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A first-principles derived approach is combined with the inverse Monte Carlo technique to determine the atomic orderings leading to prefixed properties in Pb(Sc_{0.5}Nb_{0.5})O_{3} perovskite alloy. We find that some arrangements between Sc…

Materials Science · Physics 2009-11-07 Jorge Iniguez , L. Bellaiche

Using an extension of a first-principles method developed by King-Smith and Vanderbilt [Phys. Rev. B {\bf 49}, 5828 (1994)], we investigate the effects of in-plane epitaxial strain on the ground-state structure and polarization of eight…

Materials Science · Physics 2009-12-22 Oswaldo Dieguez , Karin M. Rabe , David Vanderbilt

The use of laser with a Gaussian-beam profile is frequently adopted in attempts of crystallizing non-single-crystal thin films; however, it merely results in the formation of poly-crystal thin films. In this paper, selective area…

Applied Physics · Physics 2022-11-17 Willam Bodeau , Kaisei Otoge , Wenchang Yeh , Nobuhiko P. Kobayashi

A method for obtaining a smooth, single crystal diamond surface is presented, whereby a sacrificial defective layer is created by implantation and graphitized by annealing before being selectively etched. We have used O+ at 240 keV, the…

We consider site percolation on a correlated bi-colored simple cubic lattice. The correlated medium is constructed from a strongly alternating bi-colored simple cubic lattice due to anti-site disordering. The percolation threshold is…

Disordered Systems and Neural Networks · Physics 2007-05-23 Yuriy Yu. Tarasevich , Elena N. Manzhosova

The protection of halide perovskites is important for the performance and stability of emergent perovskite-based optoelectronic technologies. In this work, we investigate the potential inorganic protective coating materials ZnO, SrZrO3, and…

Materials Science · Physics 2022-02-22 Azimatu Fangnon , Marc Dvorak , Ville Havu , Milica Todorovic , Jingrui Li , Patrick Rinke

While nature provides a plethora of perovskite materials, only a few exhibits large ferroelectricity and possibly multiferroicity. The majority of perovskite materials have the non-polar CaTiO$_3$(CTO)structure, limiting the scope of their…

Materials Science · Physics 2022-05-25 Hongwei Wang , Fujie Tang , Massimiliano Stengel , Hongjun Xiang , Qi An , Tony Low , Xifan Wu

Using the full-potential linearized-augmented-plane-wave (FLAPW) method, we have analyzed systematically the trends in the structural and electronic properties of the 3d and 4d transition-metal oxides SrMO_3 (M = Ti, V, Zr and Nb). The…

Materials Science · Physics 2016-08-31 I. R. Shein , V. L. Kozhevnikov , A. L. Ivanovskii

Ten years have passed since the description of the perovskite to post-perovskite transition in MgSiO3 and its' impact on the mineralogy and rheology of the D" region at the base of the Earth's mantle. Much work has explored the mechanisms…

We present a high-pressure x-ray diffuse scattering study of the ABO$_3$ ferroelectric perovskites BaTiO_3 and KNbO_3. The well-known diffuse lines are observed in all the phases studied. In KNbO_3, we show that the lines are present up to…

Materials Science · Physics 2009-11-13 Sylvain Ravy , Jean-Paul Itie , Alain Polian , Michael Hanfland

Perovskites with tunable and switchable polarization hold immense promise for unlocking novel functionalities. Using density-functional theory, we reveal that intrinsic defects can induce, enhance, and control polarization in…

Materials Science · Physics 2025-06-03 Wahib Aggoune , Matthias Scheffler

The lattice constants of Strontium titanate perovskite has been studied using the Density functional theory formalism at the PBE and the HSE levels of theory. The study has been done in all the 3 existing phases; namely cubic, orthorhombic…

Materials Science · Physics 2021-12-22 Manaswita Kar

Strain engineering with different substrate facets is promising for tuning functional properties of thin film perovskite oxides. By choice of facet, different surface symmetries and chemical bond directions for epitaxial interfaces can be…

Materials Science · Physics 2020-11-26 K. Kjærnes , T. Bolstad , D. M. Evans , E. Lysne , B. A. D. Williamson , D. Meier , S. M. Selbach , T. Tybell

We report a study on the interface between polar high-k materials and the Si(001)-(2X1) reconstructed surface with LaAlO3 taken as a prototype material. The construction of the interface is based on the prior growth of metal lines followed…

Materials Science · Physics 2015-06-25 Isabelle Devos , Pierre Boulenc

Water-soluble sacrificial layers based on epitaxially-grown, single crystalline (Ca, Sr, Ba)3Al2O6 layer are widely used for creating free-standing perovskite oxide membranes. However, obtaining these sacrificial layers with intricate…

Materials Science · Physics 2024-05-20 Shivasheesh Varshney , Martí Ramis , Sooho Choo , Mariona Coll , Bharat Jalan

Hole-doped perovskite bismuthates such as Ba$_{1-x}$K$_x$BiO$_3$ and Sr$_{1-x}$K$_x$BiO$_3$ are well-known bismuth-based oxide high-transition-temperature superconductors. Reported thin bismuthate films show relatively low quality, likely…

The surface composition of polycrystalline niobium-doped strontium titanate (SrTiO3 : Nb) is studied using X-ray photoelectron emission microscopy (XPEEM) for many grain orientations in order to characterise the surface chemistry with high…

Lead titanate (PbTiO3) is a classical example of a ferroelectric perovskite oxide illustrating a displacive phase transition accompanied by a softening of a symmetry-breaking mode. The underlying assumption justifying the soft-mode theory…

Materials Science · Physics 2015-06-12 J. Frantti , Y. Fujioka , A. Puretzky , Y. Xie , Z. -G. Ye , A. M. Glazer

Metal halide perovskites single-crystalline thin films (SCTFs) have recently emerged as promising materials for the next generation of optoelectronic devices due to their superior intrinsic properties. However, it is still challenging to…

Applied Physics · Physics 2020-11-03 Yu-Hao Deng

Renewable energy sources are of great interest to combat global warming, yet promising sources like photovoltaic (PV) cells are not efficient and cheap enough to act as an alternative to traditional energy sources. Perovskite has high…