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Because of their high photon flux, X-ray free-electron lasers (FEL) allow to resolve the structure of individual nanoparticles via coherent diffractive imaging (CDI) within a single X-ray pulse. Since the inevitable rapid destruction of the…

We present a novel axial ptychographic coherent diffractive imaging (AP-CDI) technique designed to overcome the critical throughput bottleneck of conventional methods. By replacing the 2D raster scan with a simple 1D axial scan, our…

Optics · Physics 2025-11-24 Qijun You , Lingshuo Meng , Fangrui Quan , Wei Cao

Coherent X-ray diffraction microscopy is a method of imaging non-periodic isolated objects at resolutions only limited, in principle, by the largest scattering angles recorded. We demonstrate X-ray diffraction imaging with high resolution…

The advent of nonlinear X-ray processes like sum-frequency generation and four-wave mixing raises the possibility of non-linear X-ray imaging, combining the high-resolution and elemental specificity of X-ray imaging with the state…

Optics · Physics 2025-12-18 Arnab Sarkar , Allan S. Johnson

Bragg coherent x-ray diffractive imaging is a powerful technique for investigating dynamic nanoscale processes in nanoparticles immersed in reactive, realistic environments. Its temporal resolution is limited, however, by the oversampling…

Materials Science · Physics 2016-05-25 A. Ulvestad , A. Tripathi , S. O. Hruszkewycz , W. Cha , S. M. Wild , G. B. Stephenson , P. H. Fuoss

Understanding and ultimately controlling the transformations and properties of nanoscale systems, from proteins to synthetic nanomaterial assemblies, is limited by the inability to uncover their dynamics on their characteristic length and…

Modern imaging techniques at the molecular scale rely on utilizing novel coherent light sources like X-ray free electron lasers for the ultimate goal of visualizing such objects as individual biomolecules rather than crystals. Here, unlike…

We present simulations of Bragg Coherent X-ray Diffractive Imaging (CXDI) data from finite crystals in the frame of the dynamical theory of x-ray diffraction. The developed approach is based on numerical solution of modified Takagi-Taupin…

Materials Science · Physics 2017-08-30 A. G. Shabalin , O. M. Yefanov , V. L. Nosik , V. A. Bushuev , I. A. Vartanyants

Coherent X-ray diffraction imaging (CXDI) experiments are intrinsically limited by shot noise, a lack of prior knowledge about the sample's support, and missing measurements due to the experimental geometry. We propose a flexible, iterative…

Biological Physics · Physics 2017-03-03 Liang Shi , Gordon Wetzstein , Thomas J. Lane

We report X-ray Photon Correlation Spectroscopy (XPCS) results on a bidimensional (2D) gel formed by a Langmuir monolayer of gold nanoparticles. The system allows an experimental determination of the fourth order time correlation function…

Soft Condensed Matter · Physics 2012-03-29 D. Orsi , L. Cristofolini , G. Baldi , A. Madsen

Recent advances in the field of attosecond science hold the promise of tracking electronic processes at the shortest space and time scales. Imaging methods that combine attosecond temporal with nanometer spatial resolution are currently out…

Coherent x-ray diffractive imaging is extended to high resolution strain analysis in crystalline nanostructured devices. The application potential is demonstrated by determining the strain distribution in (Ga,Mn)As/GaAs nanowires. By…

Understanding surface dynamics during epitaxial film growth is key to growing high quality materials with controllable properties. X-ray photon correlation spectroscopy (XPCS) using coherent x-rays opens new opportunities for in situ…

We have developed a new method of data processing for radio telescope observation data to measure time-dependent temporal coherence, and we named it cross-correlation spectrometry (XCS). XCS is an autocorrelation procedure that expands time…

Solar and Stellar Astrophysics · Physics 2016-09-28 Kazuhiro Takefuji , Hiroshi Imai , Mamoru Sekido

The morphology and the microscopic internal dynamics of a bidimensional gel formed by spontaneous aggregation of gold nanoparticles confined at the water surface are investigated by a suite of techniques, including grazing-incidence x-ray…

Soft Condensed Matter · Physics 2015-06-19 D. Orsi , B. Ruta , Y. Chushkin , A. Pucci , G. Ruggeri , G. Baldi , T. Rimoldi , L. Cristofolini

X-ray diffraction studies of nanoporous gold face the poorly understood diffraction scenario where large coherent crystals are riddled with nanoscale holes. Theoretical considerations derived in this study show that the ligament size of the…

Materials Science · Physics 2017-12-27 Matthias Graf , Bao-Nam Dinh Ngô , Jörg Weissmüller , Jürgen Markmann

This study explores the possibility to measure dynamics of proteins in solution using X-ray photon correlation spectroscopy (XPCS) at nearly diffraction limited storage rings (DLSR). We calculate the signal to noise ratio (SNR) of XPCS…

Instrumentation and Detectors · Physics 2019-10-01 Johannes Möller , Michael Sprung , Anders Madsen , Christian Gutt

Coherent diffractive imaging has enabled the structural analysis of individual free nanoparticles in a single shot and offers the tracking of their light induced dynamics with unprecedented spatial and temporal resolution. The retrieval of…

Optics · Physics 2020-05-07 Björn Kruse , Benjamin Liewehr , Christian Peltz , Thomas Fennel

Grain-boundary (GB) dynamics control the stability, mechanical, and functional response of nanocrystalline materials, but direct experimental access to their slow non-equilibrium motion has been limited. Here we establish X-ray photon…

We report on a new x-ray imaging method, which combines the high spatial resolution of coherent diffraction imaging with the ability of dark field microscopy to map grains within thick polycrystalline specimens. An x-ray objective serves to…

Instrumentation and Detectors · Physics 2020-07-15 Anders Filsøe Pedersen , Virginie Chamard , Carsten Detlefs , Tao Zhou , Dina Carbone , Henning Friis Poulsen