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Photon coincidence spectroscopy is a promising technique for probing the nonlinear regime of cavity quantum electrodynamics in the optical domain, however its accuracy is mitigated by two factors: higher-order photon correlations, which…

Quantum Physics · Physics 2009-09-25 L. Horvath , B. C. Sanders

A handful of active galactic nuclei (AGN) have shown strong spectral variations in the optical band between epochs that are years apart. The appearance or disappearance of broad emission lines in their spectra completely changes their…

High Energy Astrophysical Phenomena · Physics 2017-11-15 F. Marin

Molecular vibrations couple to visible light only weakly, have small mutual interactions, and hence are often ignored for non-linear optics. Here we show the extreme confinement provided by plasmonic nano- and pico-cavities can sufficiently…

Unprecedented material compatibility and ease of integration, in addition to the unique and diverse optoelectronic properties of layered materials have generated significant interest in their utilization in nanophotonic devices. While…

Optics · Physics 2018-06-12 Taylor Fryett , Alan Zhan , Arka Majumdar

Strong coupling of molecules to vacuum fields has been widely reported to lead to modified chemical properties such as reaction rates. However, some recent attempts to reproduce infrared strong coupling results have not been successful,…

Mesoscale and Nanoscale Physics · Physics 2024-01-03 Philip A. Thomas , Wai Jue Tan , Vasyl G. Kravets , Alexander N. Grigorenko , William L. Barnes

We derive a coupled mode theory for the interaction of an optical cavity with a waveguide that includes waveguide dispersion. The theory can be applied to photonic crystal cavity waveguide structures. We derive an analytical solution to the…

Optics · Physics 2009-11-11 Edo Waks , Jelena Vuckovic

Polariton chemistry exploits the strong interaction between quantized excitations in molecules and quantized photon states in optical cavities to affect chemical reactivity. Molecular polaritons have been experimentally realized by the…

Chemical Physics · Physics 2023-09-06 Jonathan J. Foley , Jonathan F. McTague , A. Eugene DePrince

Recent experiments have demonstrated that molecular polaritons, hybrid states of light and matter formed by the strong coupling between molecular electronic or vibrational excitations and an optical cavity, can substantially modify the…

Chemical Physics · Physics 2021-07-08 Nguyen Thanh Phuc

Photon-photon interactions are an essential requirement of quantum photonic information processing. One way to generate these interactions is to utilize an atom strongly coupled to an optical cavity. This system exhibits the photon blockade…

Quantum Physics · Physics 2022-05-31 Harjot Singh , Edo Waks

We consider an ensemble of diatomic molecules resonantly coupled to an optical cavity under strong coupling conditions at normal incidence. Photodissociation dynamics is examined via direct numerical integration of the coupled…

Chemical Physics · Physics 2023-03-08 Maxim Sukharev , Joseph Subotnik , Abraham Nitzan

We theoretically propose a scheme for photon blockade in a cavity quantum electrodynamical system consisting of an N-type atomic medium interacting with a single-mode Fabry-Perot cavity. In contrast to inefficient…

Quantum Physics · Physics 2023-05-19 Xin Su , Jiang-Shan Tang , Keyu Xia

The progress in understanding the optical and microscopic properties of polaritons relies on various optical cavities to confine electromagnetic radiation, which causes a demand for new platforms with higher $Q$-factors and better…

We report experimental evidence of the interaction between intersubband polaritons and longitudinal optical phonons in non-dispersive mid-infrared cavities, under resonant optical injection. The light emission originating from spontaneous…

Polaritons are the collective excitations of many atoms dressed by resonant photons, which can be used to explain the slow light propagation with the mechanism of electromagnetically induced transparency. As quasi-particles, these…

Quantum Physics · Physics 2009-11-13 Lan Zhou , Jing Lu , D. L. Zhou , C. P. Sun

We experimentally demonstrate simultaneous spatial and temporal compression in the propagation of light pulses in multimode nonlinear optical fibers. We reveal that the spatial beam self-cleaning recently discovered in graded-index…

The lack of interactions between single photons prohibits direct nonlinear operations in quantum optical circuits, representing a central obstacle in photonic quantum technologies. Here, we demonstrate multi-mode nonlinear photonic circuits…

Multilayer assemblies of metal nanoparticles can act as photonic structures, where collective plasmon resonances hybridize with cavity modes to create plasmon-polariton states. For sufficiently strong coupling, plasmon polaritons…

The phonon-polariton spectrum in dielectric medium with the third order nonlinearity was theoretically obtained. Dependence of number of polariton spectrum branches on intensity of electromagnetic field was investigated. The appearance of…

Optics · Physics 2012-05-08 I. V. Dzedolik , O. S. Karakchieva

When mid-infrared light interacts with nanoscale polar dielectric structures optical phonon propagation cannot be ignored, leading to a rich nonlocal phenomenology which we have only recently started to uncover. In properly crafted…

Mesoscale and Nanoscale Physics · Physics 2021-08-10 Christopher R. Gubbin , Simone De Liberato

When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Yu Zhang , Tammie Nelson , Sergei Tretiak
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