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Related papers: How to cleave cubic perovskite oxides

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We report surface reconstruction (RC)-dependent growths of SrTiO3 and SrVO3 on a SrTiO3 (001) surface with two different coexisting surface RCs, namely (2x1) and c(6x2). Up to the coverage of several layers, epitaxial growth was forbidden…

Materials Science · Physics 2011-04-25 Soo-hyon Phark , Young Jun Chang , Tae Won Noh

The perovskite SrVO$_3$ is of interest for a variety of applications due to its simple metallic character and stability in reducing environments. Here we report the preparation of single-crystal SrVO$_3$ using the laser floating zone…

Strongly Correlated Electrons · Physics 2022-03-02 Tanya Berry , Shannon Bernier , Gudrun Auffermann , Tyrel M. McQueen , W. Adam Phelan

Tuning the work functions of materials is of practical interest for maximizing the performance of microelectronic and (photo)electrochemical devices, as the efficiency of these systems depends on the ability to control electronic levels at…

Materials Science · Physics 2021-04-07 Yihuang Xiong , Weinan Chen , Wenbo Guo , Hua Wei , Ismaila Dabo

A device for UHV cleavage of crystal specimens for the use with STM has been suggested and developed. We present a device suitable for the precise cleavage of semiconductors. The device needs only small space and can be easily mounted in a…

First-principles total-energy calculations are carried out for (001) surfaces of the cubic perovskite ATiO3 compounds PbTiO3, BaTiO3, and SrTiO3. Both AO-terminated and TiO2-terminated surfaces are considered, and fully-relaxed atomic…

Materials Science · Physics 2015-06-25 B. Meyer , J. Padilla , David Vanderbilt

We provide insights into the influence of surface termination on the oxygen vacancy incorporation for the perovskite model material SrTiO3 during annealing in reducing gas environments. We present a novel approach to control to tailor the…

Materials Science · Physics 2019-11-15 Felix V. E. Hensling , Christoph Baeumer , Marc-André Rose , Felix Gunkel , Regina Dittmann

The (001) surfaces of polar perovskites BaTiO$_3$ and PbTiO$_3$ have been studied from first principles at T=0 K. For both cases of polarization, the most stable TiO-terminated interfaces show intrinsic ferroelectricity. In the topmost…

Materials Science · Physics 2008-03-12 M. Fechner , S. Ostanin , I. Mertig

The surface/interface species in perovskite oxides play an essential role in many novel emergent physical phenomena and chemical processes. With low eigen-energy in the terahertz region, such species at buried interfaces remain poorly…

The highly conducting and transparent inorganic perovskites SrBO$_3$ with V, Nb, Mo, and their mixtures at the B-site have recently attracted the attention of the oxide electronics community as novel alternative transparent conducting…

Using cross-sectional scanning tunneling microscopy on in situ fractured SrTiO$_{3}$, one of the most commonly used substrates for the growth of complex oxide thin films and superlattices, atomically smooth terraces have been observed on…

Mesoscale and Nanoscale Physics · Physics 2009-12-22 Nathan P. Guisinger , Tiffany S. Santos , Jeffrey R. Guest , Te-Yu Chien , Anand Bhattacharya , John W. Freeland , Matthias Bode

We report that a deionized water etching and thermal annealing technique can be effective for preparing atomically-flat and singly-terminated surfaces of single crystalline SrTiO3 substrates. After a two-step thermal-annealing and…

Materials Science · Physics 2013-09-09 J. G. Connell , B. J. Isaac , D. R. Strachan , S. S. A. Seo

We report the first observation of coherent surface states on cubic perovskite oxide SrVO3(001) thin films through spectroscopic imaging scanning tunneling microscopy. A direct link between the observed atomic-scale interference patterns…

The Fe^{4+}-containing cubic perovskite phase SrFeO_3-x is of interest both for its high-temperature, oxygen-conducting properties as a solid oxide fuel cell component, and at low temperatures, where it exhibits a plethora of helical…

Materials Science · Physics 2012-10-23 D. C. Peets , Jung-hwa Kim , M. Reehuis , P. Dosanjh , B. Keimer

The local structure and oxidation state of the cobalt impurity in SrTiO$_3$ is studied by X-ray absorption fine structure (XAFS) spectroscopy. The synthesis conditions, under which cobalt predominantly (up to 76%) substitutes the atoms at…

Materials Science · Physics 2021-08-21 I. A. Sluchinskaya , A. I. Lebedev

The water gas shift reaction (WGS) is important and widely applied in the production of H2. Cu modified perovskites are promising catalysts for WGS reactions in hydrogen generation. However, the structure-dependent stability and reaction…

Suspended micro-structures based on complex oxides relies on surface micro-machining processes such as those based on sacrificial layers. These processes prevent to physically access the microstructures from both sides, as substantial part…

ABO3 oxides with the perovskite-related structures are attracting significant interest due to their promising physical and chemical properties for many applications requiring tunable chemistry, including fuel cells, catalysis, and…

Materials Science · Physics 2021-07-13 Su Jeong Heo , Andriy Zakutayev

Although perovskite oxides hold promise in applications ranging from solid oxide fuel cells to catalysts, their surface chemistry is poorly understood at the molecular level. Here we follow the formation of the first monolayer of water at…

We describe a simple procedure for optimising the growth condition for high quality single crystals of the strontium ruthenate perovskites using an image furnace. The procedure involves carefully measuring the mass lost during crystal…

Materials Science · Physics 2009-11-10 R. S. Perry , Y. Maeno

The possibility to segregate cobalt and iron in a single perovskite, at a nanoscale in the form of layers has been investigated, using sol gel technic synthesis. Quite remarkably, it is shown that such a nanoscale ordering, which can only…