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We apply a fundamental definition of time delay, as the difference between the time a particle spends within a finite region of a potential and the time a free particle spends in the same region, to determine results for photoionization of…

Atomic Physics · Physics 2015-06-12 Jing Su , Hongcheng Ni , Andreas Becker , Agnieszka Jaroń-Becker

We present calculations for attosecond atomic delays in photoionization of noble gas atoms based on full two-color two-photon Random-Phase Approximation with Exchange in both length and velocity gauge. Gauge invariant atomic delays are…

Atomic Physics · Physics 2019-11-06 Jimmy Vinbladh , Jan Marcus Dahlström , Eva Lindroth

The process of reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) can become resonant with a discrete atomic level either in the intermediate or the final continuous states. Experimental observations of…

Atomic Physics · Physics 2021-09-01 Anatoli S. Kheifets

We use the non-relativistic random phase approximation with exchange to perform calculations of valence shell photoionization of Ne, Ar, Kr and Xe from their respective thresholds to photon energy of 200 eV. The energy derivative of the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets

An autoionizing resonance in molecular N$_2$ is excited by an ultrashort XUV pulse and probed by a subsequent weak IR pulse, which ionizes the contributing Rydberg states. Time- and angular-resolved photoelectron spectra recorded with a…

We explore how the spectral phase of atto\-second pulse trains influences the optical cross section in transient absorption (TA) spectroscopy. The interaction of extreme ultraviolet (XUV) and time-delayed near-infrared (NIR) fields with an…

Atomic Physics · Physics 2025-06-12 J. Jakob , C. Bauer , M. -J. Ilhan , D. Bharti , C. Ott , T. Pfeifer , K. Bartschat , A. Harth

We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…

Quantum Physics · Physics 2015-05-27 A. Picón , A. Bahabad , H. C. Kapteyn , M. M. Murnane , A. Becker

We study laser-assisted photoionization by attosecond pulses using a time-independent formalism based on diagrammatic many-body perturbation theory. Our aim is to provide an ab inito route to the "delays" for this above-threshold ionization…

Atomic Physics · Physics 2015-06-12 J. M. Dahlström , T. Carette , E. Lindroth

We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H$_2$ molecule. Time resolution of XUV ionization of H$_2$ is gained through the phase retrieval capability of attosecond angular…

Atomic Physics · Physics 2026-03-03 Vladislav V. Serov , Anatoli S. Kheifets

Attosecond measurements reveal new physical insights in photo ionization dynamics from atoms, molecules and condensed matter. However, on such time scales even small timing jitter can significantly reduce the time resolution in pump-probe…

Optics · Physics 2020-05-20 Constantin Krüger , Jaco Fuchs , Laura Cattaneo , Ursula Keller

It is shown that it is feasible to use ultrashort time delay between two XUV femtosecond pulses in order to control two photon resonant ionization. The proposal is demonstrated on the spectrum of Helium, in terms of nonperturbative…

Atomic Physics · Physics 2019-08-22 Theodoros Mercouris , Yannis Komninos , Cleanthes A. Nicolaides

We present a theoretical study of the photoelectron attosecond beating at the basis of RABBIT (Reconstruction of Attosecond Beating By Interference of Two-photon transitions) in the presence of autoionizing states. We show that, as a…

Atomic Physics · Physics 2015-01-14 Álvaro J. Galán , Luca Argenti , Fernando Martín

Shape resonances in physics and chemistry arise from the spatial confinement of a particle by a potential barrier. In molecular photoionization, these barriers prevent the electron from escaping instantaneously, so that nuclei may move and…

We use R-Matrix theory with Time dependence (RMT) to investigate multiphoton ionization of ground-state atomic carbon with initial orbital magnetic quantum number $M_L$=0 and $M_L$=1 at a laser wavelength of 390 nm and peak intensity of…

Atomic Physics · Physics 2014-10-08 H. F. Rey , H. W. van der Hart

We introduce circular under-threshold RABBITT (cuRABBITT) as a new interferometric method to probe discrete electronic excitations in atoms with attosecond resolution. By combining circularly polarized attosecond pulses with broadband…

Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…

A theoretical investigation of photoabsorption and photoionization of Fe^{14+} extending beyond an earlier frame transformation R-matrix implementation is performed using a fully-correlated, Breit-Pauli R-matrix formulation including both…

Atomic Physics · Physics 2015-06-04 M. F. Hasoglu , T. W. Gorczyca , M. A. Bautista , Z. Felfli , S. T. Manson

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We analyze interference processes in atomic ionization induced by a two-color laser with fundamental frequency $\omega $ and its second harmonic $2\omega $. The interplay between inter- and intracycle interference processes give rise to…

Atomic Physics · Physics 2021-09-13 Diego G. Arbó , Sebastián D. López

The precise control of light-matter interaction serves as a cornerstone for diverse quantum technologies, spanning from quantum computing to advanced atom optics. Typical experiments often feature multi-mode fields and require atoms with…

Quantum Physics · Physics 2025-07-08 Sabrina Hartmann , Nicolija Momčilović , Alexander Friedrich