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In recent years it became possible to align molecules in free space using ultrashort laser pulses. Here we explore two schemes for controlling molecule-surface scattering process, which are based on the laser-induced molecular alignment. In…

Chemical Physics · Physics 2015-05-28 Yuri Khodorkovsky , J. R. Manson , Ilya Sh. Averbukh

We describe a pulsed rotating supersonic beam source, evolved from an ancestral device [M. Gupta and D. Herschbach, J. Phys. Chem. A 105, 1626 (2001)]. The beam emerges from a nozzle near the tip of a hollow rotor which can be spun at…

The optical manipulation of electron spins is of great benefit to solid-state quantum information processing. In this letter, we provide a comparative study on the ultrafast optical manipulation of single electron spin in the doped and…

Other Condensed Matter · Physics 2009-11-11 Jinshuang Jin , Xin-Qi Li , YiJing Yan

The capacity of optical communication channels can be increased by space division multiplexing in structured optical fibers. Radial core optical fibers allows for the propagation of twisted light--eigenmodes of orbital angular momentum,…

Quantum Physics · Physics 2021-09-08 G. Cañas , E. S. Gómez , E. Baradit , G. Lima , S. P. Walborn

We present efficient theoretical tools for describing the optical pumping of atoms by light propagating at arbitrary directions with respect to an external magnetic field, at buffer-gas pressures that are small enough for velocity-selective…

Atomic Physics · Physics 2013-02-28 R. Marsland , B. H. McGuyer , B. A. Olsen , W. Happer

Advanced techniques for manipulation of internal states, standard in atomic physics, are demonstrated for a charged molecular species for the first time. We address individual hyperfine states of ro-vibrational levels of a diatomic ion by…

Atomic Physics · Physics 2015-05-08 U. Bressel , A. Borodin , J. Shen , M. Hansen , I. Ernsting , S. Schiller

We suggest a protocol for the sympathetic cooling of a molecular asymmetric top rotor co-trapped with laser-cooled atomic ions, based on resonant coupling between the molecular ion's electric dipole moment and a common normal mode of the…

Quantum Physics · Physics 2026-02-04 Monika Leibscher , Alexander Blech , Christiane P. Koch

Precision interferometry with quantum states has emerged as an essential tool for experimentally answering fundamental questions in physics. Optical quantum interferometers are of particular interest due to mature methods for generating and…

The ability to manipulate individual atoms and molecules using a scanning tunnelling microscope (STM) has been crucial for the development of a vast array of atomic scale devices and structures ranging from nanoscale motors and switches to…

Strongly Correlated Electrons · Physics 2021-02-03 Léonard Desvignes , Vasily S. Stolyarov , Marco Aprili , Freek Massee

Fast and efficient state preparation of molecules can be accomplished by optical pumping. Molecular structure that most obviously facilitates cycling involves a strong electronic transition, with favorable vibrational branching (diagonal…

Atomic Physics · Physics 2023-03-29 James B. Dragan , Ivan O. Antonov , Brian C. Odom

We present a new platform facilitating quantum logic control of polar molecular ions in a segmented ring ion trap, paving the way for precision measurements. This approach focuses on achieving near-unity state preparation and detection, as…

Atomic Physics · Physics 2023-07-27 Yan Zhou , Joshua O. Island , Matt Grau

We show that spin-orbit coupling in a quantum dot molecule allows for coherent manipulation of two electron spin states using Raman transitions. Such two-electron spin states defined by the singlet and triplet states of two exchange coupled…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Hakan E. Türeci , J. M. Taylor , A. Imamoglu

We show that optomechanical systems in the quantum regime can be used to demonstrate EPR-type quantum entanglement between the optical field and the mechanical oscillator, via quantum-state steering. Namely, the conditional quantum state of…

Quantum Physics · Physics 2012-11-20 Helge Mueller-Ebhardt , Haixing Miao , Stefan Danilishin , Yanbei Chen

This paper provides a framework for the control of quantum mechanical systems with scattering states, i.e., systems with continuous spectra. We present the concept and prove a criterion of the approximate strong smooth controllability. Our…

Quantum Physics · Physics 2007-05-23 Re-Bing Wu , Tzyh-Jong Tarn , Chun-Wen Li

In this paper, we study the dynamics of a system of $n$ coupled, self-propelled particles: $\ddot r_k = (\alpha-\beta |\dot r_k|^2)\dot r_k - \frac{\gamma}{n}\sum_{m=1}^n(r_k-r_m)$, $r_k\in \mathbb R^2.$ Numerical experiments indicate that,…

Dynamical Systems · Mathematics 2025-11-17 Carl Kolon , Constantine Medynets , Irina Popovici

We describe bichromatic superradiant pump-probe spectroscopy as a tomographic probe of the Wigner function of a dispersing particle beam. We employed this technique to characterize the quantum state of an ultracold atomic beam, derived from…

Quantum Physics · Physics 2009-11-13 Kevin L. Moore , Subhadeep Gupta , Kater W. Murch , Dan M. Stamper-Kurn

In recent experiments on ultracold matter, molecules have been produced from ultracold atoms by photoassociation, Feshbach resonances, and three-body recombination. The created molecules are translationally cold, but vibrationally highly…

Quantum Physics · Physics 2007-05-23 Christiane P. Koch , José P. Palao , Ronnie Kosloff , Françoise Masnou-Seeuws

As an alternative to commonly used electrical methods, we have investigated the optical pumping of charged exciton complexes addressing impurity related transitions with photons of the appropriate energy. Under these conditions, we…

Mesoscale and Nanoscale Physics · Physics 2010-07-15 G. Munoz-Matutano , B. Alen , J. Martinez-Pastor , L. Seravalli , P. Frigeri , S. Franchi

Optically addressable solid-state spins have been extensively studied for quantum technologies, offering unique advantages for quantum computing, communication, and sensing. Advancing these applications is generally limited by finding…

Rapid and repeated photon cycling has enabled precision metrology and the development of quantum information systems using a variety of atoms and simple molecules. Extending optical cycling to structurally complex molecules would provide…

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