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This is a review of exciton dynamics in conjugated polymers. Exciton dynamics encompass multiple time and length scales. Ultrafast femtosecond processes are intrachain and involve a quantum mechanical correlation of the exciton and nuclear…

Chemical Physics · Physics 2021-02-15 William Barford

Semiconductor nanocrystals could replace conventional bulk materials completely in displays and light-emitting diodes. Exciton transport dominates over charge carrier transport for materials with high exciton binding energies and long…

We consider exciton polaritons in a semiconductor microcavity with a saturable absorber in the growth direction of the heterostructure. This feature promotes additional nonlinear losses of the system with the emergence of bistability of the…

Mesoscale and Nanoscale Physics · Physics 2015-08-12 D. V. Karpov , I. G. Savenko , H. Flayac , N. N. Rosanov

We investigate the steady-state cooling dynamics of vibrational degrees of freedom related to a nanomechanical oscillator coupled with a laser-pumped quantum dot in an optical resonator. Correlations between phonon-cooling and quantum-dot…

Quantum Physics · Physics 2015-06-19 Sergiu Carlig , Mihai A. Macovei

A review is given on the recent spectroscopic studies of the electronic excitation induced processes of large-scale atomic displacements in atomic cryocrystals, including defect formation, atomic and molecular desorption.

Condensed Matter · Physics 2007-05-23 A. N. Ogurtsov

The optical properties of atomically thin semiconductors are dominated by excitons, tightly bound electron-hole pairs, which give rise to particularly rich and remarkable physics. Despite their importance, the microscopic formation…

Monolayer semiconductors hold great potential for nanoscale electronics, optoelectronics, and photonics. Excitons dominate their optical properties. As their electric fields extend outside the monolayer, they are sensitive to their…

We demonstrate for the first time that impact ionization (II) [the inverse of Auger recombination (AR)] occurs with very high efficiency in semiconductor nanocrystals (NCs). Interband optical excitation of PbSe NCs at low pump intensities,…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. D. Schaller , V. I. Klimov

Non-Markovian and non-equilibrium phonon effects are believed to be key ingredients in the energy transfer in photosynthetic complexes, especially in complexes which exhibit a regime of intermediate exciton-phonon coupling. In this work, we…

Quantum Physics · Physics 2011-07-08 Patrick Rebentrost , Alán Aspuru-Guzik

One-dimensional models with topological non-trivial band structures are a simple and effective way to study novel and exciting concepts in topological photonics. In this work we are studying the propagation of light-matter quasi-particles,…

We investigate the dynamics of single- and multi-photon emission from detuned strongly coupled systems based on the quantum-dot-photonic-crystal resonator platform. Transmitting light through such systems can generate a range of…

Semiconductor microcavities are widely used to study collective interactions of cavity exciton-polaritons leading to their condensation phenomenon. Exciton-light interaction is highly enhanced in such structures due to the resonance…

Mesoscale and Nanoscale Physics · Physics 2014-07-17 Mikhail Lebedev , Andrey Parakhonsky , Andrey Demenev

The realization of exciton-polaritons -- hybrid excitations of semiconductor quantum well excitons and cavity photons -- has been of great technological and scientific significance. In particular, the short-range collisional interaction…

Quantum Gases · Physics 2018-07-17 Valentin Walther , Robert Johne , Thomas Pohl

Modification of electromagnetic quantum fluctuations in the form of quadrature-squeezing is a central quantum resource, which can be generated from nonlinear optical processes. Such a process is facilitated by coherent two-photon excitation…

Quantum Physics · Physics 2022-11-14 Emil V. Denning , Andreas Knorr , Florian Katsch , Marten Richter

Organic semiconductors exhibit properties of individual molecules and extended crystals simultaneously. The strongly bound excitons they host are typically described in the molecular limit, but excitons can delocalize over many molecules,…

Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that…

Mesoscale and Nanoscale Physics · Physics 2022-03-02 Valentin Walther , Lida Zhang , Susanne F. Yelin , Thomas Pohl

We extend the original idea of reduced nuclear amplitudes to capture individual helicity amplitudes and discuss various applications to exclusive processes involving the deuteron. Specifically, we consider deuteron form factors, structure…

Nuclear Theory · Physics 2023-05-03 J. Flores , S. S. Chabysheva , J. R. Hiller

We study theoretically the optical response of a nanohybrid comprising a symmetric quantum dimer emitter coupled to a metal nanoparticle (MNP). The interactions between the exitonic transitions in the dimer and the plasmons in the MNP lead…

Mesoscale and Nanoscale Physics · Physics 2015-11-11 Bintoro S. Nugroho , Victor A. Malyshev , Jasper Knoester

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

Materials Science · Physics 2022-02-17 Gabriel Antonius , Steven G. Louie

The interplay of migration, recombination, and dissociation of excitons in disordered media is studied theoretically in the low temperature regime. An exact expression for the photoluminescence spectrum is obtained. The theory is applied to…

Condensed Matter · Physics 2009-10-28 M. C. J. M. Vissenberg , M. J. M. de Jong