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Optical properties of heterostructures composed of layered 2D materials, such as transition metal dichalcogenides (TMDs) and graphene, are broadly explored. Of particular interest are light-induced energy transfer mechanisms in these…

Materials Science · Physics 2024-09-17 Amir Kleiner , Daniel Hernangómez-Pérez , Sivan Refaely-Abramson

Interlayer excitons are observed coexisting with intralayer excitons in bi-layer, few-layer, and bulk MoSe2 single crystals by confocal reflection contrast spectroscopy. Quantitative analysis using the Dirac-Bloch-Equations provides…

Materials Science · Physics 2018-06-13 Jason Horng , Tineke Stroucken , Long Zhang , Eunice Y. Paik , Hui Deng , Stephan W. Koch

Space-resolved X-ray diffraction measurements performed on gradient-etched CuInGaSe2 (CIGS) solar cells provide information about stress and texture depth profiles in the absorber layer. An important parameter for CIGS layer growth…

Exciton binding energies of hundreds of meV and strong light absorption in the optical frequency range make transition metal dichalcogenides (TMDs) promising for novel optoelectronic nanodevices. In particular, atomically thin TMDs can be…

Mesoscale and Nanoscale Physics · Physics 2018-04-24 Simon Ovesen , Samuel Brem , Christopher Linderälv , Mikael Kuisma , Paul Erhart , Malte Selig , Ermin Malic

Time-Dependent Density Functional Theory (TDDFT) has been currently established as a computationally cheaper, yet effective, alternative to the Many-Body Perturbation Theory (MBPT) for calculating the optical properties of solids. Within…

Materials Science · Physics 2026-04-13 M. Arruabarrena , A. Leonardo , A. Ayuela

We present first-principles many-body calculations of the dielectric constant, quasiparticle band structure, and optical absorption spectrum of monolayer MoS$_2$ using a supercell approach. As the separation between the periodically…

Materials Science · Physics 2014-01-15 Falco Hüser , Thomas Olsen , Kristian S. Thygesen

Transition metal dichalcogenides (TMDs) are regarded as a possible materials platform for quantum information science and related device applications. In TMD monolayers, the dephasing time and inhomogeneity are crucial parameters for any…

Recent measurements have shown that a continuously tunable bandgap of up to 250 meV can be generated in biased bilayer graphene [Y. Zhang et al., Nature 459, 820 (2009)], opening up pathway for possible graphene-based nanoelectronic and…

Materials Science · Physics 2010-02-11 Cheol-Hwan Park , Steven G. Louie

The electron-boson spectral density (or glue) function can be obtained from measured optical scattering rate by solving a generalized Allen formula, which relates the two quantities with an integral equation and is an inversion problem.…

Strongly Correlated Electrons · Physics 2021-12-30 Hwiwoo Park , Jun H. Park , Jungseek Hwang

X-ray diffraction based microscopy techniques such as High Energy Diffraction Microscopy rely on knowledge of the position of diffraction peaks with high precision. These positions are typically computed by fitting the observed intensities…

Image and Video Processing · Electrical Eng. & Systems 2021-06-04 Zhengchun Liu , Hemant Sharma , Jun-Sang Park , Peter Kenesei , Antonino Miceli , Jonathan Almer , Rajkumar Kettimuthu , Ian Foster

Excitonic effects in solids can be calculated using the Bethe-Salpeter equation (BSE) or the Casida equation of time-dependent density-functional theory (TDDFT). In both methods, the Tamm-Dancoff approximation (TDA), which decouples…

Materials Science · Physics 2016-10-14 Young-Moo Byun , Carsten A. Ullrich

We derive and motivate a Laplacian-level, orbital-free meta-generalized-gradient approximation (LL-MGGA) for the exchange-correlation energy, targeting accurate ground-state properties of $sp$ and $sd$ metallic condensed matter, in which…

Materials Science · Physics 2022-08-02 Aaron D. Kaplan , John P. Perdew

We present an experimental and theoretical study of the high-energy excitation spectra of a dipolar supersolid. Using Bragg spectroscopy, we study the scattering response of the system to a high-energy probe, enabling measurements of the…

Photon transport through a diffusing slab can be described by the radiative transfer equation (RTE). When the slab is highly scattering and weakly absorbing, the RTE simplifies to the diffusion equation. In this paper, an inverse diffusion…

We study possible optically excited bound states in monolayer MoS2: excitons and trions. For this purpose we formulate and apply a generalized time-dependent density-matrix functional approach for bound states of multiple excitations. The…

Mesoscale and Nanoscale Physics · Physics 2014-02-18 Alfredo Ramirez-Torres , Volodymyr Turkowski , Talat S. Rahman

We utilize cavity-enhanced extinction spectroscopy to directly quantify the optical absorption of defects in MoS$_2$ generated by helium ion bombardment. We achieve hyperspectral imaging of specific defect patterns with a detection limit…

Atomic monolayers represent a novel class of materials to study localized and free excitons in two dimensions and to engineer optoelectronic devices based on their significant optical response. Here, we investigate the role of the substrate…

Mesoscale and Nanoscale Physics · Physics 2017-07-21 Oliver Iff , Yu-Ming He , Nils Lundt , Sebastian Stoll , Vasilij Baumann , Sven Höfling , Christian Schneider

Once a gravitational wave signal is detected, the measurement of its source parameters is important to achieve various scientific goals. This is done through Bayesian inference, where the analysis cost increases with the model complexity…

General Relativity and Quantum Cosmology · Physics 2023-08-29 Harsh Narola , Justin Janquart , Quirijn Meijer , K. Haris , Chris Van Den Broeck

Our ability to efficiently detect and generate far-infrared (i.e., terahertz) radiation is vital in areas spanning from biomedical imaging to interstellar spectroscopy. Despite decades of intense research, bridging the terahertz gap between…

Materials Science · Physics 2023-07-24 Zhao Tang , Greis J. Cruz , Fanhao Jia , Yabei Wu , Weiyi Xia , Peihong Zhang

The excitonic spectra of single layer GeS and GeSe are predicted by ab initio GW-Bethe Salpeter equation calculations. G 0 W 0 calculations for the band structures find a fundamental band gap of 2.85 eV for GeS and 1.70 eV for GeSe…

Mesoscale and Nanoscale Physics · Physics 2016-10-26 Lidia C. Gomes , P. E. Trevisanutto , A. Carvalho , A. S. Rodin , A. H. Castro Neto