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We have developed a model in order to account for electron-vibrational effects on absorption, luminescence of molecular aggregates and exciton-polaritons in nanofibers. The model generalizes the mean-field electron-vibrational theory…

Mesoscale and Nanoscale Physics · Physics 2019-03-22 Boris D. Fainberg

Silicon nanocrystals are produced using a two-stage gold ion implantation technique. First stage implantation using low energy ions leads to the formation of an amorphous Si (a-Si) layer. A subsequent high energy Au irradiation in the…

Mesoscale and Nanoscale Physics · Physics 2014-03-26 Gayatri Sahu , Rajesh Kumar , D. P. Mahapatra

Exciton-photon hybridization is typically realised in geometrically defined optical cavities, where tunability is achieved by modifying either the cavity or the excitonic medium. Here we investigate transition-radiation interferences in…

Semiconductor microcavity polaritons, formed via strong exciton-photon coupling, provide a quantum many-body system on a chip, featuring rich physics phenomena for better photonic technology. However, conventional polariton cavities are…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 Long Zhang , Rahul Gogna , Will Burg , Emanuel Tutuc , Hui Deng

We demonstrate theoretically that the single-photon purity of photons emitted from a quantum dot exciton prepared by phonon-assisted off-resonant excitation can be significantly higher in a wide range of parameters than that obtained by…

Mesoscale and Nanoscale Physics · Physics 2019-07-08 Michael Cosacchi , Florian Ungar , Moritz Cygorek , Alexei Vagov , Vollrath Martin Axt

Rapid progress in silicon photonics has fostered numerous chip-scale sensing, computing, and signal processing technologies. However, many crucial filtering and signal delay operations are difficult to perform with all-optical devices.…

Time resolved photoluminescence is a powerful technique to study the collective dynamics of excitons and polaritons in semiconductor nanostructures. We present a two excitation pulses technique to induce the ultrafast and controlled…

Mesoscale and Nanoscale Physics · Physics 2010-02-25 A. Amo , D. Sanvitto , L. Vina

We develop a generalized framework based on a Green's function formalism to calculate the efficiency of multiexciton gen-eration in nanocrystal quantum dots. The direct/indirect absorption and coherent/incoherent impact ionization…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Eran Rabani , Roi Baer

The coupling of excitons with atomic vibrations plays a pivotal role on the nonequilibrium optical properties of layered semiconductors. However, addressing the dynamical interaction between excitons and phonons represents a hard task both…

The low-frequency vibrational spectrum of an isolated nanometer-scale solid differs dramatically from that of a bulk crystal, causing the decay of a localized electronic state by phonon emission to be inhibited. We show, however, that an…

Materials Science · Physics 2009-10-31 Ho-Soon Yang , Michael R. Geller , W. M. Dennis

We use the spin-polarized excitons in a single quantum dot to design optical controls for basic operations in quantum computing. We examine the ultrafast nonlinear optical processes required and use the coherent nonlinear optical responses…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Pochung Chen , C. Piermarocchi , L. J. Sham

The cross section of light absorption by semiconductor quantum dots in the case of the resonance with excitons $\Gamma_6 \times \Gamma_7$ in cubical crystals $T_d$ is calculated. It is shown that an interference of stimulating and induced…

Statistical Mechanics · Physics 2007-05-23 I. G. Lang , L. I. Korovin , S. T. Pavlov

A new microscopic approach to the optical transitions in quantum dots and quantum dot molecules, which accounts for both diagonal and non-diagonal exciton-phonon interaction, is developed. The cumulant expansion of the linear polarization…

Other Condensed Matter · Physics 2015-06-25 E. A. Muljarov , T. Takagahara , R. Zimmermann

Monolayers of transition metal dichalcogenides (TMDs) have been established in the last years as promising materials for novel optoelectronic devices. However, the performance of such devices is often limited by the dissociation of tightly…

Mesoscale and Nanoscale Physics · Physics 2024-02-13 Raul Perea-Causin , Samuel Brem , Ermin Malic

Organic molecules store the energy of absorbed light in the form of charge-neutral molecular excitations -- Frenkel excitons. Usually, in amorphous organic materials, excitons are viewed as quasiparticles, localized on single molecules,…

Mesoscale and Nanoscale Physics · Physics 2013-04-02 Semion K. Saikin , Alexander Eisfeld , Stéphanie Valleau , Alán Aspuru-Guzik

Nanostructured rare-earth-ion doped materials are increasingly being investigated for on-chip implementations of quantum information processing protocols as well as commercial applications such as fluorescent lighting. However, achieving…

Mesoscale and Nanoscale Physics · Physics 2018-09-12 Thomas Lutz , Lucile Veissier , Philip J. T. Woodburn , Rufus L. Cone , Paul E. Barclay , Wolfgang Tittel , Charles W. Thiel

We experimentally investigate the non-resonant feeding of photons into the optical mode of a zero dimensional nanocavity by quantum dot multiexciton transitions. Power dependent photoluminescence measurements reveal a super-linear power…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 A. Laucht , M. Kaniber , A. Mohtashami , N. Hauke , M. Bichler , J. J. Finley

The formation of excited dimer states, so called excimers, is an important phenomenon in many organic molecular semiconductors. In contrast to Frenkel exciton-polaron excited states, an excimer is long-lived and energetically low-lying due…

The intriguing physics of carrier-carrier interactions, which likewise affect the operation of light emitting devices, stimulate the research on semiconductor structures at high densities of excited carriers, a limit reachable at large…

Long-range and fast transport of coherent excitons is important for development of high-speed excitonic circuits and quantum computing applications. However, most of these coherent excitons have only been observed in some low-dimensional…

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