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We investigate the periodic Anderson model with $\bm{k}$-dependent $c$-$f$ mixing reproducing the point nodes of the hybridization gap by using the dynamical mean-field theory combined with the exact diagonalization method. At low…

Strongly Correlated Electrons · Physics 2012-04-13 Takemi Yamada , Yoshiaki Ōno

We consider the exchange couplings present in an effective Hamiltonian of $\alpha$-RuCl$_3$, known as the K-$\Gamma$ model. This material has a honeycomb lattice, and is expected to be a representative of the Kitaev materials (which can…

Strongly Correlated Electrons · Physics 2022-04-19 Ipsita Mandal

In $\alpha$-RuCl$_3$, an external magnetic field applied within the honeycomb plane can induce a transition from a magnetically ordered state to a disordered state that is potentially related to the Kitaev quantum spin liquid. In zero…

Motivated by the possibility of an intermediate U(1) quantum spin liquid phase in out-of-plane magnetic fields and enhanced magnetic fluctuations in exfoliated {\alpha}-RuCl3 flakes, we study magneto-Raman spectra of exfoliated multilayer…

We investigate the phononic in-plane longitudinal low-temperature thermal conductivity kappa_ab of the Kitaev quantum magnet alpha-RuCl3 for large in-plane magnetic fields up to 33 T. Our data reveal for fields larger than the critical…

The magnetic insulator $\alpha$-RuCl$_{3}$ is a promising candidate to realize Kitaev interactions on a quasi-2D honeycomb lattice. We perform extensive susceptibility measurements on single crystals of $\alpha$-RuCl$_{3}$, including…

We report magnetic and thermodynamic properties of single crystal $\alpha$-RuCl$_3$, in which the Ru$^{3+}$ ($4d^5$) ion is in its low spin state and forms a honeycomb lattice. Two features are observed in both magnetic susceptibility and…

Strongly Correlated Electrons · Physics 2015-04-27 J. A. Sears , M. Songvilay , K. W. Plumb , J. P. Clancy , Y. Qiu , Y. Zhao , D. Parshall , Young-June Kim

In the class of materials called spin liquids, a magnetically ordered state cannot be attained even at milliKelvin temperatures because of conflicting constraints on each spin (for e.g. from geometric or exchange frustration). The resulting…

Increased demand for high-performance permanent magnets in the electric vehicle and wind turbine industries has prompted the search for cost-effective alternatives.Discovering new magnetic materials with the desired intrinsic and extrinsic…

Materials Science · Physics 2024-07-26 Churna Bhandari , Gavin N. Nop , Jonathan D. H. Smith , Durga Paudyal

The honeycomb Mott insulator $\alpha$-RuCl$_3$ loses its low-temperature magnetic order by pressure. We report clear evidence for a dimerized structure at $P>1$ GPa and observe the breakdown of the relativistic $j_{\rm eff}$ picture in this…

The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at…

Pursuing the exotic quantum spin liquid (QSL) state in the Kitaev material $\alpha$-RuCl$_3$ has intrigued great research interest recently. A fascinating question is on the possible existence of field-induced QSL phase in this compound.…

Strongly Correlated Electrons · Physics 2023-09-14 Xu-Guang Zhou , Han Li , Yasuhiro H. Matsuda , Akira Matsuo , Wei Li , Nobuyuki Kurita , Gang Su , Koichi Kindo , Hidekazu Tanaka

We present thermal expansion alpha, magnetostriction and specific heat C measurements of \tal, which shows a quantum phase transition from a spin-gap phase to a Neel-ordered ground state as a function of magnetic field around H_{C0}->4.8T.…

Strongly Correlated Electrons · Physics 2009-11-11 T. Lorenz , S. Stark , O. Heyer , N. Hollmann , A. Vasiliev , A. Oosawa , H. Tanaka

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

Strongly Correlated Electrons · Physics 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

A quantum spin-liquid might be realized in $\alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $\alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic…

Material realization of the non-Abelian Kitaev spin liquid phase - an example of Ising topological order (ITO) - has been the subject of intense research in recent years. The $4d$ honeycomb Mott insulator $\alpha$-RuCl$_3$ has emerged as a…

Strongly Correlated Electrons · Physics 2021-02-26 Jacob S. Gordon , Hae-Young Kee

The magnetic phase diagrams of RMnO3 (R = Er, Yb, Tm, Ho) are investigated up to 14 Tesla via magnetic and dielectric measurements. The stability range of the AFM order below the Neel temperature of the studied RMnO3 extends to far higher…

Strongly Correlated Electrons · Physics 2016-06-29 F. Yen , C. dela Cruz , B. Lorenz , E. Galstyan , Y. Y. Sun , M. Gospodinov , C. W. Chu

We report on the unusual behavior of the in-plane thermal conductivity ($\kappa$) and torque ($\tau$) response in the Kitaev-Heisenberg material $\alpha$-RuCl$_3$. $\kappa$ shows a striking enhancement with linear growth beyond H = 7 T,…

Strongly Correlated Electrons · Physics 2017-05-10 Ian A. Leahy , Christopher A. Pocs , Peter E. Siegfried , David Graf , S. -H. Do , Kwang-Yong Choi , B. Normand , Minhyea Lee

We study the spin-wave excitations in $\alpha$-RuCl$_3$ by the spin-wave theory. Starting from the five-orbital Hubbard model and the perturbation theory, we derive an effective isospin-$1/2$ model in the large Hubbard ($U$) limit. Based on…

Strongly Correlated Electrons · Physics 2017-09-07 Wei Wang , Zhao-Yang Dong , Shun-Li Yu , Jian-Xin Li

We have used a combination of neutron resonant spin-echo and triple-axis spectroscopies to determine the energy, fine structure, and linewidth of the magnon resonance in the model spin-1/2 ladder antiferromagnet IPA-CuCl_3 at temperatures T…

Strongly Correlated Electrons · Physics 2015-03-18 B. Náfrádi , T. Keller , H. Manaka , A. Zheludev , B. Keimer