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The decay of the optical phonon into the two phonons of smaller energy is calculated for Si nanocrystals. The rate of the process is in the range of 1 to 10 ps. Such anharmonic phonon decay may control the energy relaxation rate of excited…

Materials Science · Physics 2013-04-08 A. A. Prokofiev , A. N. Poddubny , I. N. Yassievich

Organic solar cells are a promising avenue for renewable energy, and our study introduces a comprehensive model to investigate exciton dissociation processes at the donor-acceptor interface. Examining quantum efficiency and emitted phonons…

Materials Science · Physics 2025-02-05 Jouda Jemaa Khabthani , Khouloud Chika , Alexandre Perrin , Didier Mayou

Excitons play major roles in optical processes in modern semiconductors, such as single-wall carbon nanotubes (SWCNTs), transition metal dichalcogenides, and 2D perovskite quantum wells. They possess extremely large binding energies…

An overview on photon echo spectroscopy under resonant excitation of the exciton complexes in semiconductor nanostructures is presented. The use of four-wave-mixing technique with the pulsed excitation and heterodyne detection allowed us to…

Mesoscale and Nanoscale Physics · Physics 2018-08-29 S. V. Poltavtsev , I. A. Yugova , I. A. Akimov D. R. Yakovlev , M. Bayer

We perform time-dependent, 2DHD numerical simulations to study the dynamics of a slowly rotating accretion flow from sub-pc to pc scales under the irradiation from the central AGN. Compared to previous work, we improve the calculation of…

High Energy Astrophysical Phenomena · Physics 2015-06-15 Chao Liu , Feng Yuan , Jeremiah P. Ostriker , Zhaoming Gan , Xiaohong Yang

We demonstrate a new method of measuring the exciton spin relaxation time in semiconductor nanostructures by continuous-wave photoluminescence. We find that for self-assembled CdTe quantum dots the degree of circular polarization of…

Materials Science · Physics 2009-11-10 S. Mackowski , T. A. Nguyen , H. E. Jackson , L. M. Smith , J. Kossut , G. Karczewski

Understanding and ultimately controlling the transformations and properties of nanoscale systems, from proteins to synthetic nanomaterial assemblies, is limited by the inability to uncover their dynamics on their characteristic length and…

Tho-photon absorption holds potential for many practical applications. We theoretically investigate the onset of this phenomenon in a semiconductor quantum dot -- metallic nanoshell composite subjected to a resonant CW excitation.…

Mesoscale and Nanoscale Physics · Physics 2021-01-08 Bintoro S. Nugroho , Alexander A. Iskandar , Victor A. Malyshev , Jasper Knoester

The goal of nanophotonics is to control and manipulate light at length scales below the diffraction limit. Typically nanostructured metals are used for this purpose, light being confined by exploiting the surface plasmon-polaritons such…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 Martin J. Gentile , William L. Barnes

We report on the possibility of describing the absorption and emission characteristics of an ensemble of silicon nanocrystals (NCs) with realistic distributions in the NC size, by the sum of the reponses of the single NCs. The individual NC…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Roberto Guerra , Francesco Cigarini , Stefano Ossicini

We investigate the relaxation dynamics of photogenerated carriers in silicon nanowires consisting of a crystalline core and a surrounding amorphous shell, using femtosecond time-resolved differential reflectivity and transmission…

Mesoscale and Nanoscale Physics · Physics 2012-12-24 Sunil Kumar , M. Khorasaninejad , M. M. Adachi , K. S. Karim , S. S. Saini , A. K. Sood

Excitons -- quasiparticles formed by the binding of an electron and a hole through electrostatic attraction -- hold promise in the fields of quantum light confinement and optoelectronic sensing. Atomically thin transition metal…

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

Materials Science · Physics 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

We analyze the many-particle correlations that affect the optical properties of two-dimensional semiconductors. These correlations manifest themselves through the specific optical resonances such as excitons, trions, etc. Starting from the…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 A. Kudlis , I. Iorsh

The nonlinear photoacoustic response of indium phosphide nanocrystals on silicon nanotip arrays is investigated using time-resolved optical pump-probe spectroscopy and synchrotron-based X-ray diffraction. Femtosecond laser excitation…

The optical absorption of a single spherical semiconductor quantum dot in an electrical field is studied taking into account the nonlocal coupling between the field of the light and the polarizability of the semiconductor. These nonlocal…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 F. Thiele , Ch. Fuchs , R. v. Baltz

In this work, we theoretically investigate the optical orientation and alignment of excitons in quantum dots with weak electron-hole exchange interaction and long exciton radiative lifetimes. This particular regime is realized in…

Mesoscale and Nanoscale Physics · Physics 2023-08-30 D. S. Smirnov , E. L. Ivchenko

Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic…

Optics · Physics 2022-03-11 J. S. Duan

We present a theory of the acoustic phonon assisted spin-flip Raman scattering (SFRS), or resonant photoluminescence with the spin flip of a photoexcited exciton localized in a bulk cubic-phase perovskite semiconductor. We consider the…

Materials Science · Physics 2024-02-05 A. V. Rodina , E. L. Ivchenko

Charge transfer between photoexcited quantum dots and molecular acceptors is one of the key limiting processes in most applications of colloidal nanostructures, most prominently in photovoltaics. An atomistic detailed description of this…

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