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A generalized class of ultra-long-range Rydberg molecules is proposed which consist of a multichannel Rydberg atom whose outermost electron creates a chemical bond with a distant ground state atom. Such multichannel Rydberg molecules…
A ground state atom immersed in the wave function of the valence electron of a Rydberg atom can generate a long-range Rydberg molecule (LRRM). In this work, using the multipole expansion of the electrostatic interaction in prolate…
We study the impact of Rydberg molecule formation on the storage and retrieval of Rydberg polaritons in an ultracold atomic medium. We observe coherent revivals appearing in the retrieval efficiency of stored photons that originate from…
We undertake a semiclassical analysis of the spectral properties (modulations of photoabsorption spectra, energy level statistics) of a simple Rydberg molecule in static fields within the framework of Closed-Orbit/Periodic-Orbit theories.…
We present an overview of our recent investigations of long-range interactions in an ultracold Cs Rydberg gas. These interactions are studied by high-resolution photoassociation spectroscopy, using excitation close to one-photon transitions…
To take full advantage of experimental facilities such as FRIB for applications to nuclear astrophysics, nuclear structure, and explorations of neutrinos and fundamental symmetries, we need a better understanding of the interplay of…
Nuclear interactions evolved via renormalization group methods to lower resolution become increasingly non-local (off-diagonal in coordinate space) as they are softened. This inhibits both the development of intuition about the interactions…
We focus on a recently developed generalized pseudospectral method for accurate, efficient treatment of certain central potentials of interest in various branches in quantum mechanics, usually having singularity. Essentially this allows…
Non-radiative energy transfer between a Rydberg atom and a polar molecule can be controlled by a DC electric field. Here we show how to exploit this control for state-resolved, non-destructive detection and spectroscopy of the molecules…
We present a novel spectroscopic method for probing the \insitu~density of quantum gases. We exploit the density-dependent energy shift of highly excited {Rydberg} states, which is of the order $10$\MHz\,/\,1E14\,cm$^{\text{-3}}$ for…
This Ph.D. tutorial discusses ultra-long-range Rydberg molecules, the exotic bound states of a Rydberg atom and one or more ground state atoms immersed in the Rydberg electron's wave function. This novel chemical bond is distinct from an…
We propose an implementation of a universal quantum gate between pairs of spatially separated atoms in a microwave cavity at finite temperature. The gate results from reversible laser excitation of Rydberg states of atoms interacting with…
We probe resonant dipolar interactions between ultracold $^{40}$K$^{87}$Rb molecules and Rydberg $^{87}$Rb atoms in an optically trapped ensemble. Through state-selective ionization detection of the KRb molecules, we observe resonant energy…
We present a method for probing the quantum capacitance associated with the Rydberg transition of surface electrons on liquid helium using radio-frequency (RF) reflectometry. Resonant microwave excitation of the Rydberg transition induces a…
Quantum reflection refers to a non-vanishing reflection probability in the absence of a classically turning point. Much attention has been paid to such reflections due to their fundamental, intriguing physics and potential practical…
Stopping and regenerating a pair of single-photon pulses at adjacent locations in coherently prepared Rydberg atomic ensembles are significantly affected by their effective interaction mediated by Rydberg excitations, and the similar…
We present combined measurements of the spatially-resolved optical spectrum and the total excited-atom number in an ultracold gas of three-level atoms under electromagnetically induced transparency conditions involving high-lying Rydberg…
Laser cooling and trapping of atomic matter waves in optical potentials has enabled rapid progress in quantum science, particularly when combined with Rydberg excitation of the atoms to induce long-range interactions. Here, we propose the…
In this work, Rydberg energy levels of the triatomic hydrogen molecule ($\rm{H_3}$) are studied with multichannel quantum-defect theory. We extract the body-frame p-wave quantum defects from highly accurate \emph{ab initio} electronic…
Radio frequency antennas based on highly excited Rydberg atom vapors can in principle reach sensitivities beyond those of any conventional wire antenna, especially at lower frequencies where very long wires are needed to accommodate the…