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A highly sensitive, general, and preferably nondestructive technique to detect polar molecules would greatly advance a number of fields, in particular quantum science with cold and ultracold molecules. Here, we propose using resonant energy…

Atomic Physics · Physics 2017-06-23 Martin Zeppenfeld

We investigate computationally a method for ultrafast preparation of alkali metal atoms in their Rydberg states using a three-dimensional model potential in the single active electron approximation. By optimizing laser pulse shapes that can…

Atomic Physics · Physics 2018-11-21 Janne Solanpää ja Esa Räsänen

Quantum sensing using Rydberg atoms offers unprecedented opportunities for next-generation radar systems, transcending classical limitations in miniaturization and spectral agility. Implementing this paradigm for radar sensing, this work…

Atomic Physics · Physics 2025-06-23 Minze Chen , Tianqi Mao , Zhiao Zhu , Haonan Feng , Ge Gao , Zhonghuai Wu , Wei Xiao , Zhongxiang Li , Dezhi Zheng

In recent years, micromachined vapor cells have been revolutionizing the field of chip-scale quantum sensors such as magnetometers and atomic clocks. In parallel, Rydberg atomic quantum sensing has emerged as a powerful technique for…

Atomic Physics · Physics 2025-07-01 Avital Giat , Kfir Levi , Ori Nefesh , Liron Stern

Quantum sensing has attracted significant attention due to its ability to measure physical quantities with extremely high accuracy. Rydberg atoms - typically alkali atoms with a highly excited valence electron that is far from the nucleus -…

Information Theory · Computer Science 2025-10-03 Javane Rostampoor , Raviraj Adve

We demonstrate the breakdown of molecular-frame dynamics induced by the uncoupling of molecular rotation from electronic motion in molecular Rydberg states. We observe this non-Born-Oppenheimer regime in the time domain through…

Atomic and Molecular Clusters · Physics 2017-07-05 Lucas J. Zipp , Adi Natan , Philip H. Bucksbaum

General relativity uses curved space-time to describe accelerating frames. The movement of particles in different curved space-times can be regarded as equivalent physical processes based on the covariant transformation between different…

Optics · Physics 2018-10-24 Fan Zhong , Jensen Li , Hui Liu , Shining Zhu

The Density Matrix Renormalization Group (DMRG) has become a powerful numerical method that can be applied to low-dimensional strongly correlated fermionic and bosonic systems. It allows for a very precise calculation of static, dynamic and…

Condensed Matter · Physics 2007-05-23 Karen Hallberg

Probing the real time dynamics of a reacting molecule remains one of the central challenges in chemistry. In this letter we show how the time-dependent wavefunction of an excited-state reacting molecule can be completely reconstructed from…

Quantum Physics · Physics 2015-05-27 David Avisar , David J. Tannor

Atomic-vapor sensors based on Rydberg atoms now face a transition towards practical applications, with several outstanding challenges. To achieve the best sensitivities, a superheterodyne mode of operation is desired, which requires the…

We propose new approach for treatment of local and non-local interactions in correlated electronic systems, which uses self-energy and the two-particle irreducible vertices, obtained from (extended) dynamical mean-field theory, as an input…

Strongly Correlated Electrons · Physics 2019-03-12 A. A. Katanin

We describe a quantum information architecture consisting of a hybrid array of optically-trapped molecules and atoms. This design leverages the large transition dipole moments of Rydberg atoms to mediate fast, high-fidelity gates between…

Atomic Physics · Physics 2023-01-13 Kenneth Wang , Conner P. Williams , Lewis R. B. Picard , Norman Y. Yao , Kang-Kuen Ni

Rydberg atom-based electric field sensing can provide all-optical readout of radio frequency fields in a dielectric environment. However, because a single set of optical fields is typically used to prepare the Rydberg state and read out its…

Recently, we introduced (e-print arXiv:1407.7128) {\em local reduced density matrix functional theory} (local RDMFT), a theoretical scheme capable of incorporating static correlation effects in Kohn-Sham equations. Here, we apply local…

Chemical Physics · Physics 2014-11-07 Nektarios N. Lathiotakis , Nicole Helbig , Angel Rubio , Nikitas I. Gidopoulos

We use the sensitive response to electric fields of Rydberg atoms to characterize all three vector components of the local electric field close to an atom-chip surface. We measured Stark-Zeeman maps of $S$ and $D$ Rydberg states using an…

We develop and study quantum and semi-classical models of Rydberg-atom spectroscopy in amplitude-modulated optical lattices. Both initial- and target-state Rydberg atoms are trapped in the lattice. Unlike in any other spectroscopic scheme,…

Quantum Physics · Physics 2020-04-01 V. S. Malinovsky , K. R. Moore , G. Raithel

Real Space Renormalization Group (RSRG) techniques and their applications, mainly to quantum mechanics and to partial differential equations, are discussed. Special emphasis is given to the theoretical insight and the reasons for the…

Statistical Mechanics · Physics 2007-05-23 Javier Rodriguez-Laguna

Precise physical descriptions of molecules can be obtained by solving the Schrodinger equation; however, these calculations are intractable and even approximations can be cumbersome. Force fields, which estimate interatomic potentials based…

Chemical Physics · Physics 2020-12-15 Peter Nekrasov , Jessica Freeze , Victor Batista

We demonstrate an all-optical, minimally invasive method for electron beam (e-beam) characterization using Rydberg electrometry. The e-beam passes through a dilute Rb vapor prepared in a quantum superposition of ground and Rydberg states…

We propose to use a permutation symmetric sample of multi-level atoms to simulate the properties of topologically ordered states. The Rydberg blockade interaction is used to prepare states of the sample which are equivalent to resonating…

Quantum Physics · Physics 2010-11-25 Anne E. B. Nielsen , Klaus Mølmer
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