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We show clear experimental evidence of co-operative terahertz (THz) dynamics observed below 3 THz (~100 cm-1), for a low-symmetry Zr-based metal-organic framework (MOF) structure, termed MIL-140A [ZrO(O2C-C6H4-CO2)]. Utilizing a combination…

Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…

Chemical Physics · Physics 2013-09-27 Konstantin E. Dorfman , Benjamin P. Fingerhut , Shaul Mukamel

The study is devoted to development and optimization of a metasurface-based sensor with graphene constituents for potential biosensing applications. A unit cell of the proposed metasurface consists of a thin flexible dielectric substrate…

Optics · Physics 2026-01-12 K. S. Kuznetsova , V. A. Pashynska , Z. E. Eremenko

Strongly correlated solids are extremely complex and fascinating quantum systems, where new states continue to emerge, especially when interaction with light triggers interplay between them. In this interplay, sub-laser-cycle electron…

Strongly Correlated Electrons · Physics 2023-03-13 V. Valmispild , E. Gorelov , M. Eckstein , A. Lichtenstein , H. Aoki , M. Katsnelson , M. Ivanov , O. Smirnova

Dual terahertz (THz) comb spectroscopy is a promising methods for high accuracy, high resolution, and broadband THz spectroscopy because the mode-resolved THz comb spectrum possesses both characteristics of broadband THz radiation and…

Biophysical force spectroscopy tools - for example optical tweezers, magnetic tweezers, atomic force microscopy, - have been used to study elastic, mechanical, conformational and dynamic properties of single biological specimens from single…

Biomolecules · Quantitative Biology 2016-06-09 Zhaokun Zhou , Mark C. Leake

Forthcoming experiments will enable us to determine high precision tomographic shear spectra. Matter density fluctuation spectra, at various $z$, should then be worked out of them, in order to constrain the model and determine the DE state…

Cosmology and Nongalactic Astrophysics · Physics 2017-03-08 Marino Mezzetti , Silvio A. Bonometto , Luciano Casarini , Giuseppe Murante

Contrary to what might be expected, when an organic dye is sputtered onto an opaque holey metal film, transmission bands can be observed at the absorption energies of the molecules. This phenomenon, known as absorption-induced transparency,…

Mesoscale and Nanoscale Physics · Physics 2016-02-10 Sergio G. Rodrigo , L. Martín-Moreno

Light-matter interactions are of fundamental scientific and technological interest. Ultrafast electron microscopy and diffraction with combined femtosecond-nanometer resolution elucidate the laser-induced dynamics in structurally…

Materials Science · Physics 2025-04-08 Till Domröse , Leonardo da Camara Silva , Claus Ropers

Infrared (IR) spectroscopy is an indispensable tool for many practical applications including material analysis and sensing. Existing IR spectroscopy techniques face challenges related to the inferior performance and the high cost of…

Optics · Physics 2017-03-13 Anna Paterova , Shaun Lung , Dmitry Kalashnikov , Leonid Krivitsky

We present an all-optical concept for measuring the electric field of light spanning from infrared to extreme ultraviolet with multi-petahertz detection bandwidth. Our approach employs a heterodyne detection of light produced by a highly…

Experimental and theoretical evidence point out to the crucial role of specific resonant intramolecular vibrational modes in the interpretation of long-lived coherences observed in two-dimensional spectra of some natural and synthetic light…

Chemical Physics · Physics 2020-07-15 Leonardo F. Calderón , Leonardo A. Pachón

While established semiconductor measurement techniques such as four-point probe or capacitance-voltage measurements require a physical contact to the material, terahertz spectroscopy is completely contact-free. Its capability to measure the…

Ultrasensitive terahertz sensing of highly absorptive aqueous solutions remains challenging due to strong absorption of water in the terahertz regime. Here, we experimentally demonstrate a cost-effective metamaterial-based sensor integrated…

Optics · Physics 2022-04-05 Min Chen , Leena Singh , Ningning Xu , Ranjan Singh , Weili Zhang , Lijuan Xie

The last years have seen a revolution in ground-based gamma-ray detectors. We can now detect the spectra of nearby TeV blazars like Mrk 421 and 501 out to approximately 20 TeV, and during the strongest flares, we can now follow fluctuations…

Astrophysics · Physics 2009-10-31 Paolo S. Coppi , Felix A. Aharonian

Spectral densities encode non-perturbative information that enters the calculation of a plethora of physical observables in strongly coupled field theories. Phenomenological applications encompass aspects of standard-model hadronic physics,…

The first experimental data from single-particle scattering experiments from free electron lasers (FELs) are now becoming available. The first such experiments are being performed on relatively large objects such as viruses, which produce…

Biomolecules · Quantitative Biology 2015-05-28 Dilano Saldin , Hin-Cheuck Poon , Peter Schwander , Miraj Uddin , Marius Schmidt

Terahertz time domain spectroscopy employing free-space radiation has frequently been used to probe the elementary excitations of low-dimensional systems. The diffraction limit blocks its use for the in-plane study of individual laterally…

Normal thermal fluctuations of the cell membrane have been studied extensively using high resolution microscopy and focused light, particularly at the peripheral regions of a cell. We use a single probe particle attached non-specifically to…

Biological Physics · Physics 2020-04-16 Rahul Vaippully , Vaibavi Ramanujan , Manoj Gopalakrishnan , Saumendra Bajpai , Basudev Roy

Nonlinear spectroscopy provides a unique perspective to understand time-resolved molecular dynamics under vibrational strong coupling (VSC). Herein, equilibrium-nonequilibrium cavity molecular dynamics simulations are performed to compute…

Chemical Physics · Physics 2026-03-26 Xinwei Ji , Tomislav Begusic , Tao E. Li
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