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We use an open-aperture Z-scan technique to show how intense few-cycle terahertz pulses can experience a nonlinear bleaching of absorption in an n-doped semiconductor due to terahertz-electric-field-driven intervalley scattering of…

Recently, computational sampling methods have been implemented to spatially characterize terahertz (THz) fields. Previous methods usually rely on either specialized THz devices such as THz spatial light modulators, or complicated systems…

Optics · Physics 2019-06-19 Jiapeng Zhao , Yiwen E , Kaia Williams , Xi-cheng Zhang , Robert Boyd

Consider the two-dimensional inverse elastic wave scattering by an infinite rough surface with a Dirichlet boundary condition. A non-interative sampling technique is proposed for detecting the rough surface by taking elastic wave…

Analysis of PDEs · Mathematics 2020-12-15 Tielei Zhu , Jiaqing Yang

Vibrational spectroscopy, comprised of infrared absorption and Raman scattering spectroscopy, is widely used for label-free optical sensing and imaging in various scientific and industrial fields. The group theory states that the two…

Chemical Physics · Physics 2019-10-09 Kazuki Hashimoto , Venkata Ramaiah Badarla , Akira Kawai , Takuro Ideguchi

Two dimensional spectroscopy is a powerful dynamical study method that has been developed in the last two decades. In 2D IR there are three experimental time periods during which the system vibrational modes of interest are excited, evolved…

Chemical Physics · Physics 2021-04-12 S. Tahereh Alavi

The spectrum of terahertz (THz) emission in gases via ionizing two-color femtosecond pulses is analyzed by means of a semi-analytic model and finite-difference-time-domain simulations in 1D and 2D geometries. We show that produced THz…

Plasma Physics · Physics 2015-02-20 Eduardo Cabrera-Granado , Yxing Chen , Ihar Babushkin , Luc Bergé , Stefan Skupin

Non-destructive testing is an important technique for detecting defects in multi-layer materials, enabling the evaluation of structural integrity without causing damage on test materials. Terahertz time-domain spectroscopy (THz-TDS) offers…

Signal Processing · Electrical Eng. & Systems 2025-02-10 Dogus Can Sevdiren , Furkan H. Ilgac , Aydin Sezgin

Terahertz (THz) waves have been significantly developed in the last fifteen years because of their great potential for applications in industrial and scientific communities1,2. The unique properties of THz waves as transparency for numerous…

Optics · Physics 2015-05-27 F. Blanchard , A. Doi , T. Tanaka , H. Hirori , H. Tanaka , Y. Kadoya , K. Tanaka

Since its first demonstration in 1995, terahertz time-domain imaging has attracted an increasingly growing interest for its ability to reveal spectral fingerprints of materials, probe changes in refractive index and absorption, as well as…

The stretching and bending vibrational spectrum and the intensities of infrared transitions in a tetrahedral molecule are studied in two boson-realization models, where the interactions between stretching and bending vibrations are…

Chemical Physics · Physics 2009-10-31 Xi-Wen Hou , Mi Xie , Shi-Hai Dong , Zhong-Qi Ma

Manipulating broadband fields in scattering media is a modern challenge across photonics and other wave domains. Recent studies have shown that complex propagation in scattering media can be harnessed to manipulate broadband light wave…

Using a quantum electrodynamic framework, we calculate the off-resonant scattering of a broad-band X-ray pulse from a sample initially prepared in an arbitrary superposition of electronic states. The signal consists of single-particle…

Chemical Physics · Physics 2015-06-19 Kochise Bennett , Jason D. Biggs , Yu Zhang , Konstantin E. Dorfman , Shaul Mukamel

We present a fast active microrheology technique exploring the phase response of a microscopic probe particle trapped in a linear viscoelastic fluid using optical tweezers under an external perturbation. Thus, we experimentally determine…

Applied Physics · Physics 2020-01-08 Shuvojit Paul , Avijit Kundu , Ayan Banerjee

Terahertz (THz) metamaterials have been developed for THz sensing, detection, imaging, and many other functions due to their unusual absorbers. However, the unusual absorption spectra change with different incident angles. Thus, we designed…

Optics · Physics 2022-02-28 Zhigang Li Wenjing Jiang , Jianyu Fu , Qing Zhao

Two-dimensional terahertz spectroscopy (2DTS) is a low-frequency analogue of two-dimensional optical spectroscopy that is rapidly maturing as a probe of a wide variety of condensed matter systems. However, a persistent problem of 2DTS is…

We have observed cyclotron resonance in a high-mobility GaAs/AlGaAs two-dimensional electron gas by using the techniques of terahertz time-domain spectroscopy combined with magnetic fields. From this, we calculate the real and imaginary…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 X. Wang , D. J. Hilton , L. Ren , D. M. Mittleman , J. Kono , J. L. Reno

We describe a new approach based on semiclassical molecular dynamics that allows to simulate infrared absorption or emission spectra of molecular systems with inclusion of anharmonic intensities. This is achieved from semiclassical power…

Chemical Physics · Physics 2018-11-12 Marco Micciarelli , Riccardo Conte , Jaime Suarez , Michele Ceotto

Infrared (IR) spectroscopy is a pivotal technique in chemical research for elucidating molecular structures and dynamics through vibrational and rotational transitions. However, the intricate molecular fingerprints characterized by unique…

Machine Learning · Computer Science 2024-02-06 Chengchun Liu , Fanyang Mo

Two-dimensional (2D) fluorescence-excitation (2D-FLEX) spectroscopy is a recently proposed nonlinear femtosecond technique for the detection of photoinduced dynamics. The method records a time-resolved fluorescence signal in its excitation-…

Chemical Physics · Physics 2024-06-24 Sebastian V. Pios , Maxim F. Gelin , Luis Vasquez , Jürgen Hauer , Lipeng Chen

Owing to its high brilliance, infrared and terahertz synchrotron radiation (IR/THz-SR) has emerged as a powerful tool for spectroscopy under extreme (i.e., technically more difficult) experimental conditions such as high pressure, high…

Strongly Correlated Electrons · Physics 2015-06-11 Shin-ichi Kimura , Hidekazu Okamura