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We study the effective spin-orbital model for honeycomb-layered transition metal compounds, applying the second-order perturbation theory to the three-orbital Hubbard model with the anisotropic hoppings. This model is reduced to the Kitaev…

Strongly Correlated Electrons · Physics 2018-04-04 Akihisa Koga , Shiryu Nakauchi , Joji Nasu

Intensive studies of the interplay between spin-orbit coupling (SOC) and electronic correlations in transition metal compounds have recently been undertaken. In particular, $j_{\rm eff}$ = 1/2 bands on a honeycomb lattice provide a pathway…

Strongly Correlated Electrons · Physics 2015-06-24 Heung-Sik Kim , V. Vijay Shankar , Andrei Catuneanu , Hae-Young Kee

Kitaev spin liquid is proposed to be promisingly realized in low spin-orbit coupling $3d$ systems, represented by Na$_3$Co$_2$SbO$_6$ and Na$_3$Ni$_2$BiO$_6$. However, the existence of Kitaev interaction is still debatable among…

Strongly Correlated Electrons · Physics 2024-06-10 Zefeng Chen , Binhua Zhang , Weiqin Zhu , Lianchuang Li , Boyu Liu , Junsheng Feng , Changsong Xu , Hongjun Xiang

We report on magnetization $M(H)$, dc/ac magnetic susceptibility $\chi(T)$, specific heat $C_{\mathrm{m}}(T)$ and muon spin relaxation ($\mu$SR) measurements of the Kitaev honeycomb iridate Cu$_2$IrO$_2$ with quenched disorder. In spite of…

The triangular-lattice system $\alpha$-RuI$_3$ is isostructural to the widely-studied $\alpha$-RuCl$_3$ compound which was identified as a potential Kitaev system but exhibits, instead of spin liquid behaviour, a magnetically ordered…

Strongly Correlated Electrons · Physics 2024-06-07 Hank C. H. Wu , Benjamin M. Huddart , Francis L. Pratt , Danrui Ni , Robert J. Cava , Stephen J. Blundell

The nature of the effective spin Hamiltonian and magnetic order in the honeycomb iridates is explored by considering a trigonal crystal field effect and spin-orbit coupling. Starting from a Hubbard model, an effective spin Hamiltonian is…

Strongly Correlated Electrons · Physics 2012-07-10 Subhro Bhattacharjee , Sung-Sik Lee , Yong Baek Kim

Recently, honeycomb cobaltates with 3$d^7$ were proposed to display Kitaev physics despite weak spin-orbit coupling. However, other theoretical and experimental works found leading XXZ Heisenberg and negligible Kitaev interactions in…

Strongly Correlated Electrons · Physics 2023-03-01 Xiaoyu Liu , Hae-Young Kee

We study a $\mathbb{Z}_3$ Kitaev model on the honeycomb lattice with nearest neighbor interactions. Based on matrix product state simulations and symmetry considerations, we find evidence that, with ferromagnetic isotropic couplings, the…

Strongly Correlated Electrons · Physics 2024-04-29 Li-Mei Chen , Tyler D. Ellison , Meng Cheng , Peng Ye , Ji-Yao Chen

We report a combined experimental and theoretical investigation of the magnetic structure of the honeycomb lattice magnet Na$_2$IrO$_3$, a strong candidate for a realization of a gapless spin-liquid. Using resonant x-ray magnetic scattering…

Materials Science · Physics 2011-07-12 X. Liu , T. Berlijn , W. -G. Yin , W. Ku , A. Tsvelik , Young-June Kim , H. Gretarsson , Yogesh Singh , P. Gegenwart , J. P. Hill

The electronic ground state in many iridate materials is described by a complex wave-function in which spin and orbital angular momenta are entangled due to relativistic spin-orbit coupling (SOC). Such a localized electronic state carries…

The Kitaev quantum spin liquid (KSL) is a theoretically predicted state of matter whose fractionalized quasiparticles are distinct from bosonic magnons, the fundamental excitation in ordered magnets. The layered honeycomb antiferromagnet…

We explore the phase diagram of the Kitaev-Heisenberg model with nearest neighbor interactions on the honeycomb lattice using the exact diagonalization of finite systems combined with the cluster mean field approximation, and supplemented…

Strongly Correlated Electrons · Physics 2017-02-01 Dorota Gotfryd , Juraj Rusnačko , Krzysztof Wohlfeld , George Jackeli , Jiří Chaloupka , Andrzej M. Oleś

Li3Co2SbO6 is prepared by molten salt ion exchange and its structure refined by the Rietveld method confirming the honeycomb-type Co/Sb ordering of its Na precursor. Monoclinic rather than trigonal symmetry of Na3Co2SbO6 is directly…

Quantum spin liquid is a disordered magnetic state with fractional spin excitations. Its clearest example is found in an exactly solved Kitaev honeycomb model where a spin flip fractionalizes into two types of anyons, quasiparticles that…

Strongly Correlated Electrons · Physics 2018-05-10 N. Janša , A. Zorko , M. Gomilšek , M. Pregelj , K. W. Krämer , D. Biner , A. Biffin , Ch. Rüegg , M. Klanjšek

Building upon the spin-1/2 Kitaev model on a honeycomb lattice, the Yao-Lee spin-orbital model provides exactly solvable quantum spin liquids with potentially better stability against perturbations due to the additional degree of freedom.…

Strongly Correlated Electrons · Physics 2026-05-21 Jiefu Cen , Hae-Young Kee

We report a $^{35}$Cl nuclear magnetic resonance study in the honeycomb lattice, $\alpha$-RuCl$_3$, a material that has been suggested to potentially realize a Kitaev quantum spin liquid (QSL) ground state. Our results provide direct…

Strongly Correlated Electrons · Physics 2017-07-26 S. -H. Baek , S. -H. Do , K. -Y. Choi , Y. S. Kwon , A. U. B. Wolter , S. Nishimoto , Jeroen van den Brink , B. Büchner

We study the emergence of magnetic order in localized spins that interact solely through their coupling to a Kitaev-type spin liquid. Using three toy models -- the Kitaev model, the Yao-Lee model, and a square-lattice generalization of the…

Strongly Correlated Electrons · Physics 2025-07-09 M. A. Keskiner , M. Ö. Oktel , Natalia B. Perkins , Onur Erten

We report on the results of 23Na NMR in the honeycomb lattice magnet Na2Co2TeO6 which has been nominated as a Kitaev material. Measurements of magnetic shift and width of the NMR line as functions of temperature and magnetic field show that…

Strongly Correlated Electrons · Physics 2022-12-21 Jun Kikuchi , Takayuki Kamoda , Nobuyoshi Mera , Yodai Takahashi , Kouji Okumura , Yukio Yasui

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

Strongly Correlated Electrons · Physics 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

Recent advances in the study of cobaltites have unveiled their potential as a promising platform for realizing Kitaev physics in honeycomb systems and the Ising model in weakly coupled chain materials. In this manuscript, we explore the…