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Absorption spectra of liquid water at 300 K are calculated from both classical and density functional theory molecular dynamics simulation data, which together span from 1 MHz to hundreds of THz, agreeing well with experimental data…

Chemical Physics · Physics 2020-09-09 Shane Carlson , Florian N. Brünig , Philip Loche , Douwe Jan Bonthuis , Roland R. Netz

This is the first in a series of two papers investigating the effect of electron-phonon coupling in two-dimensional Fourier transformed electronic spectroscopy. We present a series of one- and two-dimensional nonlinear spectroscopic…

Understanding interlayer and intralayer coupling in two-dimensional layered materials (2DLMs) has fundamental and technological importance for their large-scale production, engineering heterostructures, and development of flexible and…

The highly excited stretching vibrational energy levels and the intensities of infrared transitions in tetrahedral molecules are studied in a U(2) algebraic model. Its applications to silane and silicon tetrafluoride are presented with…

Chemical Physics · Physics 2007-05-23 Xi-Wen Hou , Zhong-Qi Ma

The nonlinear interaction between Near-Infrared (NIR) and Terahertz pulses is principally investigated as a means for the detection of radiation in the hardly accessible THz spectral region. Most studies have targeted second-order nonlinear…

Surface-enhanced infrared absorption (SEIRA) spectroscopy exploits the field enhancement near nanophotonic structures for highly sensitive characterization of (bio)molecules. The vibrational signature observed in SEIRA spectra is typically…

Terahertz spectral range (frequencies of 0.1-1 THz) has recently emerged as the next frontier for non-destructive imaging, industrial sensing and ultra-fast wireless communications. Here, we review several classes of materials such as…

Optics · Physics 2019-11-07 Mathieu Poulin , Steven Giannacopoulos , Maksim Skorobogatiy

We demonstrate results of a simulation of nonlinear reflection of intensive terahertz radiation from a silicon-on-metal metasurface involving an excitation of a high-Q trapped mode resonance. Conditions are presented to observe effects of…

Applied Physics · Physics 2019-03-15 N V Sydorchuk , S L Prosvirnin , Y Fan , F Zhang

In recent years, interesting materials have emerged which are only available as micron-scale flakes, and whose novel physics might be better understood through broadband microwave spectroscopy; examples include twisted bilayer graphene [1],…

Mesoscale and Nanoscale Physics · Physics 2022-06-08 Antonio Levy , Neil Zimmerman

Recently, two-dimensional terahertz spectroscopy (2DTS) has attracted increasing attention for studying complex solids. A number of recent studies have applied 2DTS either with long pulses or away from any material resonances, situations…

Optics · Physics 2024-09-06 Albert Liu , Ankit Disa

We present a metamaterial-based terahertz (THz) sensor for thickness measurements of subwavelength-thin materials and refractometry of liquids and liquid mixtures. The sensor operates in reflection geometry and exploits the frequency shift…

Contribution of plasma oscillation to the broadband terahertz emission is revealed by interacting two-color laser pulses with a supersonic jet of nitrogen molecules. Temporal and spectral shifts of THz waves are observed as the plasma…

Optics · Physics 2016-11-03 Na Li , Ya Bai , Tianshi Miao , Peng Liu , Ruxin Li , Zhizhan Xu

We report a comprehensive theoretical analysis of the instability achievable by using phase modulation spectroscopy to lock a terahertz local oscillator to an absorptive reference consisting of the rotational transition of molecules at room…

Atomic Physics · Physics 2025-02-20 W. F. McGrew , James Greenberg , Keisuke Nose , Brendan M. Heffernan , Antoine Rolland

Terahertz frequencies are an untapped resource for providing high-speed short-range communications. As a result, it is of interest to study the propagation characteristics of terahertz waves and to develop channel models. In previous work…

Signal Processing · Electrical Eng. & Systems 2022-10-17 Thanh Le , Ha Tran , Suresh Singh

We report real space imaging measurements of inelastic Friedel oscillations. The inelastic electron tunneling spectroscopy, using scanning tunneling microscopy, around dimers of dichlorobenze adsorbates on Au(111) surface display clear…

Mesoscale and Nanoscale Physics · Physics 2011-08-17 H. Gawronski , J. Fransson , K. Morgenstern

We demonstrate that halogenated methane 2D-Terahertz Terahertz Raman (2D-TTR) spectra are determined by the complicated structure of the instrument response function (IRF) along $f_1$ and by the molecular coherences along $f_2$.…

Chemical Physics · Physics 2020-07-20 Griffin Mead , Haw-Wei Lin , Ioan-Bogdan Magdău , Thomas F. Miller , Geoffrey A. Blake

Spectroscopies that probe electronic excitations from core levels into unoccupied orbitals, such as X-ray absorption spectroscopy and electron energy loss spectroscopy, are widely used to gain insight into the electronic and chemical…

Materials Science · Physics 2022-09-12 Marcus Annegarn , Juhan Matthias Kahk , Johannes Lischner

Resistivity is one of the most important characteristics in the semiconductor industry. The most common way to measure resistivity is the four-point probe method, which requires physical contact with the material under test. Terahertz time…

Spectroscopy is a powerful tool for studying molecules and is commonly performed on large thermal molecular ensembles that are perturbed by motional shifts and interactions with the environment and one another, resulting in convoluted…

We introduce THz Stark spectroscopy by using intense single-cycle terahertz pulses as the electric field source and monitoring the induced spectral response of an isotropic molecular ensemble with a coincident femtosecond supercontinuum…

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