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Quantum states of light, such as squeezed states or entangled states, can be used to make measurements (metrology), produce images, and sense objects with a precision that far exceeds what is possible classically, and also exceeds what was…

Quantum Physics · Physics 2009-04-02 Jonathan P. Dowling

Optical supercavity modes (superstates), i.e., hybrid modes emerging from the strong coupling of two nonorthogonal modes of an open cavity, can support ultranarrow lines in scattering spectra associated with quasi bound states in the…

Optics · Physics 2020-07-29 Nikita Nefedkin , Andrea Alú , Alex Krasnok

This work examines optimized strategies for the preparation of single molecular ions in well-defined rotational quantum states in an ion trap with the example of the molecular nitrogen ion N2+. It advances a two-step approach consisting of…

Atomic Physics · Physics 2023-09-07 Aleksandr Shlykov , Mikolaj Roguski , Stefan Willitsch

We present new results on the quantum control of systems with infinitely large Hilbert spaces. A control-theoretic analysis of the control of trapped ion quantum states via optical pulses is performed. We demonstrate how resonant…

Quantum Physics · Physics 2007-05-23 C. Rangan , A. M. Bloch , C. Monroe , P. H. Bucksbaum

The selfconsistent cranking approach is extended to the case of rotation about an axis which is tilted with respect to the principal axes of the deformed potential (Tilted Axis Cranking). Expressions for the energies and the intra bands…

Nuclear Theory · Physics 2009-11-06 S. Frauendorf

We study the ability to implement unitary maps on states of the $I=9/2$ nuclear spin in \textsuperscript{87}Sr, a $d=10$ dimensional (qudecimal) Hilbert space, using quantum optimal control. Through a combination of nuclear spin-resonance…

Quantum Physics · Physics 2022-11-30 Sivaprasad Omanakuttan , Anupam Mitra , Michael J. Martin , Ivan H Deutsch

Whether quantum physics is universally valid is an open question with far-reaching implications. Intense research is therefore invested into testing the quantum superposition principle with ever heavier and more complex objects. Here we…

Genetic algorithms, as implemented in optimal control strategies, are currently successfully exploited in a wide range of problems in molecular physics. In this context, laser control of molecular alignment and orientation remains a very…

Chemical Physics · Physics 2007-05-23 O. Atabek , C. M. Dion

Chemical reactions represent a class of quantum problems that challenge both the current theoretical understanding and computational capabilities. Reactions that occur at ultralow temperatures provide an ideal testing ground for quantum…

Chemical Physics · Physics 2021-05-25 Yu Liu , Ming-Guang Hu , Matthew A. Nichols , Dongzheng Yang , Daiqian Xie , Hua Guo , Kang-Kuen Ni

Superoscillation is a counterintuitive phenomenon for its mathematical feature of ``faster-than-Fourier", which has allowed novel optical imaging beyond the diffraction limit. In this article, we introduce a superoscillating quantum control…

Quantum Physics · Physics 2025-05-20 Yongcheng Ding , Yiming Pan , Xi Chen

Laser spectroscopy of cold and trapped molecular ions is a powerful tool for fundamental physics, including the determination of fundamental constants, the laboratory test for their possible variation, and the search for a possible electric…

Atomic Physics · Physics 2016-02-26 Fabian Wolf , Yong Wan , Jan C. Heip , Florian Gebert , Chunyan Shi , Piet O. Schmidt

Control over the quantum states of individual molecules is crucial in the quest to harness their rich internal structure and dipolar interactions for applications in quantum science. In this paper, we develop a toolbox of techniques for the…

Atomic Physics · Physics 2024-08-28 Daniel K. Ruttley , Alexander Guttridge , Tom R. Hepworth , Simon L. Cornish

We propose a scheme to generate spin cat states, i.e., superpositions of maximally separated quasiclassical states on a single high-dimensional nuclear spin in a solid-state device. We exploit a strong quadrupolar nonlinearity to drive the…

Quantum Physics · Physics 2024-01-30 Pragati Gupta , Arjen Vaartjes , Xi Yu , Andrea Morello , Barry C. Sanders

A general method for rotational microwave spectroscopy and control of polar molecular ions via direct microwave addressing is considered. Our method makes use of spatially varying AC Stark shifts, induced by far off-resonant, focused laser…

Atomic Physics · Physics 2015-06-16 M. Shi , P. F. Herskind , M. Drewsen , I. L. Chuang

A new generalised group-theoretical approach, based on master Maxwell-pseudospin equations, is proposed to explain recently observed enhanced circular dichroism in the excited state emission from p-doped quantum dot ensembles under resonant…

Mesoscale and Nanoscale Physics · Physics 2013-01-30 G. Slavcheva

When circularly polarized light is scattered from a rotating target, a rotational Doppler shift (RDS) emerges from an exchange of angular momentum between the spinning object and the electromagnetic field. Here, we used coherently spinning…

Quantum mechanics predicts that massive particles exhibit wave-like behavior. Matterwave interferometry has been able to validate such predictions through ground-breaking experiments involving microscopic systems like atoms and molecules.…

Quantum Physics · Physics 2025-10-08 R. Muffato , T. S. Georgescu , M. Carlesso , M. Paternostro , H. Ulbricht

The emerging field of ultracold molecules with their rich internal structure is currently attracting a lot of interest. Various methods have been developed to produce ultracold molecules in pre-set quantum states. For future experiments it…

We demonstrate that the current laser technology used for field-free molecular alignment via a cascade of Raman rotational transitions allows for observing long-discussed non-linear quantum phenomena in the dynamics of the periodically…

Quantum Physics · Physics 2015-05-30 Johannes Floß , Ilya Sh. Averbukh

First results are presented obtained with an experimental setup developed to record IR spectra of rotationally state-selected ions. The method we use is a state-selective version of a method developed by S. Schlemmer, D. Gerlich and…

Chemical Physics · Physics 2017-05-03 Ugo Jacovella , Josef A. Agner , Hansjürg Schmutz , Johannes Deiglmayr , Frédéric Merkt
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