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Monolayer group-VIB transition metal dichalcogenides have recently emerged as a new class of semiconductors in the two-dimensional limit. The attractive properties include: the visible range direct band gap ideal for exploring…

Mesoscale and Nanoscale Physics · Physics 2015-07-30 Hongyi Yu , Xiaodong Cui , Xiaodong Xu , Wang Yao

Rydberg excitons, characterized by large spatial extension and reduced electron-hole overlap, must have a spin-valley dynamics different from that of ground state excitons. Here we report a direct measurement of spin relaxation of Rydberg…

Other Condensed Matter · Physics 2026-04-09 V. Jindal , K. Mourzidis , M. Semina , D. Lagarde , A. Balocchi , P. Renucci , T. Boulier , T. Taniguchi , K. Watanabe , M. Glazov , X. Marie

Optical interband transitions in monolayer transition metal dichalcogenides such as WSe2 and MoS2 are governed by chiral selection rules. This allows efficient optical initialization of an electron in a specific K-valley in momentum space.…

Mesoscale and Nanoscale Physics · Physics 2014-09-09 G. Wang , L. Bouet , D. Lagarde , M. Vidal , A. Balocchi , T. Amand , X. Marie , B. Urbaszek

We calculate the dispersion of spinor exciton-polaritons in a planar microcavity with its active region containing a single Transitional Metal Dichalcogenide (TMD) monolayer, taking into account excitonic and photonic spin-orbit coupling.…

Mesoscale and Nanoscale Physics · Physics 2017-10-25 O. Bleu , D. Solnyshkov , G. Malpuech

At the 2D limit, hexagonal systems such as monolayer transition metal dichalcogenides (TMDs) and graphene exhibit unique coupled spin and momentum-valley physics (valley pseudospin) owing to broken spatial inversion symmetry and strong…

Materials Science · Physics 2023-06-21 Tristan L Britt , Bradley J. Siwick

Valley pseudospin in two-dimensional (2D) transition-metal dichalcogenides (TMDs) allows optical control of spin-valley polarization and intervalley quantum coherence. Defect states in TMDs give rise to new exciton features and…

We study the neutral exciton energy spectrum fine structure and its spin dephasing in transition metal dichalcogenides such as MoS$_2$. The interaction of the mechanical exciton with its macroscopic longitudinal electric field is taken into…

Mesoscale and Nanoscale Physics · Physics 2014-05-15 M. M. Glazov , T. Amand , X. Marie , D. Lagarde , L. Bouet , B. Urbaszek

In monolayer Transition Metal Dichalcogenides (TMDs) the valence and conduction bands are spin split because of the strong spin-orbit interaction. In tungsten-based TMDs the spin-ordering of the conduction band is such that the so-called…

Preserving a high degree of valley polarization of excitons in photo-excited transition-metal dichalcogenide monolayers (TMD-MLs) is desirable for the valley-based photonic applications, but widely recognized as a hard task hindered by the…

Mesoscale and Nanoscale Physics · Physics 2020-10-13 Ping-Yuan Lo , Guan-Hao Peng , Wei-Hua Li , Yi Yang , Shun-Jen Cheng

We develop an analytical theory for edge states in monolayers of transition metal dichalcogenides based on a general boundary condition for a two-band ${\bf kp}$-Hamiltonian in case of uncoupled valleys. Taking into account {\it edge}…

Mesoscale and Nanoscale Physics · Physics 2017-12-22 V. V. Enaldiev

Spin-orbit coupling is a fundamental mechanism that connects the spin of a charge carrier with its momentum. Likewise, in the optical domain, a synthetic spin-orbit coupling is accessible, for instance, by engineering optical anisotropies…

Excitons in monolayer semiconductors have large optical transition dipole for strong coupling with light field. Interlayer excitons in heterobilayers, with layer separation of electron and hole components, feature large electric dipole that…

Mesoscale and Nanoscale Physics · Physics 2019-03-07 Wei-Ting Hsu , Bo-Han Lin , Li-Syuan Lu , Ming-Hao Lee , Ming-Wen Chu , Lain-Jong Li , Wang Yao , Wen-Hao Chang , Chih-Kang Shih

By enabling control of valley degrees of freedom in transition-metal dichalcogenides, valley-selective circular dichroism has become a key concept in valleytronics. In this manuscript, we show that valley excitons -- bound electron-hole…

Materials Science · Physics 2022-11-21 Fabio Caruso , Maximilian Schebek , Yiming Pan , Cecilia Vona , Claudia Draxl

We demonstrate room temperature chiral strong coupling of valley excitons in a transition metal dichalcogenide monolayer with spin-momentum locked surface plasmons. In this regime, we measure spin-selective excitation of directional flows…

Valleytronics targets the exploitation of the additional degrees of freedom in materials where the energy of the carriers may assume several equal minimum values (valleys) at non-equivalent points of the reciprocal space. In single layers…

Transition metal dichalcogenides represent an ideal testbed to study excitonic effects, spin-related phenomena and fundamental light-matter coupling in nanoscopic condensed matter systems. In particular, the valley degree of freedom, which…

Mesoscale and Nanoscale Physics · Physics 2017-05-16 N. Lundt , P. Nagler , A. Nalitov , S. Klembt , M. Wurdack , S. Stoll , T. H. Harder , S. Betzold , V. Baumann , A. V. Kavokin , C. Schüller , T. Korn , S. Höfling , C. Schneider

Monolayers of transition metal dichalcogenides are promising materials for valleytronic applications, since they possess two individually addressable excitonic transitions at the non-equivalent $K$ and $K'$ points with different spins,…

Mesoscale and Nanoscale Physics · Physics 2020-07-01 Malte Selig , Florian Katsch , Samuel Brem , Garnik F. Mkrtchian , Ermin Malic , Andreas Knorr

Electron-hole exchange interaction in two-dimensional transition metal dichalcogenides is extremely strong due to the dimension reduction, which promises valley-superposed excitonic states with linearly polarized optical emissions. However,…

Mesoscale and Nanoscale Physics · Physics 2024-12-11 Qiutong Wang , Ci Li , Qingjun Tong

Long-lived interlayer excitons with distinct spin-valley physics in van der Waals heterostructures based on transition metal dichalcogenides make them promising for information processing in next-generation devices. While the emission…

Mesoscale and Nanoscale Physics · Physics 2021-10-18 Alberto Ciarrocchi , Dmitrii Unuchek , Ahmet Avsar , Kenji Watanabe , Takashi Taniguchi , Andras Kis

Exciton-polaritons - coherently hybridized states of excitons and photons - are instrumental for solid-state nonlinear optics and quantum simulations. To enable engineered polariton energy landscapes and interactions, local control over the…