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A new concept for narrow-band direct nuclear laser spectroscopy of $^{229\text{m}}$Th is proposed, using a single comb mode of a vacuum ultraviolet frequency comb generated from the 7th harmonic of an Yb-doped fiber laser system. In this…

Instrumentation and Detectors · Physics 2020-07-09 Lars von der Wense , Chuankun Zhang

Thorium-229 is a unique case in nuclear physics: it presents a metastable first excited state Th-229m, just a few electronvolts above the nuclear ground state. This so-called isomer is accessible by VUV lasers, which allows transferring the…

The $^{229}\text{Th}$ isotope is a promising candidate for nuclear clocks, with its transition frequency influenced by electron-induced nuclear frequency shifts. This effect is comparatively small and requires high-precision theoretical…

Atomic Physics · Physics 2025-05-09 Ran Si , Chaofan Shi , Nan Xue , Xiangjin Kong , Chongyang Chen , Bingsheng Tu , Yu-Gang Ma

$^{229}$Th, a crucial candidate for nuclear clocks and many other applications, is a typical heavy nucleus with an extremely low-energy isomeric state $^{229m}$Th. A detailed study of the nuclear structure of $^{229}$Th is performed here by…

Nuclear Theory · Physics 2025-08-28 Zi-Rui Chen , Long-Jun Wang , Yuanbin Wu

We review the ideas and concepts for a clock that is based on a radiative transition in the nucleus rather than in the electron shell. This type of clock offers advantages like an insensitivity against field-induced systematic frequency…

Nuclear Experiment · Physics 2015-06-18 Ekkehard Peik , Maxim Okhapkin

For the isotope $^{229}$Th we investigate the possibility of two-photon laser spectroscopy of the nuclear clock transition (148.38 nm) using intense monochromatic laser field at twice the wavelength (296.76 nm). Our estimates show that due…

The 8 eV first nuclear excited state in $^{229}$Th is a candidate for implementing an nuclear clock. Doping $^{229}$Th into ionic crystals such as CaF$_2$ is expected to suppress non-radiative decay, enabling nuclear spectroscopy and the…

Peik and Tamm [Europhys. Lett. 61, 181 (2003)] proposed a nuclear clock based on the isomeric transition between the ground state and the first excited state of thorium-229. This transition was recognized as a potentially sensitive probe of…

Atomic Physics · Physics 2021-01-19 Pavel Fadeev , Julian C. Berengut , Victor V. Flambaum

The exceptionally low-energy isomeric transition in $^{229}$Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large…

We report the results of a direct search for the $^{229}$Th ($I^{p} = 3/2^+\leftarrow 5/2^+$) nuclear isomeric transition, performed by exposing $^{229}$Th-doped LiSrAlF$_6$ crystals to tunable vacuum-ultraviolet synchrotron radiation and…

The $^{229}$Th nucleus has a unique transition at only 8 eV which could be used for a novel nuclear clock. We investigate theoretically the prospects of driving this transition with vortex light beams carrying orbital angular momentum.…

Atomic Physics · Physics 2024-04-22 Tobias Kirschbaum , Thorsten Schumm , Adriana Pálffy

LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that…

$^{229}$Th with a low-lying nuclear isomeric state is an essential candidate for a nuclear clock as well as many other applications. Laser excitation of the isomeric state has been a long-standing goal. With relativistic $^{229}$Th ions in…

We aim to perform direct optical spectroscopy of the Th-229 nuclear isomer to measure its energy and lifetime, and to demonstrate optical coupling to the nucleus. To this end, we develop Th-doped CaF2 crystals, which are transparent at the…

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

Nuclear Experiment · Physics 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

The results of experimental studies of the low-energy isomeric state in the $^{229}$Th nucleus are presented. The work is consisted of several stages. During the first stage $^{229}$Th nuclei were excited with the inverse internal…

We present a comprehensive theoretical investigation of hyperfine-resolved excitation and detection of the low-energy isomeric state of $^{229}$Th in trapped $^{229}\mathrm{Th}^{3+}$ ions. Using a quantum master equation approach, we…

Atomic Physics · Physics 2026-05-01 Wu Wang , Ke Zhang , Ke-Mi Xu , Shan-Gui Zhou

Thorium-229, with its exceptionally low-energy nuclear excited state, is a key candidate for developing nuclear clocks. $^{229}$Th-doped CaF$_2$ crystals, benefiting from calcium fluoride's wide band gap, show great promise as solid-state…

The recent laser excitation of the low-lying Th-229 isomer transition is starting a revolution in ultralight dark matter searches. The enhanced sensitivity of this transition to the large class of dark matter models dominantly coupling to…

High Energy Physics - Phenomenology · Physics 2025-05-20 Elina Fuchs , Fiona Kirk , Eric Madge , Chaitanya Paranjape , Ekkehard Peik , Gilad Perez , Wolfram Ratzinger , Johannes Tiedau

The recent demonstration of laser excitation of the $\approx 8$ eV isomeric state of Thorium-229 is a significant step towards a nuclear clock. The low excitation energy likely results from a cancellation between electromagnetic and strong…

High Energy Physics - Phenomenology · Physics 2025-09-16 Andrea Caputo , Doron Gazit , Hans-Werner Hammer , Joachim Kopp , Gil Paz , Gilad Perez , Konstantin Springmann