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We propose an approach to probe coherent spin-state dynamics of molecules using circularly polarized hard x-ray pulses. For the dynamically aligned nitric oxide molecules in a coherent superposition spin-orbit coupled electronic state that…

Optics · Physics 2024-01-02 Xiaoyu Mi , Ming Zhang , Zheng Li

Bragg coherent X-ray diffraction imaging (BCDI) is a non-destructive, lensless method for 3D-resolved, nanoscale strain imaging in micro-crystals. A challenge, particularly for new users of the technique, is accurate mapping of experimental…

Materials Science · Physics 2021-03-05 David Yang , Nicholas W. Phillips , Felix Hofmann

We present time-resolved x-ray reflectivity measurements on laser excited coherent and incoherent surface deformations of thin metallic films. Based on a kinematical diffraction model, we derive the surface amplitude from the diffracted…

Lensless X-ray imaging provides element-specific nanoscale insights into thick samples beyond the reach of conventional light and electron microscopy. Coherent diffraction imaging (CDI) methods, such as ptychographic tomography, can recover…

We present proof-of-concept imaging measurements of a polycrystalline material that integrate the elements of conventional high-energy X-ray diffraction microscopy with coherent diffraction imaging techniques, and that can enable in-situ…

Coherent x-ray micro-diffraction and local mechanical loading can be combined to investigate the mechanical deformation in crystalline nanostructures. Here we present measurements of plastic deformation in a copper crystal of sub-micron…

Materials Science · Physics 2013-05-31 G. Beutier , M. Verdier , M. De Boissieu , B. Gilles , F. Livet , M. -I. Richard , T. W. Cornelius , S. Labat , O. Thomas

Visualization of internal deformation fields in crystalline materials helps bridge the gap between theoretical models and practical applications. Applying Bragg coherent diffraction imaging under X-ray dynamical diffraction conditions…

Applied Physics · Physics 2025-12-29 Longlong Wu , David Yang , Wei Wang , Shinjae Yoo , Ross J. Harder , Wonsuk Cha , Aiguo Li , Ian K. Robinson

X-ray photon correlation spectroscopy was used to measure the diffusive dynamics of colloidal particles in a shear flow. The results presented here show how the intensity autocorrelation functions measure both the diffusive dynamics of the…

Soft Condensed Matter · Physics 2009-11-13 Sebastian Busch , Torben Haugaard Jensen , Yuriy Chushkin , Andrei Fluerasu

Corrosion is a major concern for many industries, as corrosive environments can induce structural and morphological changes that lead to material dissolution and accelerate material failure. The progression of corrosion depends on nanoscale…

Sophisticated thin film growth techniques increasingly rely on the addition of a plasma component to open or widen a processing window, particularly at low temperatures. However, the addition of the plasma into the growth environment also…

Colloidal gels assembled from nanoparticles (NPs) are a versatile class of soft network-based materials capable of rich dynamic, mechanical, and even optical or magnetic responses to stimuli. Understanding how their hierarchically organized…

Structure determination is a key application of XFELs and 4th generation synchrotron sources, particularly using the coherent and pulsed X-ray radiation from X-ray free-electron lasers (XFEL). Scientific interest focuses on understanding…

Instrumentation and Detectors · Physics 2025-03-07 Markus Kuster , Robert Hartmann , Steffen Hauf , Peter Holl , Tonn Rüter , Lothar Strüder

Correlative microscopy is a powerful technique that combines the advantages of multiple imaging modalities to achieve a comprehensive understanding of investigated samples. For example, fluorescence microscopy provides unique functional…

The routine atomic-resolution structure determination of single particles is expected to have profound implications for probing the structure-function relationship in systems ranging from energy materials to biological molecules.…

The investigation of the static and dynamic structural properties of colloidal systems relies on techniques capable of atomic resolution in real space and femtosecond resolution in time. Recently, the cross-correlation function (CCF)…

Other Condensed Matter · Physics 2015-11-20 Tatiana Latychevskaia , Giulia Fulvia Mancini , Fabrizio Carbone

Time-resolved femtosecond x-ray diffraction patterns from laser-excited molecular iodine are used to create a movie of intramolecular motion with time and space resolution of $30~$fs and $0.3$ \AA . The high spatial fidelity is due to…

We present calculations of the time lags and the coherence function of X-ray photons for a novel model of radiation emission from accretion powered, high-energy sources. Our model involves only Comptonization of soft photons injected near…

Astrophysics · Physics 2009-10-30 Xin-Min Hua , Demosthenes Kazanas , Lev Titarchuk