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X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…

Unique intensity features arising from dynamical diffraction arise in coherent x-ray nanobeam diffraction patterns of crystals having thicknesses larger than the x-ray extinction depth or exhibiting combinations of nanoscale and mesoscale…

Materials Science · Physics 2020-02-27 A. Pateras , J. Park , Y. Ahn , J. A. Tilka , M. V. Holt , H. Kim , L. J. Mawst , P. G. Evans

Two-color X-ray imaging with Free Electron Laser pulses offers a powerful approach for probing ultrafast structural dynamics in nanoscale systems, combining (near-)atomic spatial resolution with femtosecond temporal precision. The first…

Coherent diffraction imaging (CDI) of single molecules at atomic resolution is a major goal for the x-ray free electron lasers (XFELs). However, during an imaging pulse, the fast laser-induced ionization may strongly affect the recorded…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Zoltan Jurek , Robert Thiele , Beata Ziaja , Robin Santra

Using simultaneous observations in X-rays and optical, we have performed a homogeneous analysis of the cross-correlation behaviours of four X-ray binaries: SWIFT J1753.5-0127, GX 339-4, Sco X-1, and Cyg X-2. With high time-resolution…

We present a first experiment combining high pression and coherent X-ray diffraction. By using a dedicated diamond anvil cell, we show that the degree of coherence of the X-ray beam is preserved when the X-ray beam passes through the…

Other Condensed Matter · Physics 2015-05-14 D. Le Bolloc'h , J. P. Itié , A. Polian , S. Ravy

We demonstrate that in situ coherent diffractive imaging (CDI), which harnesses the coherent interference between a strong and a weak beam illuminating a static and dynamic structure, can be a very dose-efficient imaging method. At low…

We report the development of deep learning coherent electron diffractive imaging at sub-angstrom resolution using convolutional neural networks (CNNs) trained with only simulated data. We experimentally demonstrate this method by applying…

Materials Science · Physics 2022-04-19 Dillan J. Chang , Colum M. O'Leary , Cong Su , Salman Kahn , Alex Zettl , Jim Ciston , Peter Ercius , Jianwei Miao

The highly transient nature of shock loading and pronounced microstructure effects on dynamic materials response call for {\it in situ}, temporally and spatially resolved, x-ray-based diagnostics. Third-generation synchrotron x-ray sources…

Other Condensed Matter · Physics 2015-06-04 S. N. Luo , B. J. Jensen , D. E. Hooks , K. Fezzaa , K. J. Ramos , J. D. Yeager , K. Kwiatkowski , 1 , T. Shimada

This paper introduces Spectral Incoherent Diffractive Imaging (SIDI) as a novel method for achieving dark-field imaging of nanostructures with heterogeneous oxidation states. With SIDI, shifts in photoemission profiles can be spatially…

Optics · Physics 2023-12-25 Tamme Wollweber , Kartik Ayyer

We have developed a 3 dimensional Coherent Diffraction Imaging (CDI) algorithm to retrieve phases of diffraction patterns of samples in Grazing Incidence Small Angle X-ray Scattering (GISAXS) experiments. The algorithm interprets the…

Instrumentation and Detectors · Physics 2023-07-26 Yi Yang , Sunil K. Sinha

Established x-ray diffraction methods allow for high-resolution structure determination of crystals, crystallized protein structures or even single molecules. While these techniques rely on coherent scattering, incoherent processes like…

Coherent diffraction imaging is a high-resolution imaging technique whose potential can be greatly enhanced by applying the extrapolation method presented here. We demonstrate enhancement in resolution of a non-periodical object…

We developed a microscope intended to probe, using a parallel heterodyne receiver, the fluctuation spectrum of light quasi-elastically scattered by gold nanoparticles diffusing in viscous fluids. The cutoff frequencies of the recorded…

Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…

Instrumentation and Detectors · Physics 2020-05-06 Yanwen Sun , Mike Dunne , Paul Fuoss , Taito Osaka , Aymeric Robert , Mark Sutton , Makina Yabashi , Diling Zhu

Coherent diffractive imaging (CDI), using both X-rays and electrons, has made extremely rapid progress over the past two decades. The associated reconstruction algorithms are typically iterative, and seeded with a crude first estimate. A…

Image and Video Processing · Electrical Eng. & Systems 2019-06-25 Konstantin M. Pavlov , Kaye S. Morgan , Vasily I. Punegov , David M. Paganin

Confocal x-ray fluorescence microscopy (CXRF) allows direct detection of x-ray fluorescence from a micron-scale 3D volume of an extended, unthinned sample. We have previously demonstrated the use of a novel collection optic, fabricated from…

Instrumentation and Detectors · Physics 2016-07-07 David N Agyeman-Budu , Sanjukta Choudhury , Ian Coulthard , Robert Gordon , Emil Hallin , Arthur R Woll

We have developed an improved method of time-resolved x-ray reflectivity (XRR) using monochromatic synchrotron radiation. Our method utilizes a polycapillary x-ray optic to create a range of incident angles and an area detector to collect…

Materials Science · Physics 2019-03-27 Howie Joress , Shane Quinlan Arlington , Timothy P. Weihs , Joel D. Brock , Arthur Woll

Complex-field imaging is indispensable for numerous applications at wavelengths from X-ray to THz, with amplitude describing transmittance (or reflectivity) and phase revealing intrinsic structure of the target object. Coherent diffraction…

Image and Video Processing · Electrical Eng. & Systems 2021-04-07 Meng Li , Liheng Bian , Guoan Zheng , Andrew Maiden , Yang Liu , Yiming Li , Qionghai Dai , Jun Zhang

Understanding and interpreting dynamics of functional materials \textit{in situ} is a grand challenge in physics and materials science due to the difficulty of experimentally probing materials at varied length and time scales. X-ray photon…