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Here, the underlying mechanisms behind valley de-polarization is investigated in chemical vapor deposited 1L-MoS$_{2}$. Temperature dependent polarization resolved photoluminescence spectroscopy was carried out on as-grown, transferred and…

Two-dimensional semiconductors feature valleytronics phenomena due to locking of the spin and momentum valley of the electrons. However, the valley polarization is intrinsically limited in monolayer crystals by the fast intervalley…

Mesoscale and Nanoscale Physics · Physics 2019-07-10 Long Zhang , Rahul Gogna , G. William Burg , Jason Horng , Eunice Paik , Yu-Hsun Chou , Kyounghwan Kim , Emanuel Tutuc , Hui Deng

Degenerate extrema in the energy dispersion of charge carriers in solids, also referred to as valleys, can be regarded as a binary quantum degree of freedom, which can potentially be used to implement valleytronic concepts in van der Waals…

Two-dimensional (2D) van-der-Waals materials are a promising platform for exciton state engineering. In this paper, we study the properties of excitons in 2D group VI transition-metal dichalcogenide (TMD) semiconductors that are modified by…

Strongly Correlated Electrons · Physics 2026-05-08 Jose M. Torres-Lopez , Sudipta Kundu , Felipe H. da Jornada , Tony Heinz , Allan H. MacDonald

We study the effect of the exciton fine-structure splitting on the polarisation-entanglement of photon pairs produced by the biexciton cascade in a single quantum dot. The entanglement is found to persist despite separations between the…

We show that, because of the inevitable twist and lattice mismatch in heterobilayers of transition metal dichalcogenides, interlayer excitons have six-fold degenerate light cones anomalously located at finite velocities on the parabolic…

Mesoscale and Nanoscale Physics · Physics 2015-11-05 Hongyi Yu , Yong Wang , Qingjun Tong , Xiaodong Xu , Wang Yao

Manipulating quantum states through light-matter interactions has been actively pursued in two-dimensional (2D) materials research. Significant progress has been made towards the optical control of the valley degrees of freedom in…

Materials Science · Physics 2023-10-17 Jiawei Ruan , Zhenglu Li , Chin Shen Ong , Steven G. Louie

In the archetypal monolayer semiconductor WSe$_2$, the distinct ordering of spin-polarized valleys (low-energy pockets) in the conduction band allows for studies of not only simple neutral excitons and charged excitons (i.e., trions), but…

Materials Science · Physics 2022-08-15 Dinh Van Tuan , Su-Fei Shi , Xiaodong Xu , Scott A. Crooker , Hanan Dery

The variety of excitonic states in tungsten-based dichalcogenide monolayers stems from unique interplay between the spin and valley degrees of freedom. One of the exciton species is the indirect exciton (momentum or valley dark), which is…

Mesoscale and Nanoscale Physics · Physics 2022-08-23 Pengke Li , Cedric Robert , Dinh Van Tuan , Lei Ren , Xavier Marie , Hanan Dery

Excitons are key to the optoelectronic applications of van der Waals semiconductors with the potential for versatile on-demand tuning of properties. Yet, their electrical manipulation is complicated by their inherent charge neutrality and…

Mesoscale and Nanoscale Physics · Physics 2024-04-16 Sarthak Das , Ding Huang , Ivan Verzhbitskiy , Zi-En Ooi , Chit Siong Lau , Rainer Lee , Calvin Pei Yu Wong , Kuan Eng Johnson Goh

The valley degree of freedom in atomically thin transition-metal dichalcogenides provides a natural binary index for information processing. Exciton-polaritons formed under strong light-matter coupling offer a promising route to overcome…

Mesoscale and Nanoscale Physics · Physics 2026-01-23 Xingzhou Chen , Yuanjun Guan , Areg Ghazaryan , Shiran Sun , Lingxiao Yu , Ruitao Lv , Artem Volosniev , Zheng Sun , Jian Wu

We investigate the effect on disorder potential on exciton valley polarization and valley coherence in monolayer WSe2. By analyzing polarization properties of photoluminescence, the valley coherence (VC) and valley polarization (VP) is…

Monolayer transition metal dichalcogenides are a promising platform to investigate many-body interactions of excitonic complexes. In monolayer tungsten diselenide, the ground-state exciton is dark (spin-indirect), and the valley degeneracy…

Controlling excitons at the nanoscale in semiconductor materials represents a formidable challenge in the fields of quantum photonics and optoelectronics. Achieving this control holds great potential for unlocking strong exciton-exciton…

We report magneto-optical spectroscopy of gated monolayer MoS$_2$ in high magnetic fields up to 28T and obtain new insights on the many-body interaction of neutral and charged excitons with the resident charges of distinct spin and valley…

We have experimentally studied the pump-probe Kerr rotation dynamics in WSe$_2$ monolayers. This yields a direct measurement of the exciton valley depolarization time $\tau_v$. At T=4K, we find $\tau_v\approx 6$ps, a fast relaxation time…

Mesoscale and Nanoscale Physics · Physics 2014-10-10 C. R. Zhu , K. Zhang , M. Glazov , B. Urbaszek , T. Amand , Z. W. Ji , B. L. Liu , X. Marie

In this letter we study the valley degeneracy splitting of the transition-metal dichalcogenides monolayer by first-principles calculations. The local magnetic moments are introduced into the system when the transition-metal atoms are…

Materials Science · Physics 2016-09-06 Xiaofang Chen , Liangshuai Zhong , Xiao Li , Jingshan Qi

Excitons in monolayer transition metal dichalcogenide are endowed with intrinsic valley-orbit coupling between their center-of-mass motion and valley pseudospin. When trapped in a confinement potential, e.g., generated by strain field, we…

Mesoscale and Nanoscale Physics · Physics 2023-05-11 Di Zhang , Sha Deng , Dawei Zhai , Wang Yao , Qizhong Zhu

The Letter reports an experimental observation of the classical version of valley polarized states in a two-dimensional hexagonal sonic crystal, where the inversion-symmetry breaking of scatterers induces an omnidirectional frequency gap.…

Mesoscale and Nanoscale Physics · Physics 2017-05-31 Liping Ye , Chunyin Qiu , Jiuyang Lu , Xinhua Wen , Yuanyuan Shen , Manzhu Ke , Fan Zhang , Zhengyou Liu

Valleytronics is rapidly emerging as an exciting area of basic and applied research. In two dimensional systems, valley polarisation can dramatically modify physical properties through electron-electron interactions as demonstrated by such…

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