Related papers: Analysis of RABITT time delays using the stationar…
Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a powerful photoelectron spectroscopy, offering direct access to internal dynamics of the target. It is being increasingly applied to molecular…
In this work we develop an approach for a molecular hydrogen ion (H2+) in the Born-Oppenheimer approximation while exposed to intense short-pulse radiation. Our starting point is the R-Matrix incorporating Time (RMT) formulation for atomic…
The reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) is one of the most widely used techniques for obtaining both the relative phases of harmonics forming an attosecond pulse train and the phase of…
One of the most ubiquitous techniques within attosecond science is the so-called Reconstruction of Attosecond Bursts by Interference of Two-Photon Transitions (RABBITT). Originally proposed for the characterization of attosecond pulses, it…
Extracting single photoionization time delays associated with atomic (or molecular) species from attosecond time scale two-photon experiments usually relies on the theoretical description of continuum-continuum transitions. The available…
We present an analytical model capable of describing two-photon ionization of atoms with attosecond pulses in the presence of intermediate and final isolated autoionizing states. The model is based on the finite-pulse formulation of…
We revisit the time-resolved photoemission in neon atoms as probed by attosecond streaking. We calculate streaking time shifts for the emission of 2p and 2s electrons and compare the relative delay as measured in a recent experiment by…
Characterizing time delays in molecular photoionization as a function of the ejected electron emission direction relative to the orientation of the molecule and the light polarization axis pro-vides unprecedented insights into the…
Recent angle-resolved RABBITT experiments have shown that the photoionization time delay depends on the emission angle of the photoelectron. In this work we demonstrate that for photoemission from helium accompanied by shake-up (correlation…
We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal…
We theoretically explore a variant of RABBITT spectroscopy in which the attosecond-pulse train comprises isolated pairs of consecutive harmonics of the fundamental infrared probe frequency. In this scheme, one-photon and two-photon…
We report an experiment of observation of classical double-slit interference fringes of two-photon interference. In the experiment, a commercial continuous-wave multi-mode F-P laser diode without either mode-locked or frequency-locked is…
Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…
The Wigner delay is defined as the energy derivative of the scattering phase of a particle in a given potential, unveiling the time taken (or gained) due to the interaction. The characterisation of this delay plays a central role in…
We investigate signatures of anisotropy on the dynamics of time-resolved near-threshold molecular photoemission, through simulations on a one-dimension asymmetric model molecule. More precisely, we study the relationship between the…
We present analytical expressions of momentum-resolved core-level photoemission time delay in a molecular frame of a heteronuclear diatomic molecule upon photoionization by a linearly polarized soft x-rays attosecond pulse. For this…
A unified scheme using the R-matrix method has been developed for electron-ion recombination subsuming heretofore separate treatments of radiative and dielectronic recombination (RR and DR). The ab initio coupled channel approach unifies…
We report a joint experimental and theoretical study of a three-sideband (3-SB) modification of the "reconstruction of attosecond beating by interference of two-photon transitions" (RABBIT) setup. The 3-SB RABBIT scheme makes it possible to…
We employ Reconstruction of Attosecond Beating By Interference of Two-photon Transitions with an advanced energy resolution (rainbow RABBITT) to resolve under-threshold discrete excitations and above-threshold auto-ionizing states in the He…
We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…