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Honeycomb iridates are thought to have strongly spin-anisotropic exchange interactions that could lead to an extraordinary state of matter known as the Kitaev quantum spin liquid. The realization of this state requires almost perfectly…

Quantum spin liquid involves fractionalized quasipariticles such as spinons and visons. They are expressed as itinerant Majorana fermions and $Z_2$ fluxes in the Kitaev model with bond-dependent exchange interactions on a honeycomb spin…

Strongly Correlated Electrons · Physics 2020-02-05 Y. Nagai , T. Jinno , Y. Yoshitake , J. Nasu , Y. Motome , M. Itoh , Y. Shimizu

The layered honeycomb iridate $\alpha$-Li$_2$IrO$_3$ displays an incommensurate magnetic structure with counterrotating moments on nearest-neighbor sites, proposed to be stabilized by strongly-frustrated anisotropic Kitaev interactions…

Strongly Correlated Electrons · Physics 2019-03-06 Sungkyun Choi , S. Manni , J. Singleton , C. V. Topping , T. Lancaster , S. J. Blundell , D. T. Adroja , V. Zapf , P. Gegenwart , R. Coldea

We report results of our study of a newly synthesized honeycomb iridate NaxIrO3 (0.60 < x < 0.80). Single-crystal NaxIrO3 adopts a honeycomb lattice noticeably without distortions and stacking disorder inherently existent in its sister…

Strongly Correlated Electrons · Physics 2021-07-28 Hengdi Zhao , Bing Hu , Feng Ye , Minhyea Lee , Pedro Schlottmann , Gang Cao

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

The magnetic orders in Na$_2$IrO$_3$ and $\alpha-$RuCl$_3$, honeycomb systems with strong spin-orbit coupling and correlations, have been recently described by models with the dominant Kitaev interactions. In this work we discuss how the…

Strongly Correlated Electrons · Physics 2017-02-10 Yuriy Sizyuk , Peter Woelfle , Natalia B. Perkins

In extended Heisenberg-Kitaev-Gamma-type spin models, hidden-SU(2)-symmetric points are isolated points in parameter space that can be mapped to pure Heisenberg models via nontrivial duality transformations. Such points generically feature…

Strongly Correlated Electrons · Physics 2023-10-11 Wilhelm G. F. Krüger , Wenjie Chen , Xianghong Jin , Yuan Li , Lukas Janssen

The quest for quantum spin liquids has garnered significant attention due to their rich physics and disruptive prospects in quantum communication and computation. Spin-orbit coupling, electron correlation, and structural distortion play…

Strongly Correlated Electrons · Physics 2024-12-24 Deepak K Roy , Mukul Kabir

Recent work shows that a quantum spin liquid can arise in realistic fermionic models on a honeycomb lattice. We study the quantum spin-1/2 Heisenberg honeycomb model, considering couplings J1, J2, and J3 up to third nearest neighbors. We…

Strongly Correlated Electrons · Physics 2015-05-27 Johannes Reuther , Dmitry Abanin , Ronny Thomale

The Kitaev spin model offers an exact quantum spin liquid in the ground state, which has stimulated exploration of its material realization over the last decade. Thus far, most of the candidates are found in $4d$- and $5d$-electron…

Strongly Correlated Electrons · Physics 2020-11-03 Seong-Hoon Jang , Ryoya Sano , Yasuyuki Kato , Yukitoshi Motome

The Kitaev honeycomb model provides a paradigmatic example of an exactly solvable quantum spin liquid (QSL), in which the spin degrees of freedom fractionalize into itinerant Majorana fermions coupled to a static background of…

Strongly Correlated Electrons · Physics 2024-06-28 Vitor Dantas , Wen-Han Kao , Natalia B. Perkins

The 5d-electron honeycomb compound H$_3$LiIr$_2$O$_3$ [K. Kitagawa $et$ $al.$, Nature 554, 341-345 (2018)] exhibits an apparent quantum spin liquid (QSL) state. In this intercalated spin-orbital compound, a remarkable pile up of low-energy…

Strongly Correlated Electrons · Physics 2019-02-07 Johannes Knolle , Roderich Moessner , Natalia B. Perkins

We performed 23Na NMR measurements on a single-domain crystal of the Kitaev material Na3Co2SbO6, with magnetic field applied along the crystalline a axis. A positive Curie-Weiss constant is obtained from the NMR Knight shift, which suggests…

Strongly Correlated Electrons · Physics 2024-02-14 Ze Hu , Yue Chen , Yi Cui , Shuo Li , Cong Li , Xiaoyu Xu , Ying Chen , Xintong Li , Yuchen Gu , Rong Yu , Rui Zhou , Yuan Li , Weiqiang Yu

Quantum spin liquids (QSLs) host a variety of fractionalized particles. In Kitaev's paradigmatic honeycomb model a spin-$\tfrac{1}{2}$ fractionalizes into $Z_2$ flux due to emergent $Z_2$ gauge field and matter Majorana fermions. Although…

Strongly Correlated Electrons · Physics 2026-01-22 Shi Feng , Nandini Trivedi

We report the magnetic structure and electronic properties of the honeycomb antiferromagnet $\rm NaNi_2BiO_{5.66}$. We find magnetic order with moments along the $c$ axis for temperatures below $T_{c1}=6.3(1)\>{\rm K}$ and then in the…

Strongly Correlated Electrons · Physics 2019-12-25 A. Scheie , K. Ross , P. Peter Stavropoulos , E. Seibel , J. A. Rodriguez-Rivera , J. A. Tang , Yi Li , Hae-Young Kee , R. J. Cava , C. Broholm

The family of edge-sharing tri-coordinated iridates and ruthenates has emerged in recent years as a major platform for Kitaev spin liquid physics, where spins fractionalize into emergent magnetic fluxes and Majorana fermions with Dirac-like…

Kitaev materials are promising materials for hosting quantum spin liquids and investigating the interplay of topological and symmetry-breaking phases. We use an unsupervised and interpretable machine-learning method, the tensorial-kernel…

Strongly Correlated Electrons · Physics 2021-04-06 Ke Liu , Nicolas Sadoune , Nihal Rao , Jonas Greitemann , Lode Pollet

Compounds of transition metal ions with strong spin-orbit coupling recently attracted attention due to the possibility to host frustrated bond-dependent anisotropic magnetic interactions. In general, such interactions lead to complex phase…

Strongly Correlated Electrons · Physics 2019-02-21 Juraj Rusnačko , Dorota Gotfryd , Jiří Chaloupka

We report the existence of a phase transition at high temperature in the 3D Kitaev candidate material, $\beta$-Li$_2$IrO$_3$. We show that the transition is bulk, intrinsic and orders a tiny magnetic moment with a spatially anisotropic…

While phase transitions between magnetic analogs of three states of matter --- a long-range ordered state, paramagnet, and spin liquid --- have been extensively studied, the possibility of "liquid-liquid" transitions, namely, between…

Strongly Correlated Electrons · Physics 2017-04-05 Joji Nasu , Yasuyuki Kato , Junki Yoshitake , Yoshitomo Kamiya , Yukitoshi Motome