English

Circular RABBITT goes under threshold

Atomic Physics 2026-03-03 v3

Abstract

We introduce circular under-threshold RABBITT (cuRABBITT) as a new interferometric method to probe discrete electronic excitations in atoms with attosecond resolution. By combining circularly polarized attosecond pulses with broadband (``rainbow'') spectral analysis, we directly access two-photon ionization amplitudes and their relative phases. Time-dependent Schr\"odinger simulations, supported by Green's function theory, reveal strong resonances in helium and argon and a Cooper-like minimum in xenon. These results demonstrate that cuRABBITT provides continuous spectral mapping of bound-state resonances and extends Fano's propensity rule into the under-threshold regime. Our work establishes cuRABBITT as a powerful attosecond metrology technique, opening the way to polarization-resolved studies of resonant dynamics in atoms and molecules.

Keywords

Cite

@article{arxiv.2506.07445,
  title  = {Circular RABBITT goes under threshold},
  author = {Vladislav V. Serov and Jia-Bao Ji and Meng Han and Kiyoshi Ueda and Hans Jakob Woerner and Anatoli S. Kheifets},
  journal= {arXiv preprint arXiv:2506.07445},
  year   = {2026}
}

Comments

6 pages, 3 figures

R2 v1 2026-07-01T03:06:28.316Z