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Precision spectroscopy of atomic and molecular ions offers a window to new physics, but is typically limited to species with a cycling transition for laser cooling and detection. Quantum logic spectroscopy has overcome this limitation for…

We demonstrate that efficient optical pumping of nuclear spins in semiconductor quantum dots (QDs) can be achieved by resonant pumping of optically "forbidden" transitions. This process corresponds to one-to-one conversion of a photon…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 E. A. Chekhovich , M. N. Makhonin , K. V. Kavokin , A. B. Krysa , M. S. Skolnick , A. I. Tartakovskii

Following excitation by a strong ultra-short laser pulse, molecules develop coordinated rotational motion, exhibiting transient alignment along the direction of the laser electric field, followed by periodic full and fractional revivals…

Quantum Physics · Physics 2007-05-23 Sharly Fleischer , Ilya. Sh. Averbukh , Yehiam Prior

It is often thought that the super-sensitivity of a quantum state to an observable comes at the cost of a decreased sensitivity to other non-commuting observables. For example, a squeezed state squeezed in position quadrature is…

We show that quantum rotational wavepacket dynamics in molecules can be described by a new system-environment model, which consists of a rotational subsystem coupled to a magnetically tunable spin bath formed by the nuclear spins within the…

Quantum Physics · Physics 2025-02-25 Timur V. Tscherbul , Lincoln D. Carr

The spin states of electrons and holes confined in InAs quantum dot molecules have recently come to fore as a promising system for the storage or manipulation of quantum information. We describe here a feasible scheme for complete quantum…

Mesoscale and Nanoscale Physics · Physics 2015-01-09 Guy Z. Cohen

Ultracold molecules trapped in optical tweezers show great promise for the implementation of quantum technologies and precision measurements. We study a prototypical scenario where two interacting polar molecules placed in separate traps…

The scattering of a flying photon by a two-level system ultrastrongly coupled to a one-dimensional photonic waveguide is studied numerically. The photonic medium is modeled as an array of coupled cavities and the whole system is analyzed…

Ultracold polar molecules uniquely combine a rich structure of long-lived internal states with access to controllable long-range, anisotropic dipole-dipole interactions. In particular, the rotational states of polar molecules confined in…

Precise measurement of the particle number, spatial distribution and internal state is fundamental to all proposed experiments with ultracold molecules both in bulk gases and optical lattices. Here, we demonstrate in-situ detection of…

Quantum coherence in quantum optics is an essential part of optical information processing and light manipulation. Alkali metal vapors, despite the numerous shortcomings, are traditionally used in quantum optics as a working medium due to…

Laser beams carrying orbital angular momentum (OAM) provide an additional degree of freedom and have found wide applications ranging from optical communications and optical manipulation to quantum information. The efficient generation and…

Whereas collisions between atoms and molecules are largely understood, collisions between two molecules have proven much harder to study. In both experiment and theory, our ability to determine quantum state-resolved bimolecular cross…

A phenomenological optical potential is generalized to include the Coulomb and nuclear interactions caused by the dynamical deformation of its surface. In the high-energy approach analytical expressions for elastic and inelastic scattering…

Nuclear Theory · Physics 2009-11-11 V. K. Lukyanov , Z. Metawei , E. V. Zemlyanaya

We report generation of cascaded rotational Raman scattering up to 58th orders in coherently excited CO_2 molecules. The high-order Raman scattering, which produces a quasiperiodic frequency comb with more than 600 sidebands, is obtained…

Spin echo techniques are essential for achieving long coherence times in solid-state quantum memories for light because of inhomogeneous broadening of the spin transitions. It has been suggested that unrealistic levels of precision for the…

Quantum Physics · Physics 2015-05-20 Khabat Heshami , Nicolas Sangouard , Jiri Minar , Hugues de Riedmatten , Christoph Simon

Erbium doped solids are potential candidates for the realization of a quantum memory for photons at telecommunication wavelengths. The implementation of quantum memory proposals in rare earth ion doped solids require spectral tailoring of…

Quantum Physics · Physics 2010-02-15 B. Lauritzen , S. R. Hastings-Simon , H. de Riedmatten , M. Afzelius , N. Gisin

Because of their central importance in chemistry and biology, water molecules have been the subject of decades of intense spectroscopic investigations. Rotational spectroscopy of water vapor has yielded detailed information about the…

Chemical Physics · Physics 2020-10-07 Yaqing Zhang , Jiaojian Shi , Xian Li , Stephen L. Coy , Robert W. Field , Keith A. Nelson

We experimentally demonstrate coherent control of a quantum system, whose dynamics is chaotic in the classical limit. Interaction of diatomic molecules with a periodic sequence of ultrashort laser pulses leads to the dynamical localization…

Quantum Physics · Physics 2017-01-25 Martin Bitter , Valery Milner

Optical levitation of nano-scale systems offers a pathway to highly sensitive rotation measurements, which are critical for advancing gyroscopic technologies. While prior studies have primarily focused on controlling rotational degrees of…