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The honeycomb Kitaev model in a magnetic field is a source of a topological quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. We present experimental results for the thermal Hall effect of…

Strongly Correlated Electrons · Physics 2019-03-06 Richard Hentrich , Maria Roslova , Anna Isaeva , Thomas Doert , Wolfram Brenig , Bernd Büchner , Christian Hess

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

Mott insulators with strong spin-orbit coupling display a strongly anisotropic response to applied magnetic fields. This applies in particular to Kitaev materials, with $\alpha$-RuCl$_3$ and Na$_2$IrO$_3$ representing two important…

Strongly Correlated Electrons · Physics 2020-10-06 Eric C. Andrade , Lukas Janssen , Matthias Vojta

Layered {\alpha}-RuCl3 is a promising material to potentially realize the long-sought Kitaev quantum spin liquid with fractionalized excitations. While evidence of this exotic state has been reported under a modest in-plane magnetic field,…

Quantum spin liquids can arise from Kitaev magnetic interactions, and exhibit fractionalized excitations with the potential for a topological form of quantum computation. This review surveys recent experimental and theoretical progress on…

$\alpha$-RuCl$_3$ is considered to be the top candidate material for the experimental realization of the celebrated Kitaev model. It is however known that additional interactions beyond the Kitaev model trigger in $\alpha$-RuCl$_3$, a…

$\alpha$-RuCl$_3$ is a Mott insulator with a honeycomb lattice with strong spin-orbit coupling. We report dielectric measurements on $\alpha$-RuCl$_3$ single crystals under field. At zero field, the dielectric constant, $\epsilon$, drops…

Strongly Correlated Electrons · Physics 2018-02-20 Jia-Cheng Zheng , Yi Cui , Tian-Run Li , Ke-Jing Ran , Jinsheng Wen , Weiqiang Yu

The 2D layered insulator $\alpha$-RuCl$_3$ is a candidate material for a quantum spin-liquid state, which may be realized when a magnetic field suppresses the antiferromagnetic order present at low temperature. Oscillations in the field…

Strongly Correlated Electrons · Physics 2023-02-10 Étienne Lefrançois , Jordan Baglo , Quentin Barthélemy , Subin Kim , Young-June Kim , Louis Taillefer

Layered $\alpha$-RuCl3 has been discussed as a proximate Kitaev spin liquid compound. Raman and THz spectroscopy of magnetic excitations confirm that the low-temperature antiferromagnetic ordered phase features a broad Raman continuum,…

The honeycomb Kitaev-Heisenberg model is a source of a quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. In the quest of finding a pertinent material, $\alpha$-RuCl$_{3}$ recently emerged as…

Detailed magnetization, specific heat, and $^7$Li nuclear magnetic resonance (NMR) measurements on single crystals of the hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$ are reported. At high temperatures, {\cred anisotropy of the…

Strongly Correlated Electrons · Physics 2019-07-30 M. Majumder , F. Freund , T. Dey , M. Prinz-Zwick , N. Büttgen , Y. Skourski , A. Jesche , A. A. Tsirlin , P. Gegenwart

Insulating quantum magnets lie at the forefront both of fundamental research into quantum matter and of technological exploitation in the increasingly applied field of spintronics. In this context, the magnetic thermal transport is a…

Strongly Correlated Electrons · Physics 2020-01-22 Christopher A. Pocs , Ian A. Leahy , Hao Zheng , Gang Cao , Eun-Sang Choi , S. -H. Do , Kwang-Yong Choi , B. Normand , Minhyea Lee

We discuss the implications that new magnetocaloric, thermal expansion and magnetostriction data in $\alpha$-RuCl$_{3}$ single crystals have on its temperature-field phase diagram and uncover the magnetic-field dependence of an apparent…

Single crystal inelastic neutron scattering data contain rich information about the structure and dynamics of a material. Yet the challenge of matching sophisticated theoretical models with large data volumes is compounded by computational…

The combination of electronic correlation and spin-orbit coupling is thought to precipitate a variety of highly unusual electronic phases in solids, including topological and quantum spin liquid states. We report a Raman scattering study…

Strongly Correlated Electrons · Physics 2015-04-22 Luke J. Sandilands , Yao Tian , Kemp W. Plumb , Young-June Kim , Kenneth S. Burch

Although (CH3)2NH2CuCl3 (MCCL) was first examined in the 1930's [1], there are open questions regarding the magnetic dimensionality and nature of the magnetic properties. MCCL is proposed to be a S=1/2 alternating ferromagnetic…

Strongly Correlated Electrons · Physics 2009-11-11 M. B. Stone , W. Tian , T. P. Murphy , S. E. Nagler , D. G. Mandrus

The layered honeycomb magnet $\alpha$-RuCl$_3$ has emerged as a promising candidate for realizing a Kitaev quantum spin liquid. Previous studies have reported oscillation-like anomalies in the longitudinal thermal conductivity and…

Strongly Correlated Electrons · Physics 2025-04-01 Y. Xing , R. Namba , K. Imamura , K. Ishihara , S. Suetsugu , T. Asaba , K. Hashimoto , T. Shibauchi , Y. Matsuda , Y. Kasahara

An external magnetic field can induce a transition in $\alpha$-RuCl$_3$ from an ordered zigzag state to a disordered state that is possibly related to the Kitaev quantum spin liquid. Here we present new field dependent inelastic neutron…

Kitaev-type interactions between neighbouring magnetic moments emerge in the honeycomb material ${\alpha}$-RuCl3. It is debated however whether these Kitaev interactions are ferromagnetic or antiferromagnetic. With electron energy loss…

Motivated by impurity-induced magnetic ordering phenomena in spin-gap materials like TlCuCl3, we develop a mean-field theory for strongly disordered antiferromagnets, designed to capture the broad distribution of coupling constants in the…

Strongly Correlated Electrons · Physics 2007-05-23 Heidrun Weber , Matthias Vojta