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We present an approximate analytic expression for the photoluminescence spectral function of a model polariton system, which describes a quantum dot, with a finite number of fermionic levels, strongly interacting with the lowest photon mode…
We present a general and efficient approach to compute phase-resolved multidimensional spectra of anharmonic molecular polaritons, based on a semiclassical evolution of the molecular Hamiltonian and cavity field in the large-$\mathcal{N}$…
In this article, we study the effects of intrinsic nonlinear optomechanical interaction on the linear response of a driven-dissipative optomechanical system to a weak time-dependent perturbation. By calculating the linear response of the…
Strong coupling between various kinds of material excitations and optical modes has recently shown potential to modify chemical reaction rates in both excited and ground states. The ground-state modification in chemical reaction rates has…
Quantum nonlinear optics is a quickly growing field with large technological promise, at the same time involving complex and novel many-body phenomena. In the usual scenario, optical nonlinearities originate from the interactions between…
The achievement of large values of the light-matter coupling in nanoengineered photonic structures can lead to multiple photonic resonances contributing to the final properties of the same hybrid polariton mode. We develop a general theory…
A light-matter hybrid quasiparticle, called a polariton, is formed when molecules are strongly coupled to an optical cavity. Recent experiments have shown that polariton chemistry can manipulate chemical reactions. Polariton chemistry is a…
Plasmonic nanocavities enable the confinement of molecules and electromagnetic fields within nano-metric volumes. As a consequence, the molecules experience a remarkably strong interaction with the electromagnetic field, to such an extent…
Microcavity polaritons are light-matter quasiparticles that arise from the strong coupling between excitons and photons confined in a semiconductor microcavity. They typically operate at visible or near visible wavelengths. They combine the…
The interaction of quantum light with matter like that inside a cavity is known to give rise to mixed light-matter states called polaritons. We discuss the impact of rotation of the cavity on the polaritons. It is shown that the number of…
Nonadiabatic phenomena are investigated in the rovibrational motion of molecules confined in an infrared cavity. Conical intersections (CIs) between vibrational polaritons, similar to CIs between electronic polaritonic surfaces, are found.…
In this work we investigate the effects that multi-mode photonic environments, e.g., optical cavities, have on the properties of quantum matter. We highlight the importance of the non-perturbative mass renormalization procedure for ab…
Small organic molecules with a {\pi}-conjugated system that consists of only a few double or triple bonds can have significantly smaller optical excitation energies when equipped with donor- and acceptor groups, which raises the quantum…
We employ an exact quantum mechanical simulation technique to investigate a model of cavity-modified chemical reactions in the condensed phase. The model contains the coupling of the reaction coordinate to a generic solvent, cavity coupling…
Light-matter systems allow to realize a strongly correlated phase where photons are present. In these systems strong correlations are achieved by optical nonlinearities, which appear due to the coupling of photons to atomic-like structures.…
A nonlinear self-focusing material can amplify random small-amplitude phase modulations present in an optical beam, leading to the formation of amplitude singularities commonly referred to as optical caustics. By imposing polarization…
We consider the coupled propagation of an optical field and its second harmonic in a quadratic nonlinear medium governed by a coupled system of Schrodinger equations. We prove the existence of ring-profiled optical vortex solitons appearing…
Despite the potential paradigm breaking capability of microcavities to control chemical processes, the extent to which photonic devices change properties of molecular materials is still unclear, in part due to challenges in modeling hybrid…
A general theory of polariton parametric photoluminescence in spatially inhomogeneous systems is developed. The quantum Langevin equations are solved in a generalized Bogoliubov de Gennes approximation. We apply the formalism to the…
Electron-phonon coupling in semiconductor quantum dots plays a significant role in determining the optical properties of excited excitons, especially the spectral nature of emitted photons. This paper presents a comprehensive theory and…