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The presence of small hematite (Fe2O3) clusters at low coverage on titanium dioxide (TiO2) surface has been observed to enhance photocatalytic activity, while excess loading of hematite is detrimental. We conduct a comprehensive density…

Materials Science · Physics 2024-04-09 Kati Asikainen , Matti Alatalo , Marko Huttula , Bernardo Barbiellini , S. Assa Aravindh

Titanium dioxide (TiO$_2$) has rich physical properties with potential implications in both fundamental physics and new applications. Up-to-date, the main focus of applied research is to tune its optical properties, which is usually done…

Twistronics, originally conceptualized within the electronics domain to modulate electronic properties through the twist angle between stacked two-dimensional (2D) materials, presents a groundbreaking approach in material science. This…

Applied Physics · Physics 2024-02-22 Ingrid Torres , Alex Krasnok

The electronic properties of quasi-one-dimensional anatase TiO2 nanostructures, in the form of thin nanowires having (101) and (001) facets, have been systematically investigated using the standard, hybrid density functional and…

Mesoscale and Nanoscale Physics · Physics 2014-07-08 Hatice Unal , Oguz Gulseren , Sinasi Ellialtioglu , Ersen Mete

We demonstrate control of the carrier density of single phase anatase TiO2 thin films by nearly two orders of magnitude by modulating the growth kinetics during pulsed laser deposition, under fixed thermodynamic conditions. The resistivity…

Materials Science · Physics 2015-06-05 T. Tachikawa , M. Minohara , Y. Nakanishi , Y. Hikita , M. Yoshita , H. Akiyama , C. Bell , H. Y. Hwang

We perform first-principles calculations to investigate the band structure, density of states, optical absorption, and the imaginary part of dielectric function of Cu, Ag, and Au-doped anatase TiO2 in 72 atoms systems. The electronic…

Materials Science · Physics 2015-08-10 Meili Guo , Jiulin Du

Light chargeable metal-ion batteries using semiconductor heterostructures are gaining enormous interest. A few such heterostructures such as MoS2/MoOy and TiS2/TiO2 have been shown to function as photocathodes in photochargeable Li-ion…

Materials Science · Physics 2023-07-07 Raheel Hammad , Amar Kumar , Tharangattu N. Narayanan , Soumya Ghosh

The rutile TiO$_2$ (110) surface reduced by the bridging oxygen vacancy, bridging hydroxyl group or Ti interstitial atom has been investigated by calculating their electronic structures using the density functional theory plus U method. It…

Materials Science · Physics 2015-10-13 Daoyu Zhang , Minnan Yang , Shuai Dong

We report the existence of metallic two-dimensional electron gases (2DEGs) at the (001) and (101) surfaces of bulk-insulating TiO2 anatase due to local chemical doping by oxygen vacancies in the near-surface region. Using angle-resolved…

Materials Science · Physics 2015-07-15 T. C. Rödel , F. Fortuna , F. Bertran , M. Gabay , M. J. Rozenberg , A. F. Santander-Syro , P. Le Fèvre

There is immense interest in how the local environment influences the electronic structure of materials at the single layer limit. We characterize moir\'e induced spatial variations in the electronic structure of in-situ grown monolayer…

Atomically thin semiconductors exhibit tunable exciton resonances that can be harnessed for dynamic manipulation of visible light in ultra-compact metadevices. However, the rapid nonradiative decay and dephasing of excitons at room…

Optics · Physics 2025-02-18 Tom Hoekstra , Jorik van de Groep

We have used density functional theory calculations based on the projector augmented wave method to investigate the electronic structure of Au-incorporated anatase TiO$_2$(001) surface. Due to the coordination with several level oxygens, Au…

Strongly Correlated Electrons · Physics 2009-07-18 E. Mete , O. Gulseren , S. Ellialtioglu

The quasiparticle electronic structure and optical excitation of anatase TiO$_2$ is determined within the framework of many-body perturbation theory (MBPT) by combining the $G_0W_0$ method and the Bethe-Salpeter Equation (BSE). A modified…

Materials Science · Physics 2021-12-07 Sruthil Lal S. B , D Murali , Matthias Posselt , Assa Aravindh Sasikala Devi , Alok Sharan

We determine the surface reconstruction of SrTiO3 used to achieve superconducting FeSe films in experiments, which is different from the 1x1 TiO2 terminated SrTiO3 assumed by most previous theoretical studies. In particular, we identify the…

Structural and electronic properties comparison between anatase, rutile and monoclinic TiO2(B) titania polymorphs in bulk and related nanostructures simulated by two-dimensional slabs has been performed by means of density functional theory…

Materials Science · Physics 2011-08-16 Luciana Fernández-Werner , Ricardo Faccio , Helena Pardo , Álvaro W. Mombrú

Wrinkles and nanobubbles are an integral and often unavoidable part of integrating 2D van der Waals semiconductors into actual device architectures. Despite their ubiquitous nature, quantitative correlation between such spatially…

Materials Science · Physics 2026-04-01 Soumyadip Hazra , Sraboni Dey , Arijit Kayal , Narendra Shah , Renjith Nadarajan , Joy Mitra

Understanding and controlling the photoexcited quasiparticle (QP) dynamics in monolayer transition metal dichalcogenides lays the foundation for exploring the strongly interacting, non-equilibrium 2D quasiparticle and polaritonic states in…

Materials Science · Physics 2024-10-04 Akiyoshi Park , Rohit Kantipudi , Jonas Göser , Yinan Chen , Duxing Hao , Nai-Chang Yeh

The present work reports on the enhancement of TiO2 nanotubes photoelectrochemical water splitting rate by decorating the nanostructure with an amine layer in a hydrothermal process using diethylenetriamine (DETA). The aminate coated TiO2…

Materials Science · Physics 2016-10-14 Seyedsina Hejazi , Nhat Truong Nguyen , Anca Mazare , Patrik Schmuki

Here we report a strategy, by taking a prototypical model system for photocatalysis (viz. N-doped (TiO$_2$)$_n$ clusters), to accurately determine low energy metastable structures that can play a major role with enhanced catalytic…

Materials Science · Physics 2021-01-26 Shikha Saini , Pooja Basera , Manish Kumar , Preeti Bhumla , Saswata Bhattacharya

In this work we study the electronic structure and magnetism of a TiO2 film grown on another non-magnetic oxide such as a LaAlO3 (001) substrate, concentrating on the role played by structural relaxation and oxygen vacancies. Using Density…

Materials Science · Physics 2008-11-14 Valeria Ferrari , Mariana Weissmann