chi(T)$, specific heat $C_{\mathrm{m}}(T)$ and muon spin relaxation ($\mu$SR) measurements of the Kitaev honeycomb iridate Cu$_2$IrO$_2$ with quenched disorder. In spite of…

The family of edge-sharing tri-coordinated iridates and ruthenates has emerged in recent years as a major platform for Kitaev spin liquid physics, where spins fractionalize into emergent magnetic fluxes and Majorana fermions with Dirac-like…

Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal…

Strongly Correlated Electrons · Physics 2018-02-14 Y. J. Yu , Y. Xu , K. J. Ran , J. M. Ni , Y. Y. Huang , J. H. Wang , J. S. Wen , S. Y. Li

We use time-domain terahertz spectroscopy to measure the low energy conductivity and magnons in RuCl$_3$ under external magnetic field. At zero field, an oscillation with a frequency of 0.62 THz is clearly observed in time-domain spectrum…

Strongly Correlated Electrons · Physics 2018-09-19 L. Y. Shi , Y. Q. Liu , T. Lin , M. Y. Zhang , S. J. Zhang , L. Wang , Y. G. Shi , T. Dong , N. L. Wang

Honeycomb lattice Kitaev magnets exhibit exotic magnetic properties governed by the Kitaev interaction. This study delves into $\alpha$-RuCl$_3$, a prototypical example described by effective Hamiltonians encompassing bond-dependent Kitaev…

Strongly Correlated Electrons · Physics 2025-05-29 Hamid Mosadeq , Mohammad-Hossein Zare

We consider the quasi-two-dimensional pseudo-spin-1/2 Kitaev - Heisenberg model proposed for A2IrO3 (A=Li, Na) compounds. The spin-wave excitation spectrum, the sublattice magnetization, and the transition temperatures are calculated in the…

Strongly Correlated Electrons · Physics 2016-08-24 A. A. Vladimirov , D. Ihle , N. M. Plakida

$\alpha$-RuCl$_3$ has attracted enormous attention since it has been proposed as a prime candidate to study fractionalized magnetic excitations akin to Kitaev's honeycomb-lattice spin liquid. We have performed a detailed specific-heat…

Strongly Correlated Electrons · Physics 2017-07-19 A. U. B. Wolter , L. T. Corredor , L. Janssen , K. Nenkov , S. Schönecker , S. -H. Do , K. -Y. Choi , R. Albrecht , J. Hunger , T. Doert , M. Vojta , B. Büchner

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

Strongly Correlated Electrons · Physics 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

The pure Kitaev honeycomb model harbors a quantum spin liquid in zero magnetic fields, while applying finite magnetic fields induces a topological spin liquid with non-Abelian anyonic excitations. This latter phase has been much sought…

Strongly Correlated Electrons · Physics 2020-03-31 Dirk Wulferding , Youngsu Choi , Seung-Hwan Do , Chan Hyeon Lee , Peter Lemmens , Clement Faugeras , Yann Gallais , Kwang-Yong Choi

Raman scattering has been employed to investigate lattice and magnetic excitations of the honeycomb Kitaev material $\alpha$-RuCl$_3$ and its Heisenberg counterpart CrCl$_3$. Our phonon Raman spectra give evidence for a first-order…

Strongly Correlated Electrons · Physics 2017-06-07 A. Glamazda , P. Lemmens , S. -H. Do , Y. S. Kwon , K. -Y. Choi

The honeycomb Kitaev-Heisenberg model is a source of a quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. In the quest of finding a pertinent material, $\alpha$-RuCl$_{3}$ recently emerged as…

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