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We show that inversion symmetry breaking together with spin-orbit coupling leads to coupled spin and valley physics in monolayers of MoS2 and other group-VI dichalcogenides, making possible controls of spin and valley in these 2D materials.…

Mesoscale and Nanoscale Physics · Physics 2012-05-09 Di Xiao , Gui-Bin Liu , Wanxiang Feng , Xiaodong Xu , Wang Yao

We have investigated the steady-sate valley polarization and valley coherence of encapsulated MoS2 monolayer as a function of the temperature and the power density with a continuous wave laser excitation. Both valley polarization and…

Materials Science · Physics 2021-11-01 Fabian Cadiz , Stefan Gerl , Takashi Taniguchi , Kenji Watanabe

The polarization analysis of optical transitions in monolayer and bilayer transition-metal dichalcogenides provides invaluable information on the spin and valley (pseudospin) degrees of freedom. To explain optical properties of a given…

Materials Science · Physics 2015-10-06 Hanan Dery , Yang Song

Monolayers of semiconducting transition metal dichalcogenides are two-dimensional direct-gap systems which host tightly-bound excitons with an internal degree of freedom corresponding to the valley of the constituting carriers. Strong…

In monolayer transition metal dichalcogenides time-reversal symmetry, combined with space-inversion symmetry, defines the spin-valley degree of freedom. As such, engineering and control of time-reversal symmetry by optical or magnetic…

Heterostructures comprising different monolayer semiconductors provide a new system for fundamental science and device technologies, such as in the emerging field of valleytronics. Here, we realize valley-specific interlayer excitons in…

Mesoscale and Nanoscale Physics · Physics 2016-01-13 Pasqual Rivera , Kyle L. Seyler , Hongyi Yu , John R. Schaibley , Jiaqiang Yan , David G. Mandrus , Wang Yao , Xiaodong Xu

In atomically thin transition metal dichalcogenides (TMDs), reduced dielectric screening of the Coulomb interaction leads to strongly correlated many-body states, including excitons and trions, that dominate the optical properties.…

The coupled spin-valley physics in transition metal dichalcogenides (TMDs) endows exciton states with valley degrees of freedom, making them promising for valleytronic applications in TMDs monolayers and/or their heterostructures. Although…

Applied Physics · Physics 2022-12-07 Yingying Chen , Zeyi Liu , Junchao Hu , Junze Li , Wendian Yao , Dehui Li

We investigate the valley relaxation due to intervalley coupling in a single-electron bilayer graphene quantum dot. The valley relaxation is assisted by both the emission of acoustic phonons via the deformation potential and bond-length…

Mesoscale and Nanoscale Physics · Physics 2024-02-29 Lin Wang , Guido Burkard

The emerging field of valleytronics aims to exploit the valley pseudospin of electrons residing near Bloch band extrema as an information carrier. Recent experiments demonstrating optical generation and manipulation of exciton valley…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 Kai Hao , Lixiang Xu , Fengcheng Wu , Philipp Nagler , Kha Tran , Xin Ma , Christian Schüller , Tobias Korn , Allan H. MacDonald , Galan Moody , Xiaoqin Li

The newly developed two-dimensional layered materials provide perfect platform for valley-spintronics exploration. To determine the prospect of utilizing the valley degree of freedom, it is of great importance to directly detect and…

Mesoscale and Nanoscale Physics · Physics 2016-05-10 Tengfei Yan , Xiaofen Qiao , Pingheng Tan , Xinhui Zhang

Due to degeneracies arising from crystal symmetries, it is possible for electron states at band edges ("valleys") to have additional spin-like quantum numbers. An important question is whether coherent manipulation can be performed on such…

Local energy extrema of the bands in momentum space, or valleys, can endow electrons in solids with pseudo-spin in addition to real spin. In transition metal dichalcogenides this valley pseudo-spin, like real spin, is associated with a…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Grant Aivazian , Zhirui Gong , Aaron M Jones , Rui-Lin Chu , Jiaqiang Yan , David G Mandrus , Chuanwei Zhang , David Cobden , Wang Yao , Xiaodong Xu

Optical properties of semiconducting monolayer transition metal dichalcogenides have received a lot of attention in recent years, following the discovery of the valley selective optical population of either $K_{+}$ or $ K_{-}$ valleys at…

Other Condensed Matter · Physics 2022-05-17 Andrey Geondzhian , Angel Rubio , Massimo Altarelli

A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

Charge carriers in two-dimensional transition metal dichalcogenides (TMDs), such as WSe$_2$, have their spin and valley-pseudospin locked into an optically-addressable index that is proposed as a basis for future information processing. The…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Weijie Li , Xin Lu , Jiatian Wu , Ajit Srivastava

Electric dipole radiation can be controlled by coherent optical feedback, as has previously been studied by modulating the photonic environment for point dipoles placed both in optical cavities and near metal mirrors. In experiments…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 Christopher Rogers , Dodd Gray , Nathan Bogdanowicz , Takashi Taniguchi , Kenji Watanabe , Hideo Mabuchi

We propose a mechanism of intravalley spin-flip scattering in spin-valley coupled two dimensional systems by transferring momentum of light into exciton center of mass using optical vortex (OV) beams. By varying the dispersion of light…

Mesoscale and Nanoscale Physics · Physics 2022-10-11 A. K. Pattanayak , P. Das , D. Chakrabarty , A. Dhara , S. Paul , S. Maji , M. M. Brundavanam , S. Dhara

In doped transition metal dichalcogenides, optically created excitons (bound electron-hole pairs) can strongly interact with a Fermi sea of electrons to form Fermi polaron quasiparticles. When there are two distinct Fermi seas, as is the…

Resonances between excitonic transitions and nuclear coordinates have been shown to drive a variety of excited-state dynamical phenomena in molecular systems. Here, we report mixed quantum--classical simulations showing similar resonances…

Materials Science · Physics 2026-03-31 Alex Krotz , Roel Tempelaar