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Polaritonic states, which arise from strong coupling between light and matter, show great promise in modifying chemical reactivity. However, reproducible enhancement of chemical reactions with polaritons is challenging due to a lack of…

Chemical Physics · Physics 2025-01-14 Shahzad Alam , Yicheng Liu , Russell J. Holmes , Renee R. Frontiera

We propose to detect the Mott insulator-superfluid quantum phase transition in an array of coupled cavities by studying the polariton and photon fluctuations in a block of linear dimension M (in units of the lattice constant of the array).…

Other Condensed Matter · Physics 2008-09-10 Davide Rossini , Rosario Fazio , Giuseppe Santoro

A quantum system composed of a molecule and an atomic ensemble, confined in a microscopic cavity, is investigated theoretically. The indirect coupling between atoms and the molecule, realized by their interaction with the cavity radiation…

Chemical Physics · Physics 2020-05-05 Tamás Szidarovszky , Gábor J. Halász , Ágnes Vibók

The scattering of a positron by a muon in the presence of a linearly polarized laser field is investigated in the first Born approximation. The theoretical results reveals: 1) at large scattering angle, an amount of multiphoton processes…

Atomic Physics · Physics 2018-03-14 Wen-Yuan Du , Bing-Hong Wang , Shu-Min Li

Recent experiments and theory demonstrate that the the ground state properties and chemical reactivity of molecules can be modified inside an optical cavity. The vibrational strong or ultrastrong coupling results in the formation of…

Chemical Physics · Physics 2022-12-01 Qi Yu

We theoretically and experimentally investigate nonlinear Zeeman effects within a polarised single-photon source that uses a single 87Rb atom strongly coupled to a high finesse optical cavity. The breakdown of the atomic hyperfine structure…

Quantum Physics · Physics 2018-08-15 Thomas D. Barrett , Dustin Stuart , Oliver Barter , Axel Kuhn

In this work we investigate anharmonic vibrational polaritons formed due to strong light-matter interactions in an optical cavity between radiation modes and anharmonic vibrations beyond the long-wavelength limit. We introduce a…

Quantum Physics · Physics 2024-09-13 Dipti Jasrasaria , Arkajit Mandal , David R. Reichman , Timothy C. Berkelbach

Vibrational polaritons form in a planar Fabry-Perot microcavity when a vibrational mode of a layer of molecules is near resonant with an infrared cavity mode. Herein, dispersion relations of vibrational polaritons are studied when the…

Chemical Physics · Physics 2024-06-18 Tao E. Li

Optomechanical systems explore and exploit the coupling between light and the mechanical motion of matter. A nonlinear coupling offers access to rich new physics, in both the quantum and classical regimes. We investigate a dynamic, as…

Quantum Physics · Physics 2016-10-26 P. Z. G. Fonseca , E. B. Aranas , J. Millen , T. S. Monteiro , P. F. Barker

In multimode optical systems, the spectral covariance matrix encodes all the information about quantum correlations between the quadratures of Gaussian states. Recent research has revealed that, in scenarios that are more common than…

Quantum Physics · Physics 2026-03-11 Bakhao Dioum , Virginia D'Auria , Giuseppe Patera

Integrated photonics has been a promising platform for analog quantum simulation of condensed matter phenomena in strongly correlated systems. To that end, we explore the implementation of all-photonic quantum simulators in coupled cavity…

By means of analytical and numerical methods we analyze the phase diagram of polaritons in one-dimensional coupled cavities. We locate the phase boundary, discuss the behavior of the polariton compressibility and visibility fringes across…

Quantum Physics · Physics 2007-10-29 Davide Rossini , Rosario Fazio

We report on the realization of polariton quantum boxes in a semiconductor microcavity under strong coupling regime. The quantum boxes consist of mesas that confine the cavity photon, etched on top of the spacer of a microcavity. For mesas…

I analyze a scheme that is capable of producing large Kerr nonlinearities on cavity-atom polaritons in a cavity QED system consisting of multiple three-level atoms confined in a cavity mode. A weak control laser coupled to the atoms from…

Optics · Physics 2015-05-14 Yifu Zhu

We reveal the existence of polariton soliton solutions in the array of weakly coupled optical cavities, each containing an ensemble of interacting qubits. An effective complex Ginzburg-Landau equation is derived in the continuum limit…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 I. -H. Chen , Y. Y. Lin , Y. -C. Lai , E. S. Sedov , A. P. Alodjants , S. M. Arakelian , R. -K. Lee

Optical nonreciprocity is important in photonic information processing to route the optical signal or prevent the reverse flow of noise. By adopting the strong nonlinearity associated with a few atoms in a strongly coupled cavity QED system…

The emergence of confined structures and pattern formation are exceptional manifestations of concurring nonlinear interactions found in a variety of physical, chemical and biological systems[1]. Optical solitons are a hallmark of extreme…

Optics · Physics 2020-01-29 Felix Kurtz , Claus Ropers , Georg Herink

An ensemble of identical, intrinsically non-interacting molecules exposed to quantum light is discussed. Their interaction with the quantum light induces interactions between the molecules. The resulting hybrid light-matter states exhibit…

Chemical Physics · Physics 2024-06-19 Lorenz S. Cederbaum

All-optical modulation of light relies on exploiting intrinsic material nonlinearities. However, this optical control is rather challenging due to the weak dependence of the refractive index and absorption coefficients on the concentration…

The coherent strong coupling of molecules with confined light fields to create polaritons - part matter, part light - is opening exciting opportunities ranging from extended exciton transport and inter-molecular energy transfer to modified…

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