Related papers: Hidden nonlinear optical susceptibilities in linea…
Organic microcavities are photonic nanostructures that strongly confine the electromagnetic field, allowing exotic quantum regimes of light-matter interaction with disordered organic semiconductors. The unambiguous interpretation of the…
Photon pairs and heralded single photons, obtained from cavity-assisted parametric down-conversion (PDC), play an important role in quantum communications and technology. This motivated a thorough study of the spectral and temporal…
Organic microcavities can be engineered to reach exotic quantum regimes of strong and ultrastrong light-matter coupling. However, the microscopic interpretation of their spectroscopic signals can be challenging due to the competition…
Nonlinear interactions between phonon modes govern the behavior of vibrationally highly excited solids and molecules. Here, we demonstrate theoretically that optical cavities can be used to control the redistribution of energy from a highly…
Nonlinear optical wave propagation manifests in a multitude of frequencies generated from quantum-noise, and selecting desired nonlinear products usually requires seeding the medium with extraneous waves, employing spatial or spectral…
We calculate the intensity of the polariton mediated inelastic light scattering in semiconductor microcavities. We treat the exciton-photon coupling nonperturbatively and incorporate lifetime effects in both excitons and photons, and a…
Molecular polaritons arise when molecules interact so strongly with light that they become entangled with each other. This light-matter hybridization alters the chemical and physical properties of the molecular system and allows chemical…
The photon blockade (PB) effect in emitter-cavity systems depends on the anharmonicity of the ladder of dressed energy eigenstates. The recent developments in color center photonics are leading toward experimental demonstrations of…
Polaritonic chemistry exploits strong light-matter coupling between molecules and confined electromagnetic field modes to enable new chemical reactivities. In systems displaying this functionality, the choice of the cavity determines both…
Recently the possibility of generating nonclassical polariton states by means of parametric scattering has been demonstrated. Excitonic polaritons propagate in a complex interacting environment and contain real electronic excitations…
Motivated by the recent advances in optical imaging and tracking of wave-packet propagation in optical cavities, we systematically explore the non-Hermitian polariton dynamics within a decay-tunable multimode cavity model. The complex…
We propose collective nuclear polaritons formed by hybridizing a 229Th nuclear ensemble with a vacuum-ultraviolet cavity mode generated via four-wave mixing, achieving a collective light-matter coupling that scales as $\sqrt{N}$. In the…
Nonlinear optical effects provide a natural way of light manipulation and interaction, and form the foundation of applied photonics -- from high-speed signal processing and telecommunication, to ultra-high bandwidth interconnects and…
We study a 2D system of trion-polaritons at the quantum level and demonstrate that for monolayer semiconductors they can exhibit a strongly nonlinear optical response. The effect is due to the composite nature of trion-based excitations…
Resonant coupling of a vibration to a cavity mode has been reported to dramatically modify spontaneous Raman scattering, but subsequent studies have produced conflicting results. In this Letter, we develop a microscopic quantum framework…
Nonlinear optical cavities are crucial both in classical and quantum optics; in particular, nowadays optical parametric oscillators are one of the most versatile and tunable sources of coherent light, as well as the sources of the highest…
Phase transitions, where observable properties of a many-body system change discontinuously, can occur in both open and closed systems. Ultracold atoms have provided an exemplary model system to demonstrate the physics of closed-system…
Breaking the time-reversal symmetry of light is of great importance for fundamental physics and has attracted increasing interest in the study of non-reciprocal photonic devices. Here, we experimentally demonstrate a chiral cavity QED…
Nonlinear optical phenomena are typically local. Here we predict the possibility of highly nonlocal optical nonlinearities for light propagating in atomic media trapped near a nano-waveguide, where long-range interactions between the atoms…
We report a significant advancement in ultra low power light-by-light phase modulation using open semiconductor microcavities in the strong light-matter coupling regime. We achieve cross-phase modulation of up to 247$\pm$17 mrad per…