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The growing demand for efficient energy storage has driven the search for advanced anode materials for lithium- and sodium-ion batteries (LIBs and SIBs). In this context, we report the application of HOP-graphene (a 5-6-8-membered 2D carbon…

Density function theory calculations were carried out to clarify storage states of Lithium (Li) ions in graphene clusters. The adsorption energy, spin polarization, charge distribution, electronic gap, surface curvature and dipole momentum…

Materials Science · Physics 2015-06-03 N. Kheirabadi , A. Shafiekhani

We propose fabrication of the fiber-shaped lithium ion batteries assembled by twisting a cathode filament together with an anode filament. The cathode filament is fabricated by depositing a LiFePO4 (LFP)-composite layer onto a steel-filled…

Applied Physics · Physics 2018-01-16 Hang Qu , Xin Lu , Maksim Skorobogatiy

We carefully investigated the storage of lithium in titania films on various substrates as a function of thickness. The experiments enable us to precisely separate contributions from bulk and boundary storage. The battery capacity…

Chemical Physics · Physics 2023-03-24 Chuanlian Xiao , Hongguang Wang , Peter A. van Aken , Robert Usiskin , Joachim Maier

Lithium (Li) metal anodes are essential for developing next-generation high-energy-density batteries. However, Li dendrite/whisker formation caused short-circuiting issue and short cycle life have prevented lithium metal from being viably…

Materials Science · Physics 2022-05-02 Bingyu Lu , Wurigumula Bao , Weiliang Yao , Jean-Marie Doux , Chengcheng Fang , Ying Shirley Meng

Linking electrode microstructure to electrochemical performance is essential for optimizing Li-ion batteries. However, this requires mechanistic 4D observations at ultimate spatio-temporal scales, which remains elusive. Here we demonstrate…

The growth of the semiconductor and solar industry has been exponential in the last two decades due to the computing and energy demands of the world. Silicon (Si) is one of the main constituents for both sectors and, thus, is used in large…

Recent years have seen a rapidly escalating demand for battery technologies capable of storing more energy, charging more quickly and having longer usable lifetimes, driven largely by increased electrification of transport and by grid-scale…

Li+ transport within a solid electrolyte interphase (SEI) in lithium ion batteries has challenged molecular dynamics (MD) studies due to limited compositional control of that layer. In recent years, experiments and ab initio simulations…

Chemical Physics · Physics 2018-01-29 Ajay Muralidharan , Mangesh I. Chaudhari , Lawrence R. Pratt , Susan B. Rempe

Understanding solid liquid interfaces at high spatial and chemical resolution is crucial for advancing electrochemical energy storage technologies, yet this remains a persistent challenge due to the lack of characterisation techniques that…

Sodium-ion batteries have gained much interest over the past years and especially layered oxides are highly considered as cathodes for the next generation of batteries. However, there are still significant challenges to overcome in these…

Materials Science · Physics 2025-12-09 Konstantin Köster , Payam Kaghazchi

This theoretical investigation delves into the structural, electronic, and electrochemical properties of two hexagonal iron-arsenide monolayers, 1T-FeAs and 1H-FeAs, focusing on their potential as anode materials for Lithium-ion batteries.…

Materials Science · Physics 2025-01-28 Ajay Kumar , Prakash Parida

Lithium intercalation into graphite is the foundation for the lithium-ion battery, and the thermodynamics of the lithiation of graphitic electrodes have been heavily investigated. Intercalated lithium in bulk graphite undergoes structural…

Materials Science · Physics 2022-01-06 Joshua V. Pondick , Sajad Yazdani , Milad Yarali , Serrae N. Reed , David J. Hynek , Judy J. Cha

Spatially-resolved neutron powder diffraction with gauge volume 2x2x20 mm3 has been applied to probe the lithium concentration in the graphite anode of different Li-ion cells of 18650-type in situ in charged state. Structural studies…

Materials Science · Physics 2015-03-27 A. Senyshyn , M. J. Mühlbauer , O. Dolotko , M. Hofmann , H. Ehrenberg

A flexible, light weight and high conductivity current collector is the key element that enables fabrication of high performance flexible lithium ion battery. Here we report a thin, light weight and flexible lithium ion battery that uses…

Chemical Physics · Physics 2015-11-13 Hang Qu , Jingshan Hou , Yufeng Tang , Oleg Semenikihin , Maksim Skorobogatiy

Layered LiMnO$_2$ and Li$_2$MnO$_3$ are of great interest for lithium-ion battery cathodes because of their high theoretical capacities. The practical application of these materials is, however, limited due to poor electrochemical…

Materials Science · Physics 2015-02-25 Khang Hoang

We have studied low-temperature magnetic properties as well as high-temperature lithium ion diffusion in the battery cathode materials LixNi1/3Co1/3Mn1/3O2 by the use of muon spin rotation/relaxation. Our data reveal that the samples enter…

Materials Science · Physics 2015-06-22 M. Mansson , H. Nozaki , J. M. Wikberg , K. Prsa , Y. Sassa , M. Dahbi , K. Kamazawa , K. Sedlak , I. Watanabe , J. Sugiyama

Mg batteries with oxide cathodes have the potential to significantly surpass existing Li-ion technologies in terms of sustainability, abundance, and energy density. However, Mg intercalation at the cathode is often severely hampered by the…

Materials Science · Physics 2023-03-21 Mohsen Sotoudeh , Manuel Dillenz , Johannes Döhn , Julian Hansen , Sonia Dsoke , Axel Groß

Long-term durability is a major obstacle limiting the widespread use of lithium ion batteries (LIBs) in heavy-duty applications and others demanding extended lifetime. As one of the root causes of degradation and failure of battery…

It is well-known that the microstructure of electrodes in lithium-ion batteries strongly affects their performance. Vice versa, the microstructure can exhibit strong changes during the usage of the battery due to aging effects. For a better…

Materials Science · Physics 2018-01-15 Klaus Kuchler , Daniel Westhoff , Julian Feinauer , Tim Mitsch , Ingo Manke , Volker Schmidt