Related papers: Precisely Spun Super Rotors
The rotational excitation of the three asymmetric-top molecular ion isotopologues H$_2$O$^+$, HDO$^+$, and D$_2$O$^+$ is studied theoretically using a combined framework of electron-molecule R-matrix scattering theory, multichannel…
Ultrafast electron diffraction and time-resolved serial crystallography are the basis of the ongoing revolution in capturing at the atomic level of detail the structural dynamics of molecules. However, most experiments employ the classical…
Controlling the internal degrees of freedom is a key challenge for applications of cold and ultracold molecules. Here, we demonstrate rotational-state cooling of trapped methyl fluoride molecules (CH3F) by optically pumping the population…
High-dimensional entanglement is a valuable resource for quantum communication, and photon pairs entangled in orbital angular momentum are commonly used for encoding high-dimensional quantum states. However, methods for preparation of…
State-to-state differential cross sections (DCSs) for rotationally inelastic scattering of H2O by H2 have been measured at 71.2 meV (574 cm-1) and 44.8 meV (361 cm-1) collision energy using crossed molecular beams combined with velocity map…
We show how the rotational quantum state of a linear or symmetric top rotor can be reconstructed from finite time observations of the polar angular distribution under certain conditions. The presented tomographic method can reconstruct the…
Fast control of quantum systems is essential in order to make use of quantum properties before they are degraded by decoherence. This is important for quantum-enhanced information processing, as well as for pushing quantum systems into…
We propose an optical model in which both quantum and quasi-classical states can be ideally stored using coupled resonators. The protocol is based on a time-dependent coupling between two cavities, carefully modulated to allow the complete…
Quantum control of solid-state spin qubits typically involves pulses in the microwave domain, drawing from the well-developed toolbox of magnetic resonance spectroscopy. Driving a solid-state spin by optical means offers a high-speed…
A coherent state of many spins contains quantum entanglement which increases with a decrease in the collective spin value. We present a scheme to engineer this class of pure state based on incoherent spin pumping with a few collective…
We demonstrate coherent control of both the rotational and hyperfine state of ultracold, chemically stable $^{87}$Rb$^{133}$Cs molecules with external microwave fields. We create a sample of ~2000 molecules in the lowest hyperfine level of…
A new optical pumping scheme is presented that uses incoherent Raman transitions to prepare a trapped Cesium atom in a specific Zeeman state within the 6S_{1/2}, F=3 hyperfine manifold. An important advantage of this scheme over existing…
We explore the uses of ultracold molecules as a platform for future experiments in the field of quantum simulation, focusing on two molecular species, $^{40}$Ca$^{19}$F and $^{87}$Rb$^{133}$Cs. We report the development of coherent quantum…
We consider a diatomic molecule driven by a linearly polarized laser pulse with a polarization axis rotating with a constant acceleration. This setup is referred to as optical centrifuge, and it is known to lead to high-angular momenta for…
Solid-state spins are promising as interfaces from stationary qubits to single photons for quantum communication technologies. Semiconductor quantum dots have excellent optical coherence, exhibit near unity collection efficiencies when…
A molecule can be optically accelerated to rotate unidirectionally at a frequency of a few terahertzes which is many orders higher than the classical mechanical rotor. Such a photon-induced ultrafast molecular unidirectional rotation has…
Atoms trapped in a red detuned retro-reflected Laguerre-Gaussian beam undergo orbital motion within rings whose centers are on the axis of the laser beam. We determine the wave functions, energies and degeneracies of such quantum rotors…
We propose a quantum computer architecture which is robust against decoherence and scalable. As a qubit, we adopt rotational states of a nonpolar ionic molecule trapped in an ion-trap. It is revealed that the rotational-state qubits are…
The maximally entangled states are excellent candidates for achieving Heisenberg-limited measurements in ideal quantum metrology, however, they are fragile against dissipation such as particle losses and their achievable precisions may…
Raman scattering enables unforeseen uses for the laser guide-star system of the Very Large Telescope. Here, we present the observation of one up-link sodium laser beam acquired with the ESPRESSO spectrograph at a resolution…