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Motivated by the recent synthesis of two insulating Li$_2$IrO$_3$ polymorphs, where Ir$^{4+}$ $S_{eff}$=1/2 moments form 3D ("harmonic") honeycomb structures with threefold coordination, we study magnetic Hamiltonians on the resulting…

Strongly Correlated Electrons · Physics 2014-11-26 Itamar Kimchi , James G. Analytis , Ashvin Vishwanath

Compounds of transition metal ions with strong spin-orbit coupling recently attracted attention due to the possibility to host frustrated bond-dependent anisotropic magnetic interactions. In general, such interactions lead to complex phase…

Strongly Correlated Electrons · Physics 2019-02-21 Juraj Rusnačko , Dorota Gotfryd , Jiří Chaloupka

We study the effective spin-orbital model for honeycomb-layered transition metal compounds, applying the second-order perturbation theory to the three-orbital Hubbard model with the anisotropic hoppings. This model is reduced to the Kitaev…

Strongly Correlated Electrons · Physics 2018-04-04 Akihisa Koga , Shiryu Nakauchi , Joji Nasu

The main question we address is how to probe the fractionalized excitations of a quantum spin liquid (QSL), for example, in the Kitaev honeycomb model. By analyzing the energy spectrum and entanglement entropy, for antiferromagnetic…

Strongly Correlated Electrons · Physics 2019-05-08 David C. Ronquillo , Adu Vengal , Nandini Trivedi

The honeycomb-lattice cobaltate Na$_3$Co$_2$SbO$_6$ has recently been proposed to be a proximate Kitaev quantum spin liquid~(QSL) candidate. However, non-Kitaev terms in the Hamiltonian lead to a zigzag-type antiferromagnetic~(AFM) order at…

Recent experimental evidence for a field-induced quantum spin liquid (QSL) in $\alpha$-RuCl$_3$ calls for an understanding for the ground state of honeycomb Kitaev model under a magnetic field. In this work we address the nature of an…

Strongly Correlated Electrons · Physics 2018-10-04 Hong-Chen Jiang , Chang-Yan Wang , Biao Huang , Yuan-Ming Lu

Kitaev exchange, a new paradigm in quantum magnetism research, occurs for 90$^{\circ}$ metal-ligand-metal links, $t_{2g}^5$ transition ions, and sizable spin-orbit coupling. It is being studied in honeycomb compounds but also on triangular…

Strongly Correlated Electrons · Physics 2023-10-11 Pritam Bhattacharyya , Nikolay A. Bogdanov , Satoshi Nishimoto , Stephen D. Wilson , Liviu Hozoi

Heisenberg interactions are ubiquitous in magnetic materials and have been prevailing in modeling and designing quantum magnets. Bond-directional interactions offer a novel alternative to Heisenberg exchange and provide the building blocks…

Very recently a quantum liquid was reported to form in H$_3$LiIr$_2$O$_6$, an iridate proposed to be a close realization of the Kitaev honeycomb model. To test this assertion we perform detailed quantum chemistry calculations to determine…

Strongly Correlated Electrons · Physics 2018-11-13 Ravi Yadav , Rajyavardhan Ray , Mohamed S. Eldeeb , Satoshi Nishimoto , Liviu Hozoi , Jeroen van den Brink

Kitaev quantum spin liquid, massively quantum entangled states, is so scarce in nature that searching for new candidate systems remains a great challenge. Honeycomb heterostructure could be a promising route to realize and utilize such an…

Recent experiments reveal that the honeycomb ruthenium trichloride {\alpha}-RuCl3 is a prime candidate of the Kitaev quantum spin liquid (QSL). However, there is no theoretical model which can properly describe its experimental dynamical…

Strongly Correlated Electrons · Physics 2017-08-16 Y. S. Hou , H. J. Xiang , X. G. Gong

Due to the combination of a substantial spin-orbit coupling and correlation effects, iridium oxides hold a prominent place in the search for novel quantum states of matter, including, e.g., Kitaev spin liquids and topological Weyl states.…

Strongly Correlated Electrons · Physics 2017-07-11 Vamshi M. Katukuri , Ravi Yadav , Liviu Hozoi , Satoshi Nishimoto , Jeroen van den Brink

The electronic ground state in many iridate materials is described by a complex wave-function in which spin and orbital angular momenta are entangled due to relativistic spin-orbit coupling (SOC). Such a localized electronic state carries…

The S=3/2 Kitaev honeycomb model (KHM) is a quantum spin liquid (QSL) state coupled to a static Z$_2$ gauge field. Employing an SO(6) Majorana representation of spin 3/2's, we find an exact representation of the conserved plaquette fluxes…

Strongly Correlated Electrons · Physics 2022-07-07 Hui-Ke Jin , W. M. H. Natori , F. Pollmann , J. Knolle

This paper reviews the current progress on searching the Kitaev spin liquid state in 3d electron systems. Honeycomb cobaltates were recently proposed as promising candidates to realize the Kitaev spin liquid state, due to the more localized…

Strongly Correlated Electrons · Physics 2021-10-05 Huimei Liu

In $\alpha$-RuCl$_3$, an external magnetic field applied within the honeycomb plane can induce a transition from a magnetically ordered state to a disordered state that is potentially related to the Kitaev quantum spin liquid. In zero…

Recently, layered honeycomb cobaltates have been predicted as a new promising system for realizing the Kitaev quantum spin liquid, a many-body quantum entangled ground state characterized by fractional excitations. However, these…

Competition and cooperation between electron correlation and relativistic spin-orbit coupling give rise to diverse exotic quantum phenomena in solids. An illustrative example is spin-orbit entangled quantum liquids, which exhibit remarkable…

Strongly Correlated Electrons · Physics 2024-03-15 Yi-Feng Zhao , Seong-Hoon Jang , Yukitoshi Motome

The Kitaev honeycomb model has received significant attention for its exactly solvable quantum spin liquid ground states and fractionalized excitations. For realizing the model, layered cobalt oxides have been considered a promising…

Strongly Correlated Electrons · Physics 2025-01-27 Yuchen Gu , Xianghong Jin , Yuan Li

Topological spin liquids in two spatial dimensions are stable phases in the presence of a small magnetic field, but may give way to field-induced phenomena at intermediate field strengths. Sandwiched between the low-field spin liquid…

Strongly Correlated Electrons · Physics 2021-02-17 Ciarán Hickey , Matthias Gohlke , Christoph Berke , Simon Trebst
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