Related papers: $^{229}\mathrm{ThF}_4$ thin films for solid-state …
The 7.6-eV-isomer of Thorium-229 offers the opportunity to perform high resolution laser spectroscopy of a nuclear transition. We give a brief review of the investigations of this isomer. The nuclear resonance connecting ground state and…
State-resolved laser spectroscopy at the 10$^{-12}$ precision level recently reported in $arXiv$:2406.18719 determined the fractional change in nuclear quadrupole moment between the ground and isomeric state of $^{229}\rm{Th}$, $\Delta…
The isotope $^{229}$Th is unique in that it possesses an isomeric state of only a few eV above the ground state, suitable for nuclear laser excitation. An optical clock based on this transition is expected to be a very sensitive probe for…
We propose a simple approach to measure the energy of the few-eV isomeric state in Th-229. To this end, U-229 nuclei are doped into VUV-transparent crystals, where they undergo alpha decay into Th-229, and, with a probability of 2%,…
Clocks based on nuclear isomer transitions promise exceptional stability and precision. The low transition energy of the thorium-229 isomer makes it an ideal candidate, as it has been excited by a vacuum-ultraviolet laser and is highly…
The nucleus of 229Thorium presents a unique isomer state of very low energy and long lifetime, current estimates are around 7.8 eV and seconds to hours respectively. This nuclear transitions therefore is a promising candidate for a novel…
Thorium-doped LiCaAlF$_6$ and LiSrAlF$_6$ (Th:LiCAF and Th:LiSAF) are promising crystals for a solid-state nuclear clock based on the 8 eV transition in $^{229}$Th; however, their complex crystal structures complicate understanding the…
When Th nuclei are doped in CaF$_2$ crystals, a set of electronic defect states appears in the crystal bandgap which would otherwise provide complete transparency to vacuum-ultraviolet radiation. The coupling of these defect states to the 8…
Recent advances in laser excitation of the low-energy nuclear isomer transition in $^{229}$Th have opened avenues for developing nuclear clocks, a novel quantum technology with exceptional performance and sensitivity to exotic physics. Here…
$^{229}$Th is the only nucleus currently under investigation for the development of a nuclear optical clock (NOC) of ultra-high accuracy. The insufficient knowledge of the first nuclear excitation energy of $^{229}$Th has so far hindered…
A comparative vacuum ultraviolet spectroscopy study conducted at ISOLDE-CERN of the radiative decay of the $^{229m}$Th nuclear clock isomer embedded in different host materials is reported. The ratio of the number of radiative decay photons…
The low-energy isomeric transition in Thorium-229 offers a unique interface between nuclear and atomic physics, presenting a resource for quantum technologies that is notably resilient to environmental decoherence. While early experiments…
M\"ossbauer spectroscopy is widely used in biochemistry, geology, and solid-state physics to obtain structural information on materials. Here, we extend this technique into the optical range using a vacuum ultraviolet laser to probe the…
Given the drastic progress achieved during recent years in our knowledge on the decay and nuclear properties of the thorium isomer 229mTh, the focus of research on this potential nuclear clock transition will turn in the near future from…
Building on recent advances of the embedded cluster approach combined with multiconfigurational theory, this work investigates the electronic states in thorium-doped CaF2 crystals. Th:CaF2 is currently establishing as a promising material…
The 10-minute radiative lifetime of the first excited $^{229}$Th$^{4+}$ nuclear state in ionic crystals provides narrow spectroscopic linewidths, enabling the realization of a solid-state nuclear clock. Due to the 4+ noble gas…
We report a candidate with unique advantages in the cultivation of solid-state nuclear clock material, Th:SrF2 crystal. It not only has a segregation coefficient close to 1, which can achieve highly efficient and uniform doping of Th, but…
The paper considers a principal possibility of creating a nuclear light source of the vacuum ultra violet (VUV) range based on the $^{229}$Th nucleus. This nuclear light source can help to solve two main problems -- excitation of the…
Laser excitation of thorium-229 nuclei in doped wide bandgap crystals has been demonstrated recently, opening the possibility of developing ultrastable solid-state clocks and sensitive searches for new physics. We develop a quantitative…
We calculate hyperfine structure of $^{229}$Th and its ions (Th~IV, Th~III, Th~II, Th~I) to reveal the dependence of the nuclear clock frequency on the hyperfine interaction (hfi). We calculate first and second-order hfi shifts and…